bond problem

John johnb... at gmail.com
Sat Apr 4 21:41:11 UTC 2009


Dear all,

I'm trying to reproduce Blumberger & Sprik’s article. “Quantum versus
classical electron transfer energy as reaction coordinate for aqueous
Ru2+/Ru3+ redox reaction”  I want to calculate Ru2+ and Ru3+ separately. I
am stuck in this file.



-------------------------------------------------------------------------

 &FORCE_EVAL
  METHOD QS
  &DFT
     LSD
     CHARGE +2
     BASIS_SET_FILE_NAME ~/bin/GTH_BASIS1
     POTENTIAL_FILE_NAME ~/bin/GTH_POTENTIALS
    &SCF
      SCF_GUESS ATOMIC
    &END SCF
    &XC
     &XC_FUNCTIONAL
       &LYP
       &END
       &BECKE88
       &END
     &END XC_FUNCTIONAL
    &END XC
  &END DFT
  &SUBSYS
   &CELL
    ABC 9.860 9.860 9.860
    UNIT ANGSTROM
   &END CELL
   &TOPOLOGY
    CONNECTIVITY GENERATE
    &GENERATE
        CREATE_MOLECULES
    &END GENERATE
    COORD_FILE_FORMAT OFF
   &END TOPOLOGY
   &COORD
  Fe       -2.8799089789        4.4833993160       -0.9253798435
  O        -4.5590653502        4.9284583342       -0.0621601829
  H        -4.9705923716        4.3640441785        0.6893891668
  H        -5.3164182399        5.5362415756       -0.2538566219
  O        -6.3299935050        4.6501002553       -3.2165611248
  H        -6.2549146971        3.6508586162       -3.3792673655
  H        -6.9156034477        4.8348081172       -3.9501089172
  O        -2.2309178755        1.9923408769        2.7645911766
  H        -2.1565313777        1.2884476066        3.3749391873
  H        -2.9197925757        2.4899670577        3.2035338211
  O        -6.0770832172       -2.7231315785       -9.5448709624
  H        -6.6824231738       -1.9822385218       -9.4211280474
  H        -5.9382474726       -3.0338301873       -8.6189155739
  O        -1.5590539933        8.4581237145        2.8351416768
  H        -0.7014554610        8.2291741700        2.4524975037
  H        -2.0130061115        8.5474909348        1.9935461408
  O         9.2452622342       -5.2016109500        5.4580407027
  H         9.0803631056       -5.7141148150        4.6416799086
  H         9.9239068093       -4.6374143187        5.0948223542
  O        -2.2747965553       -3.6412773460       -0.5034106904
  H        -1.3309475835       -3.3368322136       -0.4927701592
  H        -2.6785712553       -2.7337453156       -0.3003969352
  O        -5.0150050737       -6.7585442027        1.9265699321
  H        -5.1775069842       -7.7010260951        1.7351149107
  H        -5.8697740333       -6.3925551219        2.1581907946
  O         0.8447530721        6.9676594900       11.9177287714
  H         1.7073334916        7.3677191845       11.6947056467
  H         0.6518913920        6.5141851347       11.1177738640
  O         6.0591575870        2.6714044751       -1.4726489030
  H         5.3474665764        2.0757487291       -1.1127385014
  H         6.4466468961        2.0834641415       -2.1735884409
  O         3.4899901096       -1.6971208479       -4.9827700523
  H         3.7505437278       -2.0037236132       -5.8540717308
  H         4.1006777437       -2.1268748806       -4.4328135502
  O        -1.9498492896        3.8218715791        0.7845270001
  H        -1.5328361779        4.4385739266        1.4442998839
  H        -2.0488871006        2.9605980239        1.2847914463
  O         0.9321859840       -7.8126933636       -7.4250105857
  H         0.0329414295       -8.0583782013       -7.5266562638
  H         1.1486171832       -8.1200037817       -6.5120872061
  O        -1.2177439540        3.9800638489       -1.8131933683
  H        -0.6840991767        3.1313826129       -1.5906664292
  H        -0.9145330384        4.0982865398       -2.7613003118
  O        -3.3284227931       -1.8974729757        7.2635935278
  H        -2.4263964010       -1.6247806670        6.8788457601
  H        -3.8045549804       -1.0362892279        7.1060434158
  O         3.1479370099       -0.6458937922       -2.5276483725
  H         3.3884480789       -0.8514820589       -3.4557508136
