<div>Dear CP2K experts,</div><div><br /></div><div>In my calculations using the Quickstep method I noticed in some cases slightly different total energies in the newest released version (2026.2) compared to several older versions (e.g. 2024.1). In my more detailed tests I could see that the differences were present when an element with d valence electrons (e.g. gold) was among the atoms. Forces on the atoms in 2026.2 are also slightly different, also the Kohn-Sham gap. You can see my example runs - a gold dimer in a rather arbitrary orthorombic cell. The same input file was used for both the runs.</div><div><br /></div><div>On the positive side, I see that the SCF convergence with the newest CP2K is much easier (less iterations) in cases when the difference in the total energies occurs. I did this kind of test also with graphene (no d electrons) and in this case the energies were identical.</div><div><br /></div><div>My question is if I am doing someting wrong, something which induces the differences in the case of d electrons or if it is a real feature of CP2K 2026.2 that it gives slightly different (lower) total energies in such cases?</div><div><br /></div><div>Thanks for your valued opinions.</div><div><br /></div><div>Best wishes</div><div>Martin Konôpka.</div>
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