[CP2K-user] Convergence problem- MD calculation for metal surface

Kevin amin.ja... at gmail.com
Sat May 11 23:41:58 UTC 2019


Dear Matt,

Enclosed please find the necessary files for testing. Thank you in advance.

Kind regards,

Kevin

On Friday, May 10, 2019 at 8:37:55 PM UTC+2, Matt W wrote:
>
> If you send me all files required to run (on here or to my email), I can 
> try and have a look.
>
> On Friday, May 10, 2019 at 3:02:59 PM UTC+1, Kevin wrote:
>>
>> Dear Matt,
>>
>> I would highly appreciate that if you let me know about any updates.
>>
>> Best,
>>
>> Kevin
>>
>> On Tuesday, April 2, 2019 at 12:49:53 AM UTC+2, Kevin wrote:
>>>
>>> Dear Matt,
>>>
>>> Thanks for the feedback. Actually I have used the same super-cell size 
>>> of the optimized slab and also whenever I use AIMD it works (but it's 
>>> expensive!). So I think the structure is OK. 
>>> I even tried once with OT method and again didn't get the mentioned 
>>> error. I have encountered the error while using DFTB or PM6.
>>>
>>> On Monday, April 1, 2019 at 8:04:28 PM UTC+2, Matt W wrote:
>>>>
>>>> I've not looked at your files, but are you sure you don't have atoms on 
>>>> top of each other, maybe across periodic images?
>>>>
>>>> On Sunday, March 31, 2019 at 11:27:50 PM UTC+1, Kevin wrote:
>>>>>
>>>>>  
>>>>> Dear all,
>>>>> I'm encountering convergence problem for the MD simulation of single 
>>>>> molecule adsorption on Ni surface. This is a test case to see if I can 
>>>>> calculate my desired system. I'm using a GLE thermostat. 
>>>>> I've tried using DFTB and PM6 but in both cases I receive the error 
>>>>> below, mentioning: 
>>>>> *"Bad condition number R_COND = 0.000E+00 (smaller than the machine 
>>>>> working precision"  common/mathlib.F:709.*
>>>>> As you know, DFTB or PM6 are chosen because of their inexpensiveness! 
>>>>>
>>>>> [image: Capture.PNG]
>>>>>
>>>>>
>>>>> Here is my input file and I've attached the coordinate file:
>>>>>
>>>>>
>>>>> &GLOBAL
>>>>>         PROJECT CH4-Ni
>>>>>         RUN_TYPE MD
>>>>>         PRINT_LEVEL LOW
>>>>> &END GLOBAL
>>>>>
>>>>> &FORCE_EVAL
>>>>>         METHOD Quickstep
>>>>>         &DFT
>>>>>     &QS
>>>>>       METHOD PM6
>>>>>       &SE
>>>>>        RC_INTERACTION [angstrom] 8.0
>>>>>        RC_COULOMB     [angstrom] 8.0
>>>>>        RC_RANGE       [angstrom] 0.05
>>>>>       &END
>>>>>     &END QS
>>>>>    ! &QS
>>>>>    !   METHOD DFTB
>>>>>    !   &DFTB
>>>>>    !     SELF_CONSISTENT    T
>>>>>    !     DO_EWALD           T
>>>>>    !     DISPERSION         T
>>>>>    !     &PARAMETER
>>>>>    !       PARAM_FILE_PATH  /data/scc
>>>>>    !       PARAM_FILE_NAME  scc_parameter
>>>>>    !       UFF_FORCE_FIELD  uff_table
>>>>>    !     &END PARAMETER
>>>>>    !   &END DFTB
>>>>>    ! &END QS
>>>>>                 &SCF
>>>>>                         MAX_SCF 30
>>>>>                         EPS_SCF 5.0E-6
>>>>>                         &OUTER_SCF
>>>>>                                 MAX_SCF 30
>>>>>                                 EPS_SCF 5.0E-6
>>>>>                         &END
>>>>>                         &DIAGONALIZATION  ON
>>>>>                                 ALGORITHM STANDARD
>>>>>                         &END DIAGONALIZATION
>>>>>                         ADDED_MOS 300
>>>>>                         &SMEAR  ON
>>>>>                                 METHOD FERMI_DIRAC
>>>>>                                 ELECTRONIC_TEMPERATURE [K] 350
>>>>>                         &END SMEAR
>>>>>                         &MIXING
>>>>>                                 METHOD BROYDEN_MIXING
>>>>>                                 BETA 1.5
>>>>>                                 ALPHA   0.1
>>>>>                                 NBROYDEN  8
>>>>>                         &END MIXING
>>>>>                         &PRINT
>>>>>                                 &RESTART LOW
>>>>>                                         BACKUP_COPIES 1
>>>>>                                 &END RESTART
>>>>>                         &END PRINT
>>>>>                         SCF_GUESS ATOMIC
>>>>>                 &END SCF    
>>>>>                 &POISSON
>>>>>                         POISSON_SOLVER MT
