[CP2K-user] [CP2K:20174] Re: Vibrational Analysis

Muhammad Rafiq rafiq789.ra at gmail.com
Sun May 5 10:23:06 UTC 2024


so what should i do, which method i use


On Sunday, May 5, 2024 at 6:02:40 PM UTC+8 Marcella Iannuzzi wrote:

> It is not possible to calculate this property with this method for your 
> system with cp2k!
>
> On Sunday, May 5, 2024 at 11:54:24 AM UTC+2 rafiq... at gmail.com wrote:
>
>> (Please check my input file, when i remove the pbc then my system will 
>> not treat as periodic) so what should i change in my input please consider 
>> my input , thanks for your response
>>
>> &GLOBAL
>>   PROJECT MoP100-44-pos-1
>>   PRINT_LEVEL LOW
>>   RUN_TYPE VIBRATIONAL_ANALYSIS
>> &END GLOBAL
>>
>> &FORCE_EVAL
>>   METHOD Quickstep
>>   &SUBSYS
>>     &CELL
>>       A    12.87500000     0.00000000     0.00000000
>>       B     6.43800000    11.15094310     0.00000000
>>       C     0.00000000     0.00000000    31.10900000
>>       PERIODIC XYZ 
>>     &END CELL
>>     &COORD
>>       Mo          3.21900000    1.85900000    1.58700000
>>       Mo          3.21900000    1.85900000    4.76100000
>>       Mo          3.21900000    1.85900000    7.93500000
>>       Mo          3.21900000    1.85900000   11.00400000
>>       P           0.00000000    0.00000000    0.00000000
>>       P           0.00000000    0.00000000    3.17400000
>>       P           0.00000000    0.00000000    6.34800000
>>       P          12.87500000    0.00000000    9.58600000
>>       Mo          6.43800000    1.85900000    1.58700000
>>       Mo          6.43800000    1.85900000    4.76100000
>>       Mo          6.43800000    1.85900000    7.93500000
>>       Mo          6.43800000    1.85900000   11.00400000
>>       P           3.21900000    0.00000000    0.00000000
>>       P           3.21900000    0.00000000    3.17400000
>>       P           3.21900000    0.00000000    6.34800000
>>       P           3.21900000    0.00000000    9.58600000
>>       Mo          9.65600000    1.85900000    1.58700000
>>       Mo          9.65600000    1.85900000    4.76100000
>>       Mo          9.65600000    1.85900000    7.93500000
>>       Mo          9.65600000    1.85900000   11.00400000
>>       P           6.43800000    0.00000000    0.00000000
>>       P           6.43800000    0.00000000    3.17400000
>>       P           6.43800000    0.00000000    6.34800000
>>       P           6.43800000    0.00000000    9.58600000
>>       Mo         12.87500000    1.85900000    1.58700000
>>       Mo         12.87500000    1.85900000    4.76100000
>>       Mo         12.87500000    1.85900000    7.93500000
>>       Mo         12.87500000    1.85900000   11.00400000
>>       P           9.65600000    0.00000000    0.00000000
>>       P           9.65600000    0.00000000    3.17400000
>>       P           9.65600000    0.00000000    6.34800000
>>       P           9.65600000    0.00000000    9.58600000
>>       Mo          4.82800000    4.64600000    1.58700000
>>       Mo          4.82800000    4.64600000    4.76100000
>>       Mo          4.82800000    4.64600000    7.93500000
>>       Mo          4.82800000    4.64600000   11.00400000
>>       P           1.60900000    2.78800000    0.00000000
>>       P           1.60900000    2.78800000    3.17400000
>>       P           1.60900000    2.78800000    6.34800000
>>       P          14.48500000    2.78800000    9.58600000
>>       Mo          8.04700000    4.64600000    1.58700000
>>       Mo          8.04700000    4.64600000    4.76100000
>>       Mo          8.04700000    4.64600000    7.93500000
>>       Mo          8.04700000    4.64600000   11.00400000
>>       P           4.82800000    2.78800000    0.00000000
>>       P           4.82800000    2.78800000    3.17400000
>>       P           4.82800000    2.78800000    6.34800000
