why when i use the Mulliken in DFT+U method i get this in the SCF calculation<br /> SCF WAVEFUNCTION OPTIMIZATION<br /><br /> Step Update method Time Convergence Total energy Change<br /> ------------------------------------------------------------------------------<br /> 1 NoMix/Diag. 0.40E+00 2.6 3.24390306 -1110.1516153134 -1.11E+03<br /><br /> *** WARNING in dft_plus_u.F:1468 :: DFT+U energy contibution is negative ***<br /> *** possibly due to unphysical Mulliken charges! ***<br /><br /> 2 Broy./Diag. 0.40E+00 4.3 2.97645132 -1123.1552875487 -1.30E+01<br /><br /> *** WARNING in dft_plus_u.F:1468 :: DFT+U energy contibution is negative ***<br /> *** possibly due to unphysical Mulliken charges! ***<br /><br /> 3 Broy./Diag. 0.40E+00 4.3 2.92722206 -1135.7426405476 -1.26E+01<br /><br /> *** WARNING in dft_plus_u.F:1468 :: DFT+U energy contibution is negative ***<br /> *** possibly due to unphysical Mulliken charges! ***<br /><br /> 4 Broy./Diag. 0.40E+00 4.3 33.48244881 -1138.3027035346 -2.56E+00<br /><br /> *** WARNING in dft_plus_u.F:1468 :: DFT+U energy contibution is negative ***<br /> *** possibly due to unphysical Mulliken charges! ***<br />what can i do ?<div>thanks</div><div><br /></div>
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