[CP2K-user] Convergence problem- MD calculation for metal surface

Matt W mattwa... at gmail.com
Fri May 10 18:37:55 UTC 2019


If you send me all files required to run (on here or to my email), I can 
try and have a look.

On Friday, May 10, 2019 at 3:02:59 PM UTC+1, Kevin wrote:
>
> Dear Matt,
>
> I would highly appreciate that if you let me know about any updates.
>
> Best,
>
> Kevin
>
> On Tuesday, April 2, 2019 at 12:49:53 AM UTC+2, Kevin wrote:
>>
>> Dear Matt,
>>
>> Thanks for the feedback. Actually I have used the same super-cell size of 
>> the optimized slab and also whenever I use AIMD it works (but it's 
>> expensive!). So I think the structure is OK. 
>> I even tried once with OT method and again didn't get the mentioned 
>> error. I have encountered the error while using DFTB or PM6.
>>
>> On Monday, April 1, 2019 at 8:04:28 PM UTC+2, Matt W wrote:
>>>
>>> I've not looked at your files, but are you sure you don't have atoms on 
>>> top of each other, maybe across periodic images?
>>>
>>> On Sunday, March 31, 2019 at 11:27:50 PM UTC+1, Kevin wrote:
>>>>
>>>>  
>>>> Dear all,
>>>> I'm encountering convergence problem for the MD simulation of single 
>>>> molecule adsorption on Ni surface. This is a test case to see if I can 
>>>> calculate my desired system. I'm using a GLE thermostat. 
>>>> I've tried using DFTB and PM6 but in both cases I receive the error 
>>>> below, mentioning: 
>>>> *"Bad condition number R_COND = 0.000E+00 (smaller than the machine 
>>>> working precision"  common/mathlib.F:709.*
>>>> As you know, DFTB or PM6 are chosen because of their inexpensiveness! 
>>>>
>>>> [image: Capture.PNG]
>>>>
>>>>
>>>> Here is my input file and I've attached the coordinate file:
>>>>
>>>>
>>>> &GLOBAL
>>>>         PROJECT CH4-Ni
>>>>         RUN_TYPE MD
>>>>         PRINT_LEVEL LOW
>>>> &END GLOBAL
>>>>
>>>> &FORCE_EVAL
>>>>         METHOD Quickstep
>>>>         &DFT
>>>>     &QS
>>>>       METHOD PM6
>>>>       &SE
>>>>        RC_INTERACTION [angstrom] 8.0
>>>>        RC_COULOMB     [angstrom] 8.0
>>>>        RC_RANGE       [angstrom] 0.05
>>>>       &END
>>>>     &END QS
>>>>    ! &QS
>>>>    !   METHOD DFTB
>>>>    !   &DFTB
>>>>    !     SELF_CONSISTENT    T
>>>>    !     DO_EWALD           T
>>>>    !     DISPERSION         T
>>>>    !     &PARAMETER
>>>>    !       PARAM_FILE_PATH  /data/scc
>>>>    !       PARAM_FILE_NAME  scc_parameter
>>>>    !       UFF_FORCE_FIELD  uff_table
>>>>    !     &END PARAMETER
>>>>    !   &END DFTB
>>>>    ! &END QS
>>>>                 &SCF
>>>>                         MAX_SCF 30
>>>>                         EPS_SCF 5.0E-6
>>>>                         &OUTER_SCF
>>>>                                 MAX_SCF 30
>>>>                                 EPS_SCF 5.0E-6
>>>>                         &END
>>>>                         &DIAGONALIZATION  ON
>>>>                                 ALGORITHM STANDARD
>>>>                         &END DIAGONALIZATION
>>>>                         ADDED_MOS 300
>>>>                         &SMEAR  ON
>>>>                                 METHOD FERMI_DIRAC
>>>>                                 ELECTRONIC_TEMPERATURE [K] 350
>>>>                         &END SMEAR
>>>>                         &MIXING
>>>>                                 METHOD BROYDEN_MIXING
>>>>                                 BETA 1.5
>>>>                                 ALPHA   0.1
>>>>                                 NBROYDEN  8
>>>>                         &END MIXING
>>>>                         &PRINT
>>>>                                 &RESTART LOW
>>>>                                         BACKUP_COPIES 1
>>>>                                 &END RESTART
>>>>                         &END PRINT
>>>>                         SCF_GUESS ATOMIC
>>>>                 &END SCF    
>>>>                 &POISSON
>>>>                         POISSON_SOLVER MT
>>>>                         PERIODIC XY
>>>>       &EWALD
