[CP2K-user] [CP2K:20171] Re: Vibrational Analysis

Muhammad Rafiq rafiq789.ra at gmail.com
Sun May 5 09:54:23 UTC 2024


(Please check my input file, when i remove the pbc then my system will not 
treat as periodic) so what should i change in my input please consider my 
input , thanks for your response

&GLOBAL
  PROJECT MoP100-44-pos-1
  PRINT_LEVEL LOW
  RUN_TYPE VIBRATIONAL_ANALYSIS
&END GLOBAL

&FORCE_EVAL
  METHOD Quickstep
  &SUBSYS
    &CELL
      A    12.87500000     0.00000000     0.00000000
      B     6.43800000    11.15094310     0.00000000
      C     0.00000000     0.00000000    31.10900000
      PERIODIC XYZ 
    &END CELL
    &COORD
      Mo          3.21900000    1.85900000    1.58700000
      Mo          3.21900000    1.85900000    4.76100000
      Mo          3.21900000    1.85900000    7.93500000
      Mo          3.21900000    1.85900000   11.00400000
      P           0.00000000    0.00000000    0.00000000
      P           0.00000000    0.00000000    3.17400000
      P           0.00000000    0.00000000    6.34800000
      P          12.87500000    0.00000000    9.58600000
      Mo          6.43800000    1.85900000    1.58700000
      Mo          6.43800000    1.85900000    4.76100000
      Mo          6.43800000    1.85900000    7.93500000
      Mo          6.43800000    1.85900000   11.00400000
      P           3.21900000    0.00000000    0.00000000
      P           3.21900000    0.00000000    3.17400000
      P           3.21900000    0.00000000    6.34800000
      P           3.21900000    0.00000000    9.58600000
      Mo          9.65600000    1.85900000    1.58700000
      Mo          9.65600000    1.85900000    4.76100000
      Mo          9.65600000    1.85900000    7.93500000
      Mo          9.65600000    1.85900000   11.00400000
      P           6.43800000    0.00000000    0.00000000
      P           6.43800000    0.00000000    3.17400000
      P           6.43800000    0.00000000    6.34800000
      P           6.43800000    0.00000000    9.58600000
      Mo         12.87500000    1.85900000    1.58700000
      Mo         12.87500000    1.85900000    4.76100000
      Mo         12.87500000    1.85900000    7.93500000
      Mo         12.87500000    1.85900000   11.00400000
      P           9.65600000    0.00000000    0.00000000
      P           9.65600000    0.00000000    3.17400000
      P           9.65600000    0.00000000    6.34800000
      P           9.65600000    0.00000000    9.58600000
      Mo          4.82800000    4.64600000    1.58700000
      Mo          4.82800000    4.64600000    4.76100000
      Mo          4.82800000    4.64600000    7.93500000
      Mo          4.82800000    4.64600000   11.00400000
      P           1.60900000    2.78800000    0.00000000
      P           1.60900000    2.78800000    3.17400000
      P           1.60900000    2.78800000    6.34800000
      P          14.48500000    2.78800000    9.58600000
      Mo          8.04700000    4.64600000    1.58700000
      Mo          8.04700000    4.64600000    4.76100000
      Mo          8.04700000    4.64600000    7.93500000
      Mo          8.04700000    4.64600000   11.00400000
      P           4.82800000    2.78800000    0.00000000
      P           4.82800000    2.78800000    3.17400000
      P           4.82800000    2.78800000    6.34800000
      P           4.82800000    2.78800000    9.58600000
      Mo         11.26600000    4.64600000    1.58700000
      Mo         11.26600000    4.64600000    4.76100000
      Mo         11.26600000    4.64600000    7.93500000
      Mo         11.26600000    4.64600000   11.00400000
      P           8.04700000    2.78800000    0.00000000
      P           8.04700000    2.78800000    3.17400000
      P           8.04700000    2.78800000    6.34800000
