[CP2K-user] [CP2K:20173] Re: Vibrational Analysis

Marcella Iannuzzi marci.akira at gmail.com
Sun May 5 10:02:40 UTC 2024


It is not possible to calculate this property with this method for your 
system with cp2k!

On Sunday, May 5, 2024 at 11:54:24 AM UTC+2 rafiq... at gmail.com wrote:

> (Please check my input file, when i remove the pbc then my system will not 
> treat as periodic) so what should i change in my input please consider my 
> input , thanks for your response
>
> &GLOBAL
>   PROJECT MoP100-44-pos-1
>   PRINT_LEVEL LOW
>   RUN_TYPE VIBRATIONAL_ANALYSIS
> &END GLOBAL
>
> &FORCE_EVAL
>   METHOD Quickstep
>   &SUBSYS
>     &CELL
>       A    12.87500000     0.00000000     0.00000000
>       B     6.43800000    11.15094310     0.00000000
>       C     0.00000000     0.00000000    31.10900000
>       PERIODIC XYZ 
>     &END CELL
>     &COORD
>       Mo          3.21900000    1.85900000    1.58700000
>       Mo          3.21900000    1.85900000    4.76100000
>       Mo          3.21900000    1.85900000    7.93500000
>       Mo          3.21900000    1.85900000   11.00400000
>       P           0.00000000    0.00000000    0.00000000
>       P           0.00000000    0.00000000    3.17400000
>       P           0.00000000    0.00000000    6.34800000
>       P          12.87500000    0.00000000    9.58600000
>       Mo          6.43800000    1.85900000    1.58700000
>       Mo          6.43800000    1.85900000    4.76100000
>       Mo          6.43800000    1.85900000    7.93500000
>       Mo          6.43800000    1.85900000   11.00400000
>       P           3.21900000    0.00000000    0.00000000
>       P           3.21900000    0.00000000    3.17400000
>       P           3.21900000    0.00000000    6.34800000
>       P           3.21900000    0.00000000    9.58600000
>       Mo          9.65600000    1.85900000    1.58700000
>       Mo          9.65600000    1.85900000    4.76100000
>       Mo          9.65600000    1.85900000    7.93500000
>       Mo          9.65600000    1.85900000   11.00400000
>       P           6.43800000    0.00000000    0.00000000
>       P           6.43800000    0.00000000    3.17400000
>       P           6.43800000    0.00000000    6.34800000
>       P           6.43800000    0.00000000    9.58600000
>       Mo         12.87500000    1.85900000    1.58700000
>       Mo         12.87500000    1.85900000    4.76100000
>       Mo         12.87500000    1.85900000    7.93500000
>       Mo         12.87500000    1.85900000   11.00400000
>       P           9.65600000    0.00000000    0.00000000
>       P           9.65600000    0.00000000    3.17400000
>       P           9.65600000    0.00000000    6.34800000
>       P           9.65600000    0.00000000    9.58600000
>       Mo          4.82800000    4.64600000    1.58700000
>       Mo          4.82800000    4.64600000    4.76100000
>       Mo          4.82800000    4.64600000    7.93500000
>       Mo          4.82800000    4.64600000   11.00400000
>       P           1.60900000    2.78800000    0.00000000
>       P           1.60900000    2.78800000    3.17400000
>       P           1.60900000    2.78800000    6.34800000
>       P          14.48500000    2.78800000    9.58600000
>       Mo          8.04700000    4.64600000    1.58700000
>       Mo          8.04700000    4.64600000    4.76100000
>       Mo          8.04700000    4.64600000    7.93500000
>       Mo          8.04700000    4.64600000   11.00400000
>       P           4.82800000    2.78800000    0.00000000
>       P           4.82800000    2.78800000    3.17400000
>       P           4.82800000    2.78800000    6.34800000
>       P           4.82800000    2.78800000    9.58600000