>>>>>                         PERIODIC XY
>>>>>       &EWALD
>>>>>        EWALD_TYPE SPME
>>>>>        GMAX 25
>>>>>        O_SPLINE 5
>>>>>       &END EWALD
>>>>>                 &END POISSON
>>>>>         &END DFT
>>>>>
>>>>>         &SUBSYS
>>>>>                 &CELL
>>>>>                         ABC 12.4597 12.9485 23.1387
>>>>>                         PERIODIC XY
>>>>>                 &END CELL
>>>>>                 &COORD
>>>>> @INCLUDE 'ch4-ni.coord'
>>>>>         &END COORD
>>>>>         &TOPOLOGY
>>>>>                 &CENTER_COORDINATES
>>>>>                 &END CENTER_COORDINATES
>>>>>         &END TOPOLOGY
>>>>> &END SUBSYS
>>>>> &END FORCE_EVAL
>>>>>
>>>>> &MOTION
>>>>>         &MD
>>>>>                 ENSEMBLE NVT
>>>>>                 STEPS 10000
>>>>>                 TIMESTEP 0.5
>>>>>                 TEMPERATURE 300
>>>>>                 &THERMOSTAT
>>>>>                         REGION MASSIVE
>>>>>                         TYPE GLE
>>>>>                         &GLE
>>>>>                                 NDIM 3
>>>>>                                 A_SCALE [ps^-1] 1.00
>>>>>                                 A_LIST    2.000000000000e+0   
>>>>> 1.365763041717e+1   0.000000000000e+0
>>>>>                                 A_LIST   -1.365763041717e+1   
>>>>> 9.418257899376e-1   5.860040064992e+2
>>>>>                                 A_LIST    0.000000000000e+0  
>>>>> -5.860040064992e+2   0.000000000000e+0
>>>>>                                 C_LIST    3.071856358605e+2   
>>>>> 1.052252204958e+0  -3.083120039764e+2
>>>>>                                 C_LIST    1.052252204958e+0   
>>>>> 1.353606645969e+4   0.000000000000e+0
>>>>>                                 C_LIST   -3.083120039764e+2   
>>>>> 0.000000000000e+0   1.352888082383e+4
>>>>>                         &END GLE
>>>>>                 &END THERMOSTAT
>>>>>                 &PRINT
>>>>>                         &ENERGY
>>>>>                                 &EACH
>>>>>                                         MD 10
>>>>>                                 &END EACH
>>>>>                         &END ENERGY
>>>>>                 &END PRINT
>>>>>         &END MD
>>>>>         &FREE_ENERGY
>>>>>                 &FREE_ENERGY_INFO
>>>>>                         &EACH
>>>>>                                 MD 1000
>>>>>                         &END
>>>>>                 &END
>>>>>                 &METADYN
>>>>>                         &PRINT
>>>>>                                 &COLVAR
>>>>>                                         COMMON_ITERATION_LEVELS 3
>>>>>                                         &EACH
>>>>>                                                 MD 1
>>>>>                                         &END
>>>>>                                 &END
>>>>>                                 &HILLS
>>>>>                                         COMMON_ITERATION_LEVELS 3
>>>>>                                         &EACH
>>>>>                                                 MD 1
>>>>>                                         &END
>>>>>                                 &END
>>>>>                         &END
>>>>>                 &END METADYN
>>>>>         &END FREE_ENERGY
>>>>>         &PRINT
>>>>>                 &TRAJECTORY
>>>>>                         FORMAT XYZ
>>>>>                         &EACH
>>>>>                                 MD 20
>>>>>                         &END EACH
>>>>>                 &END TRAJECTORY
>>>>>                 &RESTART_HISTORY
>>>>>                         &EACH
>>>>>                                 MD 10000
>>>>>                         &END EACH
>>>>>                 &END RESTART_HISTORY
>>>>>                 &RESTART OFF
>>>>>                 &END RESTART
>>>>>         &END PRINT
>>>>> &END MOTION
>>>>>
>>>>> I would be grateful if anyone could take a look to my input file and 
>>>>> let me know about the possible way to get the structure converged. I've 
>>>>> already relaxed the metal structure before using it for md simulation. 
>>>>>  
>>>>> Thanks in advance.
>>>>>
>>>>> Kevin
>>>>>
>>>>
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