>>       P           4.82800000    2.78800000    9.58600000
>>       Mo         11.26600000    4.64600000    1.58700000
>>       Mo         11.26600000    4.64600000    4.76100000
>>       Mo         11.26600000    4.64600000    7.93500000
>>       Mo         11.26600000    4.64600000   11.00400000
>>       P           8.04700000    2.78800000    0.00000000
>>       P           8.04700000    2.78800000    3.17400000
>>       P           8.04700000    2.78800000    6.34800000
>>       P           8.04700000    2.78800000    9.58600000
>>       Mo         14.48500000    4.64600000    1.58700000
>>       Mo         14.48500000    4.64600000    4.76100000
>>       Mo         14.48500000    4.64600000    7.93500000
>>       Mo         14.48500000    4.64600000   11.00400000
>>       P          11.26600000    2.78800000    0.00000000
>>       P          11.26600000    2.78800000    3.17400000
>>       P          11.26600000    2.78800000    6.34800000
>>       P          11.26600000    2.78800000    9.58600000
>>       Mo          6.43800000    7.43400000    1.58700000
>>       Mo          6.43800000    7.43400000    4.76100000
>>       Mo          6.43800000    7.43400000    7.93500000
>>       Mo          6.43800000    7.43400000   11.00400000
>>       P           3.21900000    5.57600000    0.00000000
>>       P           3.21900000    5.57600000    3.17400000
>>       P           3.21900000    5.57600000    6.34800000
>>       P           3.21900000    5.57600000    9.58600000
>>       Mo          9.65600000    7.43400000    1.58700000
>>       Mo          9.65600000    7.43400000    4.76100000
>>       Mo          9.65600000    7.43400000    7.93500000
>>       Mo          9.65600000    7.43400000   11.00400000
>>       P           6.43800000    5.57600000    0.00000000
>>       P           6.43800000    5.57600000    3.17400000
>>       P           6.43800000    5.57600000    6.34800000
>>       P           6.43800000    5.57600000    9.58600000
>>       Mo         12.87500000    7.43400000    1.58700000
>>       Mo         12.87500000    7.43400000    4.76100000
>>       Mo         12.87500000    7.43400000    7.93500000
>>       Mo         12.87500000    7.43400000   11.00400000
>>       P           9.65600000    5.57600000    0.00000000
>>       P           9.65600000    5.57600000    3.17400000
>>       P           9.65600000    5.57600000    6.34800000
>>       P           9.65600000    5.57600000    9.58600000
>>       Mo         16.09400000    7.43400000    1.58700000
>>       Mo         16.09400000    7.43400000    4.76100000
>>       Mo         16.09400000    7.43400000    7.93500000
>>       Mo         16.09400000    7.43400000   11.00400000
>>       P          12.87500000    5.57600000    0.00000000
>>       P          12.87500000    5.57600000    3.17400000
>>       P          12.87500000    5.57600000    6.34800000
>>       P          12.87500000    5.57600000    9.58600000
>>       Mo          8.04700000   10.22200000    1.58700000
>>       Mo          8.04700000   10.22200000    4.76100000
>>       Mo          8.04700000   10.22200000    7.93500000
>>       Mo          8.04700000   10.22200000   11.00400000
>>       P           4.82800000    8.36300000    0.00000000
>>       P          17.70300000    8.36300000    3.17400000
>>       P          17.70300000    8.36300000    6.34800000
>>       P           4.82800000    8.36300000    9.58600000
>>       Mo         11.26600000   10.22200000    1.58700000
>>       Mo         11.26600000   10.22200000    4.76100000
>>       Mo         11.26600000   10.22200000    7.93500000
>>       Mo         11.26600000   10.22200000   11.00400000
>>       P           8.04700000    8.36300000    0.00000000
>>       P           8.04700000    8.36300000    3.17400000