>       Mo         11.26600000    4.64600000    1.58700000
>       Mo         11.26600000    4.64600000    4.76100000
>       Mo         11.26600000    4.64600000    7.93500000
>       Mo         11.26600000    4.64600000   11.00400000
>       P           8.04700000    2.78800000    0.00000000
>       P           8.04700000    2.78800000    3.17400000
>       P           8.04700000    2.78800000    6.34800000
>       P           8.04700000    2.78800000    9.58600000
>       Mo         14.48500000    4.64600000    1.58700000
>       Mo         14.48500000    4.64600000    4.76100000
>       Mo         14.48500000    4.64600000    7.93500000
>       Mo         14.48500000    4.64600000   11.00400000
>       P          11.26600000    2.78800000    0.00000000
>       P          11.26600000    2.78800000    3.17400000
>       P          11.26600000    2.78800000    6.34800000
>       P          11.26600000    2.78800000    9.58600000
>       Mo          6.43800000    7.43400000    1.58700000
>       Mo          6.43800000    7.43400000    4.76100000
>       Mo          6.43800000    7.43400000    7.93500000
>       Mo          6.43800000    7.43400000   11.00400000
>       P           3.21900000    5.57600000    0.00000000
>       P           3.21900000    5.57600000    3.17400000
>       P           3.21900000    5.57600000    6.34800000
>       P           3.21900000    5.57600000    9.58600000
>       Mo          9.65600000    7.43400000    1.58700000
>       Mo          9.65600000    7.43400000    4.76100000
>       Mo          9.65600000    7.43400000    7.93500000
>       Mo          9.65600000    7.43400000   11.00400000
>       P           6.43800000    5.57600000    0.00000000
>       P           6.43800000    5.57600000    3.17400000
>       P           6.43800000    5.57600000    6.34800000
>       P           6.43800000    5.57600000    9.58600000
>       Mo         12.87500000    7.43400000    1.58700000
>       Mo         12.87500000    7.43400000    4.76100000
>       Mo         12.87500000    7.43400000    7.93500000
>       Mo         12.87500000    7.43400000   11.00400000
>       P           9.65600000    5.57600000    0.00000000
>       P           9.65600000    5.57600000    3.17400000
>       P           9.65600000    5.57600000    6.34800000
>       P           9.65600000    5.57600000    9.58600000
>       Mo         16.09400000    7.43400000    1.58700000
>       Mo         16.09400000    7.43400000    4.76100000
>       Mo         16.09400000    7.43400000    7.93500000
>       Mo         16.09400000    7.43400000   11.00400000
>       P          12.87500000    5.57600000    0.00000000
>       P          12.87500000    5.57600000    3.17400000
>       P          12.87500000    5.57600000    6.34800000
>       P          12.87500000    5.57600000    9.58600000
>       Mo          8.04700000   10.22200000    1.58700000
>       Mo          8.04700000   10.22200000    4.76100000
>       Mo          8.04700000   10.22200000    7.93500000
>       Mo          8.04700000   10.22200000   11.00400000
>       P           4.82800000    8.36300000    0.00000000
>       P          17.70300000    8.36300000    3.17400000
>       P          17.70300000    8.36300000    6.34800000
>       P           4.82800000    8.36300000    9.58600000
>       Mo         11.26600000   10.22200000    1.58700000
>       Mo         11.26600000   10.22200000    4.76100000
>       Mo         11.26600000   10.22200000    7.93500000
>       Mo         11.26600000   10.22200000   11.00400000
>       P           8.04700000    8.36300000    0.00000000
>       P           8.04700000    8.36300000    3.17400000