  H         3.6344722272       -1.3774434262       -2.0751013265
  O         7.1879953337       -8.9239121082      -13.3442298597
  H         6.8446671365       -8.5711562075      -14.1613048318
  H         7.7254300021       -9.6624243506      -13.7044807394
  O        -8.6023482493       -3.3193550929       -5.1537580676
  H        -8.7819195227       -3.1689491809       -6.1212676794
  H        -7.8410327266       -2.7039484048       -4.9109258801
  O        -1.6312805667        5.5167292375       -6.9923342866
  H        -0.8056792472        5.7540718563       -6.5608867815
  H        -2.1505132312        6.3409324352       -7.1702717642
  O        -1.1599325173       -1.2492174249        5.5835548423
  H        -0.5586672445       -2.0053137874        5.5852786019
  H        -1.2162000273       -1.1965002980        4.5769153998
  O         0.4507584677        1.9022651399        8.0400381780
  H         0.3803588966        1.5946413528        7.1350748078
  H         0.7456410323        1.1634439653        8.5439230412
  O         2.3267512174       -0.6727042425        1.1854652355
  H         2.5458646034        0.0652573671        1.7955595250
  H         1.4034743190       -0.7956305233        1.3884420398
  O         6.5672661690       -1.0984518909        0.4890215160
  H         6.6148451731       -0.1508625403        0.5933987343
  H         5.6183713508       -1.1822689592        0.6206551821
  O        13.8241697211        1.1652120167       -0.1672218219
  H        13.2121429387        1.9116181141       -0.2940170580
  H        13.1950907565        0.4365600472       -0.0399679561
  O        -7.4988319221       -5.5555520991        1.8185232839
  H        -7.3837127821       -5.7699475363        0.8563643360
  H        -8.1964989733       -6.1053099532        2.1088034849
  O         3.2659641904        1.9791770773        6.1150563807
  H         3.4940757601        1.1736027719        6.5963750850
  H         2.3515019134        1.7588235846        5.7327525956
  O        10.6859668444        0.9023905651        5.3551106427
  H         9.8594127269        0.4030003706        5.2356781202
  H        11.1491058894        0.1555256165        5.7681348240
  O         0.3760363101       -3.1586261422       -0.8543017938
  H         0.5403724685       -2.2421497891       -0.9851024800
  H         1.2122330106       -3.5814031598       -1.0268333285
  O         5.5807230240       -7.1801081002       -5.1191205524
  H         5.3360212979       -6.4482539508       -5.7290439438
  H         4.6785146465       -7.5446958824       -4.8933286755
  O         2.6572577924        3.6535389336       -0.8327578995
  H         2.9537750589        4.1567130338       -1.6386441686
  H         1.8520090260        3.2252090800       -1.1268435488
  O        -5.8148422292       -3.3672919847        2.9400281976
  H        -6.4576770992       -4.0665517099        3.0231423099
  H        -5.0407848682       -3.8319856458        3.2242012598
  O         6.1901471261        5.2539472758       -2.5686945148
  H         5.3182543979        5.0205417149       -2.9790688482
  H         6.2705281827        6.1021482659       -3.1176707935
    &END COORD
     &KIND RU
      BASIS_SET DZV-GTH
      POTENTIAL GTH-PADE-q8
    &END KIND
    &KIND H
      BASIS_SET DZV-GTH
      POTENTIAL GTH-BP-q1
     &END KIND
    &KIND O
      BASIS_SET DZVP-GTH
      POTENTIAL GTH-BP-q6
    &END KIND
  &END SUBSYS
 &END FORCE_EVAL
 &GLOBAL
  PREFERRED_FFT_LIBRARY FFTSG
  EXTENDED_FFT_LENGTHS T
  PROJECT test
  RUN_TYPE GEO_OPT
 &END GLOBAL
 &MOTION
  &MD
   ENSEMBLE NVT
   STEPS 10000
   TIMESTEP 1.0
   TEMPERATURE 300.0
  &THERMOSTAT
   REGION GLOBAL
  &NOSE
   LENGTH 3
   YOSHIDA 3
   TIMECON 1000
   MTS 2
  &END NOSE
  &END
  &PRINT
  &ENERGY
   &EACH
    MD 10
   &END EACH
  &END ENERGY
   &END PRINT
   &END MD
   &PRINT
   &TRAJECTORY
   &EACH
    MD 10
   &END EACH
   &END TRAJECTORY
   &END PRINT
&END MOTION


-------------------------------------





 Thanks in advance
John
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