>>       P           8.04700000    8.36300000    6.34800000
>>       P           8.04700000    8.36300000    9.58600000
>>       Mo         14.48500000   10.22200000    1.58700000
>>       Mo         14.48500000   10.22200000    4.76100000
>>       Mo         14.48500000   10.22200000    7.93500000
>>       Mo         14.48500000   10.22200000   11.00400000
>>       P          11.26600000    8.36300000    0.00000000
>>       P          11.26600000    8.36300000    3.17400000
>>       P          11.26600000    8.36300000    6.34800000
>>       P          11.26600000    8.36300000    9.58600000
>>       Mo         17.70300000   10.22200000    1.58700000
>>       Mo         17.70300000   10.22200000    4.76100000
>>       Mo         17.70300000   10.22200000    7.93500000
>>       Mo         17.70300000   10.22200000   11.00400000
>>       P          14.48500000    8.36300000    0.00000000
>>       P          14.48500000    8.36300000    3.17400000
>>       P          14.48500000    8.36300000    6.34800000
>>       P          14.48500000    8.36300000    9.58600000
>>     &END COORD
>>     &KIND Mo
>>       ELEMENT Mo
>>       BASIS_SET DZVP-MOLOPT-SR-GTH-q14
>>       POTENTIAL GTH-PBE
>>     &END KIND
>>     &KIND P
>>       ELEMENT P
>>       BASIS_SET DZVP-MOLOPT-SR-GTH-q5
>>       POTENTIAL GTH-PBE
>>     &END KIND
>>   &END SUBSYS
>>
>>   &DFT
>>     BASIS_SET_FILE_NAME  BASIS_MOLOPT
>>     POTENTIAL_FILE_NAME  POTENTIAL
>> #   WFN_RESTART_FILE_NAME MoP100-44-pos-1-RESTART.kp
>>     CHARGE    0 
>>     MULTIPLICITY    1 
>>     &KPOINTS
>>       SCHEME MONKHORST-PACK  3  3  1
>>     &END KPOINTS
>>     &QS
>>       EPS_DEFAULT 1.0E-12 
>> #     EXTRAPOLATION USE_PREV_P 
>>     &END QS
>>     &POISSON
>>       PERIODIC XYZ 
>>       PSOLVER PERIODIC 
>>     &END POISSON
>>     &XC
>>       &XC_FUNCTIONAL PBE
>>       &END XC_FUNCTIONAL
>>       &VDW_POTENTIAL
>>         POTENTIAL_TYPE PAIR_POTENTIAL
>>         &PAIR_POTENTIAL
>>           PARAMETER_FILE_NAME dftd3.dat
>>           TYPE DFTD3(BJ)
>>           REFERENCE_FUNCTIONAL PBE
>>           #CALCULATE_C9_TERM T 
>>         &END PAIR_POTENTIAL
>>       &END VDW_POTENTIAL
>>     &END XC
>>     &MGRID
>>       CUTOFF  500
>>       REL_CUTOFF  65
>>     &END MGRID
>>     &SCF
>>       MAX_SCF 300
>>       EPS_SCF 1.0E-8 
>> #     SCF_GUESS RESTART 
>> #     IGNORE_CONVERGENCE_FAILURE 
>>       &DIAGONALIZATION
>>         ALGORITHM STANDARD 
>>       &END DIAGONALIZATION
>>       &MIXING 
>>         METHOD BROYDEN_MIXING
>>         ALPHA 0.4 
>>         NBROYDEN 8 
>>       &END MIXING
>>       &SMEAR
>>         METHOD FERMI_DIRAC
>>         ELECTRONIC_TEMPERATURE 300 
>>       &END SMEAR
>>       ADDED_MOS    64 
>>       &PRINT
>>         &RESTART 
>> BACKUP_COPIES 0 
>>         &END RESTART
>>       &END PRINT
>>     &END SCF
>>    &END DFT
>> &END FORCE_EVAL
>>
>> &MOTION
>>   &CONSTRAINT
>>     &FIXED_ATOMS 
>>       COMPONENTS_TO_FIX XYZ 
>>       LIST 1 2 3 5 6 7 9 10 11 13 14 15 17 18 19 21 22 23 25 26 27 29 30 
>> 31 33 34 35 37 38 39 41 42 43 45 46 47 49 50 51 53 54 55 57 58 59 61 62 63 
>> 65 66 67 69 70 71 73 74 75 77 78 79 81 82 83 85 86 87 89 90 91 93 94 95 97 
>> 98 99 101 102 103 105 106 107 109 110 111 113 114 115 117 118 119 121 122 
>> 123 125 126 127
>>     &END FIXED_ATOMS
>>   &END CONSTRAINT
>>   &PRINT
>>     &RESTART
>>       BACKUP_COPIES 0 
>>     &END RESTART
>>   &END PRINT
>> &END MOTION
>> &VIBRATIONAL_ANALYSIS
>>   DX 0.1 
>>   NPROC_REP 60 
>>   TC_PRESSURE 101325
>>   TC_TEMPERATURE 298.15 
>>   THERMOCHEMISTRY T 
>>   INTENSITIES T 
>>   FULLY_PERIODIC T 
>>   &PRINT
>>     &MOLDEN_VIB 
>>     &END MOLDEN_VIB
>>   &END PRINT
>> &END VIBRATIONAL_ANALYSIS
>>
>> On Sunday, May 5, 2024 at 5:18:00 PM UTC+8 Marcella Iannuzzi wrote:
>>
>>> Hi ....