>       P           8.04700000    8.36300000    6.34800000
>       P           8.04700000    8.36300000    9.58600000
>       Mo         14.48500000   10.22200000    1.58700000
>       Mo         14.48500000   10.22200000    4.76100000
>       Mo         14.48500000   10.22200000    7.93500000
>       Mo         14.48500000   10.22200000   11.00400000
>       P          11.26600000    8.36300000    0.00000000
>       P          11.26600000    8.36300000    3.17400000
>       P          11.26600000    8.36300000    6.34800000
>       P          11.26600000    8.36300000    9.58600000
>       Mo         17.70300000   10.22200000    1.58700000
>       Mo         17.70300000   10.22200000    4.76100000
>       Mo         17.70300000   10.22200000    7.93500000
>       Mo         17.70300000   10.22200000   11.00400000
>       P          14.48500000    8.36300000    0.00000000
>       P          14.48500000    8.36300000    3.17400000
>       P          14.48500000    8.36300000    6.34800000
>       P          14.48500000    8.36300000    9.58600000
>     &END COORD
>     &KIND Mo
>       ELEMENT Mo
>       BASIS_SET DZVP-MOLOPT-SR-GTH-q14
>       POTENTIAL GTH-PBE
>     &END KIND
>     &KIND P
>       ELEMENT P
>       BASIS_SET DZVP-MOLOPT-SR-GTH-q5
>       POTENTIAL GTH-PBE
>     &END KIND
>   &END SUBSYS
>
>   &DFT
>     BASIS_SET_FILE_NAME  BASIS_MOLOPT
>     POTENTIAL_FILE_NAME  POTENTIAL
> #   WFN_RESTART_FILE_NAME MoP100-44-pos-1-RESTART.kp
>     CHARGE    0 
>     MULTIPLICITY    1 
>     &KPOINTS
>       SCHEME MONKHORST-PACK  3  3  1
>     &END KPOINTS
>     &QS
>       EPS_DEFAULT 1.0E-12 
> #     EXTRAPOLATION USE_PREV_P 
>     &END QS
>     &POISSON
>       PERIODIC XYZ 
>       PSOLVER PERIODIC 
>     &END POISSON
>     &XC
>       &XC_FUNCTIONAL PBE
>       &END XC_FUNCTIONAL
>       &VDW_POTENTIAL
>         POTENTIAL_TYPE PAIR_POTENTIAL
>         &PAIR_POTENTIAL
>           PARAMETER_FILE_NAME dftd3.dat
>           TYPE DFTD3(BJ)
>           REFERENCE_FUNCTIONAL PBE
>           #CALCULATE_C9_TERM T 
>         &END PAIR_POTENTIAL
>       &END VDW_POTENTIAL
>     &END XC
>     &MGRID
>       CUTOFF  500
>       REL_CUTOFF  65
>     &END MGRID
>     &SCF
>       MAX_SCF 300
>       EPS_SCF 1.0E-8 
> #     SCF_GUESS RESTART 
> #     IGNORE_CONVERGENCE_FAILURE 
>       &DIAGONALIZATION
>         ALGORITHM STANDARD 
>       &END DIAGONALIZATION
>       &MIXING 
>         METHOD BROYDEN_MIXING
>         ALPHA 0.4 
>         NBROYDEN 8 
>       &END MIXING
>       &SMEAR
>         METHOD FERMI_DIRAC
>         ELECTRONIC_TEMPERATURE 300 
>       &END SMEAR
>       ADDED_MOS    64 
>       &PRINT
>         &RESTART 
> BACKUP_COPIES 0 
>         &END RESTART
>       &END PRINT
>     &END SCF
>    &END DFT
> &END FORCE_EVAL
>
> &MOTION
>   &CONSTRAINT
>     &FIXED_ATOMS 
>       COMPONENTS_TO_FIX XYZ 
>       LIST 1 2 3 5 6 7 9 10 11 13 14 15 17 18 19 21 22 23 25 26 27 29 30 
> 31 33 34 35 37 38 39 41 42 43 45 46 47 49 50 51 53 54 55 57 58 59 61 62 63 
> 65 66 67 69 70 71 73 74 75 77 78 79 81 82 83 85 86 87 89 90 91 93 94 95 97 
> 98 99 101 102 103 105 106 107 109 110 111 113 114 115 117 118 119 121 122 
> 123 125 126 127
>     &END FIXED_ATOMS
>   &END CONSTRAINT
>   &PRINT
>     &RESTART
>       BACKUP_COPIES 0 
>     &END RESTART
>   &END PRINT
> &END MOTION
> &VIBRATIONAL_ANALYSIS
>   DX 0.1 
>   NPROC_REP 60 
>   TC_PRESSURE 101325
>   TC_TEMPERATURE 298.15 
>   THERMOCHEMISTRY T 
>   INTENSITIES T 
>   FULLY_PERIODIC T 
>   &PRINT
>     &MOLDEN_VIB 
>     &END MOLDEN_VIB
>   &END PRINT
> &END VIBRATIONAL_ANALYSIS
>
> On Sunday, May 5, 2024 at 5:18:00 PM UTC+8 Marcella Iannuzzi wrote:
>
>> Hi ....