>>>>        EWALD_TYPE SPME
>>>>        GMAX 25
>>>>        O_SPLINE 5
>>>>       &END EWALD
>>>>                 &END POISSON
>>>>         &END DFT
>>>>
>>>>         &SUBSYS
>>>>                 &CELL
>>>>                         ABC 12.4597 12.9485 23.1387
>>>>                         PERIODIC XY
>>>>                 &END CELL
>>>>                 &COORD
>>>> @INCLUDE 'ch4-ni.coord'
>>>>         &END COORD
>>>>         &TOPOLOGY
>>>>                 &CENTER_COORDINATES
>>>>                 &END CENTER_COORDINATES
>>>>         &END TOPOLOGY
>>>> &END SUBSYS
>>>> &END FORCE_EVAL
>>>>
>>>> &MOTION
>>>>         &MD
>>>>                 ENSEMBLE NVT
>>>>                 STEPS 10000
>>>>                 TIMESTEP 0.5
>>>>                 TEMPERATURE 300
>>>>                 &THERMOSTAT
>>>>                         REGION MASSIVE
>>>>                         TYPE GLE
>>>>                         &GLE
>>>>                                 NDIM 3
>>>>                                 A_SCALE [ps^-1] 1.00
>>>>                                 A_LIST    2.000000000000e+0   
>>>> 1.365763041717e+1   0.000000000000e+0
>>>>                                 A_LIST   -1.365763041717e+1   
>>>> 9.418257899376e-1   5.860040064992e+2
>>>>                                 A_LIST    0.000000000000e+0  
>>>> -5.860040064992e+2   0.000000000000e+0
>>>>                                 C_LIST    3.071856358605e+2   
>>>> 1.052252204958e+0  -3.083120039764e+2
>>>>                                 C_LIST    1.052252204958e+0   
>>>> 1.353606645969e+4   0.000000000000e+0
>>>>                                 C_LIST   -3.083120039764e+2   
>>>> 0.000000000000e+0   1.352888082383e+4
>>>>                         &END GLE
>>>>                 &END THERMOSTAT
>>>>                 &PRINT
>>>>                         &ENERGY
>>>>                                 &EACH
>>>>                                         MD 10
>>>>                                 &END EACH
>>>>                         &END ENERGY
>>>>                 &END PRINT
>>>>         &END MD
>>>>         &FREE_ENERGY
>>>>                 &FREE_ENERGY_INFO
>>>>                         &EACH
>>>>                                 MD 1000
>>>>                         &END
>>>>                 &END
>>>>                 &METADYN
>>>>                         &PRINT
>>>>                                 &COLVAR
>>>>                                         COMMON_ITERATION_LEVELS 3
>>>>                                         &EACH
>>>>                                                 MD 1
>>>>                                         &END
>>>>                                 &END
>>>>                                 &HILLS
>>>>                                         COMMON_ITERATION_LEVELS 3
>>>>                                         &EACH
>>>>                                                 MD 1
>>>>                                         &END
>>>>                                 &END
>>>>                         &END
>>>>                 &END METADYN
>>>>         &END FREE_ENERGY
>>>>         &PRINT
>>>>                 &TRAJECTORY
>>>>                         FORMAT XYZ
>>>>                         &EACH
>>>>                                 MD 20
>>>>                         &END EACH
>>>>                 &END TRAJECTORY
>>>>                 &RESTART_HISTORY
>>>>                         &EACH
>>>>                                 MD 10000
>>>>                         &END EACH
>>>>                 &END RESTART_HISTORY
>>>>                 &RESTART OFF
>>>>                 &END RESTART
>>>>         &END PRINT
>>>> &END MOTION
>>>>
>>>> I would be grateful if anyone could take a look to my input file and 
>>>> let me know about the possible way to get the structure converged. I've 
>>>> already relaxed the metal structure before using it for md simulation. 
>>>>  
>>>> Thanks in advance.
>>>>
>>>> Kevin
>>>>
>>>
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