>>>
>>> This property is calculated only for molecule in gas phase, and not when 
>>> PBC are used
>>> Regards
>>> Marcella
>>>
>>> On Saturday, May 4, 2024 at 4:27:07 PM UTC+2 rafiq... at gmail.com wrote:
>>>
>>>> Like what should I write in input file for thermochemistry calculation?
>>>>
>>>> On Sat, 4 May 2024, 9:32 pm Marcella Iannuzzi, <marci... at gmail.com> 
>>>> wrote:
>>>>
>>>>> Hi...
>>>>>
>>>>>
>>>>> THERMOCHEMISTRY*: logical**= F* 
>>>>> <https://manual.cp2k.org/trunk/CP2K_INPUT/VIBRATIONAL_ANALYSIS.html#CP2K_INPUT.VIBRATIONAL_ANALYSIS.THERMOCHEMISTRY>
>>>>>
>>>>> *Lone keyword:* T
>>>>>
>>>>> Calculation of the thermochemical data. *Valid for molecules in the 
>>>>> gas phase.*
>>>>>
>>>>>
>>>>> Regards
>>>>>
>>>>> Marcella
>>>>> On Friday, May 3, 2024 at 2:23:20 PM UTC+2 rafiq... at gmail.com wrote:
>>>>>
>>>>>> &VIBRATIONAL_ANALYSIS
>>>>>>   DX 0.1 
>>>>>>   NPROC_REP 48
>>>>>>   TC_PRESSURE 101325 
>>>>>>   TC_TEMPERATURE 298.15 
>>>>>>   THERMOCHEMISTRY T
>>>>>>   FULLY_PERIODIC T
>>>>>> &END VIBRATIONAL_ANALYSIS
>>>>>>
>>>>>> Why in output file no thermochemistry? See my output file.
>>>>>>
>>>>>> VIB|                       142                  143                 
>>>>>>  144
>>>>>>  VIB|Frequency (cm^-1)   439.322414           439.460912           
>>>>>> 445.868786
>>>>>>  VIB|Red.Masses (a.u.)    34.271393            34.269852           
>>>>>>  34.289785
>>>>>>  VIB|Frc consts (a.u.)     0.003268             0.003272             
>>>>>> 0.003469
>>>>>>   ATOM  EL             X     Y     Z        X     Y     Z        X   
>>>>>>   Y     Z  
>>>>>>      3  Mo            0.01 -0.00  0.02    -0.00  0.00  0.03    -0.00 
>>>>>> -0.00 -0.03
>>>>>>      4  Mo            0.02 -0.00 -0.03    -0.00  0.01 -0.07     0.00 
>>>>>>  0.00 -0.05
>>>>>>      8  P            -0.28  0.04  0.00     0.08 -0.17  0.00     0.00 
>>>>>>  0.00  0.24
>>>>>>     11  Mo           -0.01 -0.00 -0.00     0.00 -0.00 -0.03    -0.00 
>>>>>> -0.00 -0.03
>>>>>>     12  Mo           -0.02 -0.01  0.00     0.00 -0.01  0.07     0.00 
>>>>>>  0.00 -0.05
>>>>>>     16  P             0.28  0.12  0.00    -0.08  0.17 -0.00     0.00 
>>>>>>  0.00  0.24
>>>>>>     19  Mo            0.01 -0.00  0.02    -0.00  0.00  0.03     0.00 
>>>>>> -0.00 -0.03
>>>>>>     20  Mo            0.02 -0.00 -0.03    -0.00  0.01 -0.07    -0.00 
>>>>>>  0.00 -0.05
>>>>>>     24  P            -0.28  0.04  0.00     0.08 -0.16  0.00     0.00 
>>>>>> -0.00  0.24
>>>>>>     27  Mo           -0.01 -0.00 -0.00     0.00 -0.00 -0.03     0.00 
>>>>>> -0.00 -0.03
>>>>>>     28  Mo           -0.02 -0.01  0.00     0.00 -0.01  0.07    -0.00 
>>>>>>  0.00 -0.05
>>>>>>     32  P             0.28  0.12 -0.00    -0.08  0.16 -0.01    -0.00 
>>>>>> -0.00  0.24
>>>>>>     35  Mo           -0.00 -0.00 -0.04    -0.01  0.00  0.01     0.00 