>>
>> This property is calculated only for molecule in gas phase, and not when 
>> PBC are used
>> Regards
>> Marcella
>>
>> On Saturday, May 4, 2024 at 4:27:07 PM UTC+2 rafiq... at gmail.com wrote:
>>
>>> Like what should I write in input file for thermochemistry calculation?
>>>
>>> On Sat, 4 May 2024, 9:32 pm Marcella Iannuzzi, <marci... at gmail.com> 
>>> wrote:
>>>
>>>> Hi...
>>>>
>>>>
>>>> THERMOCHEMISTRY*: logical**= F* 
>>>> <https://manual.cp2k.org/trunk/CP2K_INPUT/VIBRATIONAL_ANALYSIS.html#CP2K_INPUT.VIBRATIONAL_ANALYSIS.THERMOCHEMISTRY>
>>>>
>>>> *Lone keyword:* T
>>>>
>>>> Calculation of the thermochemical data. *Valid for molecules in the 
>>>> gas phase.*
>>>>
>>>>
>>>> Regards
>>>>
>>>> Marcella
>>>> On Friday, May 3, 2024 at 2:23:20 PM UTC+2 rafiq... at gmail.com wrote:
>>>>
>>>>> &VIBRATIONAL_ANALYSIS
>>>>>   DX 0.1 
>>>>>   NPROC_REP 48
>>>>>   TC_PRESSURE 101325 
>>>>>   TC_TEMPERATURE 298.15 
>>>>>   THERMOCHEMISTRY T
>>>>>   FULLY_PERIODIC T
>>>>> &END VIBRATIONAL_ANALYSIS
>>>>>
>>>>> Why in output file no thermochemistry? See my output file.
>>>>>
>>>>> VIB|                       142                  143                 
>>>>>  144
>>>>>  VIB|Frequency (cm^-1)   439.322414           439.460912           
>>>>> 445.868786
>>>>>  VIB|Red.Masses (a.u.)    34.271393            34.269852           
>>>>>  34.289785
>>>>>  VIB|Frc consts (a.u.)     0.003268             0.003272             
>>>>> 0.003469
>>>>>   ATOM  EL             X     Y     Z        X     Y     Z        X     
>>>>> Y     Z  
>>>>>      3  Mo            0.01 -0.00  0.02    -0.00  0.00  0.03    -0.00 
>>>>> -0.00 -0.03
>>>>>      4  Mo            0.02 -0.00 -0.03    -0.00  0.01 -0.07     0.00 
>>>>>  0.00 -0.05
>>>>>      8  P            -0.28  0.04  0.00     0.08 -0.17  0.00     0.00 
>>>>>  0.00  0.24
>>>>>     11  Mo           -0.01 -0.00 -0.00     0.00 -0.00 -0.03    -0.00 
>>>>> -0.00 -0.03
>>>>>     12  Mo           -0.02 -0.01  0.00     0.00 -0.01  0.07     0.00 
>>>>>  0.00 -0.05
>>>>>     16  P             0.28  0.12  0.00    -0.08  0.17 -0.00     0.00 
>>>>>  0.00  0.24
>>>>>     19  Mo            0.01 -0.00  0.02    -0.00  0.00  0.03     0.00 
>>>>> -0.00 -0.03
>>>>>     20  Mo            0.02 -0.00 -0.03    -0.00  0.01 -0.07    -0.00 
>>>>>  0.00 -0.05
>>>>>     24  P            -0.28  0.04  0.00     0.08 -0.16  0.00     0.00 
>>>>> -0.00  0.24
>>>>>     27  Mo           -0.01 -0.00 -0.00     0.00 -0.00 -0.03     0.00 
>>>>> -0.00 -0.03
>>>>>     28  Mo           -0.02 -0.01  0.00     0.00 -0.01  0.07    -0.00 
>>>>>  0.00 -0.05
>>>>>     32  P             0.28  0.12 -0.00    -0.08  0.16 -0.01    -0.00 
>>>>> -0.00  0.24
>>>>>     35  Mo           -0.00 -0.00 -0.04    -0.01  0.00  0.01     0.00 