      P           8.04700000    2.78800000    9.58600000
      Mo         14.48500000    4.64600000    1.58700000
      Mo         14.48500000    4.64600000    4.76100000
      Mo         14.48500000    4.64600000    7.93500000
      Mo         14.48500000    4.64600000   11.00400000
      P          11.26600000    2.78800000    0.00000000
      P          11.26600000    2.78800000    3.17400000
      P          11.26600000    2.78800000    6.34800000
      P          11.26600000    2.78800000    9.58600000
      Mo          6.43800000    7.43400000    1.58700000
      Mo          6.43800000    7.43400000    4.76100000
      Mo          6.43800000    7.43400000    7.93500000
      Mo          6.43800000    7.43400000   11.00400000
      P           3.21900000    5.57600000    0.00000000
      P           3.21900000    5.57600000    3.17400000
      P           3.21900000    5.57600000    6.34800000
      P           3.21900000    5.57600000    9.58600000
      Mo          9.65600000    7.43400000    1.58700000
      Mo          9.65600000    7.43400000    4.76100000
      Mo          9.65600000    7.43400000    7.93500000
      Mo          9.65600000    7.43400000   11.00400000
      P           6.43800000    5.57600000    0.00000000
      P           6.43800000    5.57600000    3.17400000
      P           6.43800000    5.57600000    6.34800000
      P           6.43800000    5.57600000    9.58600000
      Mo         12.87500000    7.43400000    1.58700000
      Mo         12.87500000    7.43400000    4.76100000
      Mo         12.87500000    7.43400000    7.93500000
      Mo         12.87500000    7.43400000   11.00400000
      P           9.65600000    5.57600000    0.00000000
      P           9.65600000    5.57600000    3.17400000
      P           9.65600000    5.57600000    6.34800000
      P           9.65600000    5.57600000    9.58600000
      Mo         16.09400000    7.43400000    1.58700000
      Mo         16.09400000    7.43400000    4.76100000
      Mo         16.09400000    7.43400000    7.93500000
      Mo         16.09400000    7.43400000   11.00400000
      P          12.87500000    5.57600000    0.00000000
      P          12.87500000    5.57600000    3.17400000
      P          12.87500000    5.57600000    6.34800000
      P          12.87500000    5.57600000    9.58600000
      Mo          8.04700000   10.22200000    1.58700000
      Mo          8.04700000   10.22200000    4.76100000
      Mo          8.04700000   10.22200000    7.93500000
      Mo          8.04700000   10.22200000   11.00400000
      P           4.82800000    8.36300000    0.00000000
      P          17.70300000    8.36300000    3.17400000
      P          17.70300000    8.36300000    6.34800000
      P           4.82800000    8.36300000    9.58600000
      Mo         11.26600000   10.22200000    1.58700000
      Mo         11.26600000   10.22200000    4.76100000
      Mo         11.26600000   10.22200000    7.93500000
      Mo         11.26600000   10.22200000   11.00400000
      P           8.04700000    8.36300000    0.00000000
      P           8.04700000    8.36300000    3.17400000
      P           8.04700000    8.36300000    6.34800000
      P           8.04700000    8.36300000    9.58600000
      Mo         14.48500000   10.22200000    1.58700000
      Mo         14.48500000   10.22200000    4.76100000
      Mo         14.48500000   10.22200000    7.93500000
      Mo         14.48500000   10.22200000   11.00400000
      P          11.26600000    8.36300000    0.00000000
      P          11.26600000    8.36300000    3.17400000
      P          11.26600000    8.36300000    6.34800000
      P          11.26600000    8.36300000    9.58600000
      Mo         17.70300000   10.22200000    1.58700000
      Mo         17.70300000   10.22200000    4.76100000