>>>>>>  0.00 -0.03
>>>>>>     36  Mo           -0.00 -0.00  0.08    -0.02  0.00 -0.02    -0.00 
>>>>>> -0.00 -0.05
>>>>>>     40  P             0.07  0.08 -0.01     0.29 -0.04  0.00     0.00 
>>>>>> -0.00  0.24
>>>>>>     43  Mo            0.00  0.00  0.02     0.01 -0.00 -0.01     0.00 
>>>>>>  0.00 -0.03
>>>>>>     44  Mo            0.00  0.01 -0.05     0.02 -0.00  0.02    -0.00 
>>>>>> -0.00 -0.05
>>>>>>     48  P            -0.07 -0.24  0.00    -0.29  0.04  0.00    -0.00 
>>>>>> -0.00  0.24
>>>>>>     51  Mo           -0.00 -0.00 -0.04    -0.01  0.00  0.01     0.00 
>>>>>>  0.00 -0.03
>>>>>>     52  Mo           -0.00 -0.00  0.08    -0.02  0.00 -0.02     0.00 
>>>>>> -0.00 -0.05
>>>>>>     56  P             0.07  0.08 -0.01     0.29 -0.04  0.00     0.00 
>>>>>> -0.00  0.25
>>>>>>     59  Mo            0.00  0.00  0.02     0.01 -0.00 -0.01    -0.00 
>>>>>>  0.00 -0.03
>>>>>>     60  Mo            0.00  0.01 -0.05     0.02 -0.00  0.02     0.00 
>>>>>> -0.00 -0.05
>>>>>>     64  P            -0.07 -0.24  0.00    -0.29  0.04 -0.00     0.00 
>>>>>>  0.00  0.24
>>>>>>     67  Mo            0.01 -0.00  0.02    -0.00  0.00  0.03    -0.00 
>>>>>> -0.00 -0.03
>>>>>>     68  Mo            0.02 -0.00 -0.03    -0.00  0.01 -0.07     0.00 
>>>>>> -0.00 -0.05
>>>>>>     72  P            -0.27  0.04  0.00     0.07 -0.17  0.00     0.00 
>>>>>>  0.00  0.24
>>>>>>     75  Mo           -0.01 -0.00 -0.00     0.00 -0.00 -0.03     0.00 
>>>>>> -0.00 -0.03
>>>>>>     76  Mo           -0.02 -0.01  0.00     0.00 -0.01  0.07    -0.00 
>>>>>> -0.00 -0.05
>>>>>>     80  P             0.27  0.12  0.00    -0.07  0.17 -0.00     0.00 
>>>>>>  0.00  0.24
>>>>>>     83  Mo            0.01 -0.00  0.02    -0.00  0.00  0.03    -0.00 
>>>>>> -0.00 -0.03
>>>>>>     84  Mo            0.02 -0.00 -0.03    -0.00  0.01 -0.07    -0.00 
>>>>>> -0.00 -0.05
>>>>>>     88  P            -0.27  0.04  0.00     0.07 -0.17  0.00    -0.00 
>>>>>>  0.00  0.24
>>>>>>     91  Mo           -0.01 -0.00 -0.00     0.00 -0.00 -0.03     0.00 
>>>>>>  0.00 -0.03
>>>>>>     92  Mo           -0.02 -0.01  0.00     0.00 -0.01  0.07     0.00 
>>>>>> -0.00 -0.05
>>>>>>     96  P             0.27  0.12 -0.00    -0.07  0.17 -0.00    -0.00 
>>>>>>  0.00  0.24
>>>>>>     99  Mo           -0.00 -0.00 -0.04    -0.01  0.00  0.01    -0.00 
>>>>>>  0.00 -0.03
>>>>>>    100  Mo           -0.00 -0.00  0.08    -0.02  0.00 -0.02    -0.00 
>>>>>>  0.00 -0.05
>>>>>>    104  P             0.07  0.08 -0.01     0.29 -0.04 -0.00    -0.00 
>>>>>> -0.00  0.24
>>>>>>    107  Mo            0.00  0.01  0.02     0.01 -0.00 -0.01     0.00 
>>>>>>  0.00 -0.03
>>>>>>    108  Mo            0.00  0.01 -0.05     0.02 -0.00  0.02    -0.00 
>>>>>>  0.00 -0.05
>>>>>>    112  P            -0.07 -0.24  0.00    -0.29  0.04 -0.00    -0.00 
>>>>>> -0.00  0.24