>>>>>  0.00 -0.03
>>>>>     36  Mo           -0.00 -0.00  0.08    -0.02  0.00 -0.02    -0.00 
>>>>> -0.00 -0.05
>>>>>     40  P             0.07  0.08 -0.01     0.29 -0.04  0.00     0.00 
>>>>> -0.00  0.24
>>>>>     43  Mo            0.00  0.00  0.02     0.01 -0.00 -0.01     0.00 
>>>>>  0.00 -0.03
>>>>>     44  Mo            0.00  0.01 -0.05     0.02 -0.00  0.02    -0.00 
>>>>> -0.00 -0.05
>>>>>     48  P            -0.07 -0.24  0.00    -0.29  0.04  0.00    -0.00 
>>>>> -0.00  0.24
>>>>>     51  Mo           -0.00 -0.00 -0.04    -0.01  0.00  0.01     0.00 
>>>>>  0.00 -0.03
>>>>>     52  Mo           -0.00 -0.00  0.08    -0.02  0.00 -0.02     0.00 
>>>>> -0.00 -0.05
>>>>>     56  P             0.07  0.08 -0.01     0.29 -0.04  0.00     0.00 
>>>>> -0.00  0.25
>>>>>     59  Mo            0.00  0.00  0.02     0.01 -0.00 -0.01    -0.00 
>>>>>  0.00 -0.03
>>>>>     60  Mo            0.00  0.01 -0.05     0.02 -0.00  0.02     0.00 
>>>>> -0.00 -0.05
>>>>>     64  P            -0.07 -0.24  0.00    -0.29  0.04 -0.00     0.00 
>>>>>  0.00  0.24
>>>>>     67  Mo            0.01 -0.00  0.02    -0.00  0.00  0.03    -0.00 
>>>>> -0.00 -0.03
>>>>>     68  Mo            0.02 -0.00 -0.03    -0.00  0.01 -0.07     0.00 
>>>>> -0.00 -0.05
>>>>>     72  P            -0.27  0.04  0.00     0.07 -0.17  0.00     0.00 
>>>>>  0.00  0.24
>>>>>     75  Mo           -0.01 -0.00 -0.00     0.00 -0.00 -0.03     0.00 
>>>>> -0.00 -0.03
>>>>>     76  Mo           -0.02 -0.01  0.00     0.00 -0.01  0.07    -0.00 
>>>>> -0.00 -0.05
>>>>>     80  P             0.27  0.12  0.00    -0.07  0.17 -0.00     0.00 
>>>>>  0.00  0.24
>>>>>     83  Mo            0.01 -0.00  0.02    -0.00  0.00  0.03    -0.00 
>>>>> -0.00 -0.03
>>>>>     84  Mo            0.02 -0.00 -0.03    -0.00  0.01 -0.07    -0.00 
>>>>> -0.00 -0.05
>>>>>     88  P            -0.27  0.04  0.00     0.07 -0.17  0.00    -0.00 
>>>>>  0.00  0.24
>>>>>     91  Mo           -0.01 -0.00 -0.00     0.00 -0.00 -0.03     0.00 
>>>>>  0.00 -0.03
>>>>>     92  Mo           -0.02 -0.01  0.00     0.00 -0.01  0.07     0.00 
>>>>> -0.00 -0.05
>>>>>     96  P             0.27  0.12 -0.00    -0.07  0.17 -0.00    -0.00 
>>>>>  0.00  0.24
>>>>>     99  Mo           -0.00 -0.00 -0.04    -0.01  0.00  0.01    -0.00 
>>>>>  0.00 -0.03
>>>>>    100  Mo           -0.00 -0.00  0.08    -0.02  0.00 -0.02    -0.00 
>>>>>  0.00 -0.05
>>>>>    104  P             0.07  0.08 -0.01     0.29 -0.04 -0.00    -0.00 
>>>>> -0.00  0.24
>>>>>    107  Mo            0.00  0.01  0.02     0.01 -0.00 -0.01     0.00 
>>>>>  0.00 -0.03
>>>>>    108  Mo            0.00  0.01 -0.05     0.02 -0.00  0.02    -0.00 
>>>>>  0.00 -0.05
>>>>>    112  P            -0.07 -0.24  0.00    -0.29  0.04 -0.00    -0.00 