      Mo         17.70300000   10.22200000    7.93500000
      Mo         17.70300000   10.22200000   11.00400000
      P          14.48500000    8.36300000    0.00000000
      P          14.48500000    8.36300000    3.17400000
      P          14.48500000    8.36300000    6.34800000
      P          14.48500000    8.36300000    9.58600000
    &END COORD
    &KIND Mo
      ELEMENT Mo
      BASIS_SET DZVP-MOLOPT-SR-GTH-q14
      POTENTIAL GTH-PBE
    &END KIND
    &KIND P
      ELEMENT P
      BASIS_SET DZVP-MOLOPT-SR-GTH-q5
      POTENTIAL GTH-PBE
    &END KIND
  &END SUBSYS

  &DFT
    BASIS_SET_FILE_NAME  BASIS_MOLOPT
    POTENTIAL_FILE_NAME  POTENTIAL
#   WFN_RESTART_FILE_NAME MoP100-44-pos-1-RESTART.kp
    CHARGE    0 
    MULTIPLICITY    1 
    &KPOINTS
      SCHEME MONKHORST-PACK  3  3  1
    &END KPOINTS
    &QS
      EPS_DEFAULT 1.0E-12 
#     EXTRAPOLATION USE_PREV_P 
    &END QS
    &POISSON
      PERIODIC XYZ 
      PSOLVER PERIODIC 
    &END POISSON
    &XC
      &XC_FUNCTIONAL PBE
      &END XC_FUNCTIONAL
      &VDW_POTENTIAL
        POTENTIAL_TYPE PAIR_POTENTIAL
        &PAIR_POTENTIAL
          PARAMETER_FILE_NAME dftd3.dat
          TYPE DFTD3(BJ)
          REFERENCE_FUNCTIONAL PBE
          #CALCULATE_C9_TERM T 
        &END PAIR_POTENTIAL
      &END VDW_POTENTIAL
    &END XC
    &MGRID
      CUTOFF  500
      REL_CUTOFF  65
    &END MGRID
    &SCF
      MAX_SCF 300
      EPS_SCF 1.0E-8 
#     SCF_GUESS RESTART 
#     IGNORE_CONVERGENCE_FAILURE 
      &DIAGONALIZATION
        ALGORITHM STANDARD 
      &END DIAGONALIZATION
      &MIXING 
        METHOD BROYDEN_MIXING
        ALPHA 0.4 
        NBROYDEN 8 
      &END MIXING
      &SMEAR
        METHOD FERMI_DIRAC
        ELECTRONIC_TEMPERATURE 300 
      &END SMEAR
      ADDED_MOS    64 
      &PRINT
        &RESTART 
BACKUP_COPIES 0 
        &END RESTART
      &END PRINT
    &END SCF
   &END DFT
&END FORCE_EVAL

&MOTION
  &CONSTRAINT
    &FIXED_ATOMS 
      COMPONENTS_TO_FIX XYZ 
      LIST 1 2 3 5 6 7 9 10 11 13 14 15 17 18 19 21 22 23 25 26 27 29 30 31 
33 34 35 37 38 39 41 42 43 45 46 47 49 50 51 53 54 55 57 58 59 61 62 63 65 
66 67 69 70 71 73 74 75 77 78 79 81 82 83 85 86 87 89 90 91 93 94 95 97 98 
99 101 102 103 105 106 107 109 110 111 113 114 115 117 118 119 121 122 123 
125 126 127
    &END FIXED_ATOMS
  &END CONSTRAINT
  &PRINT
    &RESTART
      BACKUP_COPIES 0 
    &END RESTART
  &END PRINT
&END MOTION
&VIBRATIONAL_ANALYSIS
  DX 0.1 
  NPROC_REP 60 
  TC_PRESSURE 101325
  TC_TEMPERATURE 298.15 
  THERMOCHEMISTRY T 
  INTENSITIES T 
  FULLY_PERIODIC T 
  &PRINT
    &MOLDEN_VIB 
    &END MOLDEN_VIB
  &END PRINT
&END VIBRATIONAL_ANALYSIS

On Sunday, May 5, 2024 at 5:18:00 PM UTC+8 Marcella Iannuzzi wrote:

> Hi ....
>
> This property is calculated only for molecule in gas phase, and not when 
> PBC are used
> Regards
> Marcella
>
> On Saturday, May 4, 2024 at 4:27:07 PM UTC+2 rafiq... at gmail.com wrote:
>
>> Like what should I write in input file for thermochemistry calculation?
>>
>> On Sat, 4 May 2024, 9:32 pm Marcella Iannuzzi, <marci... at gmail.com> 
>> wrote:
>>
>>> Hi...
>>>
>>>
>>> THERMOCHEMISTRY*: logical**= F* 
>>> <https://manual.cp2k.org/trunk/CP2K_INPUT/VIBRATIONAL_ANALYSIS.html#CP2K_INPUT.VIBRATIONAL_ANALYSIS.THERMOCHEMISTRY>
>>>
>>> *Lone keyword:* T
>>>
>>> Calculation of the thermochemical data. *Valid for molecules in the gas 
>>> phase.*
>>>
>>>
>>> Regards
>>>
>>> Marcella
>>> On Friday, May 3, 2024 at 2:23:20 PM UTC+2 rafiq... at gmail.com wrote:
>>>
>>>> &VIBRATIONAL_ANALYSIS
>>>>   DX 0.1 
>>>>   NPROC_REP 48
>>>>   TC_PRESSURE 101325 
>>>>   TC_TEMPERATURE 298.15 
>>>>   THERMOCHEMISTRY T
>>>>   FULLY_PERIODIC T
>>>> &END VIBRATIONAL_ANALYSIS
>>>>
>>>> Why in output file no thermochemistry? See my output file.