>>>>>>    115  Mo           -0.00 -0.00 -0.04    -0.01  0.00  0.01    -0.00 
>>>>>> -0.00 -0.03
>>>>>>    116  Mo           -0.00 -0.00  0.08    -0.02  0.00 -0.02     0.00 
>>>>>>  0.00 -0.05
>>>>>>    120  P             0.07  0.08 -0.00     0.29 -0.05  0.00     0.00 
>>>>>> -0.00  0.24
>>>>>>    123  Mo            0.00  0.01  0.02     0.01 -0.00 -0.01     0.00 
>>>>>>  0.00 -0.03
>>>>>>    124  Mo            0.00  0.01 -0.05     0.02 -0.00  0.02    -0.00 
>>>>>> -0.00 -0.05
>>>>>>    128  P            -0.07 -0.24  0.00    -0.29  0.05 -0.00     0.00 
>>>>>> -0.00  0.24
>>>>>>
>>>>>>
>>>>>>
>>>>>>
>>>>>>  -------------------------------------------------------------------------------
>>>>>>  -                                                                   
>>>>>>           -
>>>>>>  -                                DBCSR STATISTICS                   
>>>>>>           -
>>>>>>  -                                                                   
>>>>>>           -
>>>>>>
>>>>>>  -------------------------------------------------------------------------------
>>>>>>  COUNTER                                    TOTAL       BLAS       
>>>>>> SMM       ACC
>>>>>>  flops inhomo. stacks                           0       0.0%     
>>>>>>  0.0%      0.0%
>>>>>>  flops total                         0.000000E+00       0.0%     
>>>>>>  0.0%      0.0%
>>>>>>  flops max/rank                      0.000000E+00       0.0%     
>>>>>>  0.0%      0.0%
>>>>>>  matmuls inhomo. stacks                         0       0.0%     
>>>>>>  0.0%      0.0%
>>>>>>  matmuls total                                  0       0.0%     
>>>>>>  0.0%      0.0%
>>>>>>  number of processed stacks                     0       0.0%     
>>>>>>  0.0%      0.0%
>>>>>>  average stack size                                     0.0       0.0 
>>>>>>       0.0
>>>>>>  marketing flops                     0.000000E+00
>>>>>>
>>>>>>  -------------------------------------------------------------------------------
>>>>>>  -                                                                   
>>>>>>           -
>>>>>>  -                      DBCSR MESSAGE PASSING PERFORMANCE             
>>>>>>          -
>>>>>>  -                                                                   
>>>>>>           -
>>>>>>
>>>>>>  -------------------------------------------------------------------------------
>>>>>>  ROUTINE             CALLS      AVE VOLUME [Bytes]
>>>>>>  MP_Bcast                1                     12.
>>>>>>  MP_Allreduce      1316782                      8.
>>>>>>  MP_Alltoall      12045666                 733641.
>>>>>>
>>>>>>  -------------------------------------------------------------------------------
>>>>>>
>>>>>> -- 
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>>>>> .
>>>>>
>>>>

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