>>>>> -0.00  0.24
>>>>>    115  Mo           -0.00 -0.00 -0.04    -0.01  0.00  0.01    -0.00 
>>>>> -0.00 -0.03
>>>>>    116  Mo           -0.00 -0.00  0.08    -0.02  0.00 -0.02     0.00 
>>>>>  0.00 -0.05
>>>>>    120  P             0.07  0.08 -0.00     0.29 -0.05  0.00     0.00 
>>>>> -0.00  0.24
>>>>>    123  Mo            0.00  0.01  0.02     0.01 -0.00 -0.01     0.00 
>>>>>  0.00 -0.03
>>>>>    124  Mo            0.00  0.01 -0.05     0.02 -0.00  0.02    -0.00 
>>>>> -0.00 -0.05
>>>>>    128  P            -0.07 -0.24  0.00    -0.29  0.05 -0.00     0.00 
>>>>> -0.00  0.24
>>>>>
>>>>>
>>>>>
>>>>>
>>>>>  -------------------------------------------------------------------------------
>>>>>  -                                                                     
>>>>>         -
>>>>>  -                                DBCSR STATISTICS                     
>>>>>         -
>>>>>  -                                                                     
>>>>>         -
>>>>>
>>>>>  -------------------------------------------------------------------------------
>>>>>  COUNTER                                    TOTAL       BLAS       SMM 
>>>>>       ACC
>>>>>  flops inhomo. stacks                           0       0.0%      0.0% 
>>>>>      0.0%
>>>>>  flops total                         0.000000E+00       0.0%      0.0% 
>>>>>      0.0%
>>>>>  flops max/rank                      0.000000E+00       0.0%      0.0% 
>>>>>      0.0%
>>>>>  matmuls inhomo. stacks                         0       0.0%      0.0% 
>>>>>      0.0%
>>>>>  matmuls total                                  0       0.0%      0.0% 
>>>>>      0.0%
>>>>>  number of processed stacks                     0       0.0%      0.0% 
>>>>>      0.0%
>>>>>  average stack size                                     0.0       0.0 
>>>>>       0.0
>>>>>  marketing flops                     0.000000E+00
>>>>>
>>>>>  -------------------------------------------------------------------------------
>>>>>  -                                                                     
>>>>>         -
>>>>>  -                      DBCSR MESSAGE PASSING PERFORMANCE             
>>>>>          -
>>>>>  -                                                                     
>>>>>         -
>>>>>
>>>>>  -------------------------------------------------------------------------------
>>>>>  ROUTINE             CALLS      AVE VOLUME [Bytes]
>>>>>  MP_Bcast                1                     12.
>>>>>  MP_Allreduce      1316782                      8.
>>>>>  MP_Alltoall      12045666                 733641.
>>>>>
>>>>>  -------------------------------------------------------------------------------
>>>>>
>>>>> -- 
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