>>>>
>>>> VIB|                       142                  143                  144
>>>>  VIB|Frequency (cm^-1)   439.322414           439.460912           
>>>> 445.868786
>>>>  VIB|Red.Masses (a.u.)    34.271393            34.269852           
>>>>  34.289785
>>>>  VIB|Frc consts (a.u.)     0.003268             0.003272             
>>>> 0.003469
>>>>   ATOM  EL             X     Y     Z        X     Y     Z        X     
>>>> Y     Z  
>>>>      3  Mo            0.01 -0.00  0.02    -0.00  0.00  0.03    -0.00 
>>>> -0.00 -0.03
>>>>      4  Mo            0.02 -0.00 -0.03    -0.00  0.01 -0.07     0.00 
>>>>  0.00 -0.05
>>>>      8  P            -0.28  0.04  0.00     0.08 -0.17  0.00     0.00 
>>>>  0.00  0.24
>>>>     11  Mo           -0.01 -0.00 -0.00     0.00 -0.00 -0.03    -0.00 
>>>> -0.00 -0.03
>>>>     12  Mo           -0.02 -0.01  0.00     0.00 -0.01  0.07     0.00 
>>>>  0.00 -0.05
>>>>     16  P             0.28  0.12  0.00    -0.08  0.17 -0.00     0.00 
>>>>  0.00  0.24
>>>>     19  Mo            0.01 -0.00  0.02    -0.00  0.00  0.03     0.00 
>>>> -0.00 -0.03
>>>>     20  Mo            0.02 -0.00 -0.03    -0.00  0.01 -0.07    -0.00 
>>>>  0.00 -0.05
>>>>     24  P            -0.28  0.04  0.00     0.08 -0.16  0.00     0.00 
>>>> -0.00  0.24
>>>>     27  Mo           -0.01 -0.00 -0.00     0.00 -0.00 -0.03     0.00 
>>>> -0.00 -0.03
>>>>     28  Mo           -0.02 -0.01  0.00     0.00 -0.01  0.07    -0.00 
>>>>  0.00 -0.05
>>>>     32  P             0.28  0.12 -0.00    -0.08  0.16 -0.01    -0.00 
>>>> -0.00  0.24
>>>>     35  Mo           -0.00 -0.00 -0.04    -0.01  0.00  0.01     0.00 
>>>>  0.00 -0.03
>>>>     36  Mo           -0.00 -0.00  0.08    -0.02  0.00 -0.02    -0.00 
>>>> -0.00 -0.05
>>>>     40  P             0.07  0.08 -0.01     0.29 -0.04  0.00     0.00 
>>>> -0.00  0.24
>>>>     43  Mo            0.00  0.00  0.02     0.01 -0.00 -0.01     0.00 
>>>>  0.00 -0.03
>>>>     44  Mo            0.00  0.01 -0.05     0.02 -0.00  0.02    -0.00 
>>>> -0.00 -0.05
>>>>     48  P            -0.07 -0.24  0.00    -0.29  0.04  0.00    -0.00 
>>>> -0.00  0.24
>>>>     51  Mo           -0.00 -0.00 -0.04    -0.01  0.00  0.01     0.00 
>>>>  0.00 -0.03
>>>>     52  Mo           -0.00 -0.00  0.08    -0.02  0.00 -0.02     0.00 
>>>> -0.00 -0.05
>>>>     56  P             0.07  0.08 -0.01     0.29 -0.04  0.00     0.00 
>>>> -0.00  0.25
>>>>     59  Mo            0.00  0.00  0.02     0.01 -0.00 -0.01    -0.00 
>>>>  0.00 -0.03
>>>>     60  Mo            0.00  0.01 -0.05     0.02 -0.00  0.02     0.00 
>>>> -0.00 -0.05
>>>>     64  P            -0.07 -0.24  0.00    -0.29  0.04 -0.00     0.00 
>>>>  0.00  0.24
>>>>     67  Mo            0.01 -0.00  0.02    -0.00  0.00  0.03    -0.00 
>>>> -0.00 -0.03
>>>>     68  Mo            0.02 -0.00 -0.03    -0.00  0.01 -0.07     0.00 
>>>> -0.00 -0.05
>>>>     72  P            -0.27  0.04  0.00     0.07 -0.17  0.00     0.00 
>>>>  0.00  0.24
>>>>     75  Mo           -0.01 -0.00 -0.00     0.00 -0.00 -0.03     0.00 
>>>> -0.00 -0.03
>>>>     76  Mo           -0.02 -0.01  0.00     0.00 -0.01  0.07    -0.00 
>>>> -0.00 -0.05
>>>>     80  P             0.27  0.12  0.00    -0.07  0.17 -0.00     0.00 
>>>>  0.00  0.24
>>>>     83  Mo            0.01 -0.00  0.02    -0.00  0.00  0.03    -0.00 
>>>> -0.00 -0.03
>>>>     84  Mo            0.02 -0.00 -0.03    -0.00  0.01 -0.07    -0.00 
>>>> -0.00 -0.05
>>>>     88  P            -0.27  0.04  0.00     0.07 -0.17  0.00    -0.00 
>>>>  0.00  0.24
>>>>     91  Mo           -0.01 -0.00 -0.00     0.00 -0.00 -0.03     0.00 
>>>>  0.00 -0.03
>>>>     92  Mo           -0.02 -0.01  0.00     0.00 -0.01  0.07     0.00 
>>>> -0.00 -0.05
>>>>     96  P             0.27  0.12 -0.00    -0.07  0.17 -0.00    -0.00 
>>>>  0.00  0.24
>>>>     99  Mo           -0.00 -0.00 -0.04    -0.01  0.00  0.01    -0.00 
>>>>  0.00 -0.03
>>>>    100  Mo           -0.00 -0.00  0.08    -0.02  0.00 -0.02    -0.00 
>>>>  0.00 -0.05
>>>>    104  P             0.07  0.08 -0.01     0.29 -0.04 -0.00    -0.00 
>>>> -0.00  0.24
>>>>    107  Mo            0.00  0.01  0.02     0.01 -0.00 -0.01     0.00 
>>>>  0.00 -0.03
>>>>    108  Mo            0.00  0.01 -0.05     0.02 -0.00  0.02    -0.00 
>>>>  0.00 -0.05
>>>>    112  P            -0.07 -0.24  0.00    -0.29  0.04 -0.00    -0.00 
>>>> -0.00  0.24
>>>>    115  Mo           -0.00 -0.00 -0.04    -0.01  0.00  0.01    -0.00 
>>>> -0.00 -0.03
>>>>    116  Mo           -0.00 -0.00  0.08    -0.02  0.00 -0.02     0.00 
>>>>  0.00 -0.05
>>>>    120  P             0.07  0.08 -0.00     0.29 -0.05  0.00     0.00 
>>>> -0.00  0.24
>>>>    123  Mo            0.00  0.01  0.02     0.01 -0.00 -0.01     0.00 
>>>>  0.00 -0.03
>>>>    124  Mo            0.00  0.01 -0.05     0.02 -0.00  0.02    -0.00 
>>>> -0.00 -0.05
>>>>    128  P            -0.07 -0.24  0.00    -0.29  0.05 -0.00     0.00 
>>>> -0.00  0.24
>>>>
>>>>
>>>>
>>>>
>>>>  -------------------------------------------------------------------------------
>>>>  -                                                                     
>>>>         -
>>>>  -                                DBCSR STATISTICS                     
>>>>         -
>>>>  -                                                                     
>>>>         -
>>>>
>>>>  -------------------------------------------------------------------------------
>>>>  COUNTER                                    TOTAL       BLAS       SMM 
>>>>       ACC
>>>>  flops inhomo. stacks                           0       0.0%      0.0% 
>>>>      0.0%
>>>>  flops total                         0.000000E+00       0.0%      0.0% 
>>>>      0.0%
>>>>  flops max/rank                      0.000000E+00       0.0%      0.0% 
>>>>      0.0%
>>>>  matmuls inhomo. stacks                         0       0.0%      0.0% 
>>>>      0.0%
>>>>  matmuls total                                  0       0.0%      0.0% 
>>>>      0.0%
>>>>  number of processed stacks                     0       0.0%      0.0% 
>>>>      0.0%
>>>>  average stack size                                     0.0       0.0   
>>>>     0.0
>>>>  marketing flops                     0.000000E+00
>>>>
>>>>  -------------------------------------------------------------------------------
>>>>  -                                                                     
>>>>         -
>>>>  -                      DBCSR MESSAGE PASSING PERFORMANCE               
>>>>        -
>>>>  -                                                                     
>>>>         -
>>>>
>>>>  -------------------------------------------------------------------------------
>>>>  ROUTINE             CALLS      AVE VOLUME [Bytes]
>>>>  MP_Bcast                1                     12.
>>>>  MP_Allreduce      1316782                      8.
>>>>  MP_Alltoall      12045666                 733641.
>>>>
>>>>  -------------------------------------------------------------------------------
>>>>
>>>> -- 
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