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    <p>Dear K.AK,</p>
    <p>I see here at least a few reasons which could impair your
      calculation.</p>
    <p>1. Hybrid functional - do you really need it? Geometries even of
      3d complexes are quite good with GGA, which is tremendously faster
      in periodic calculations. Wouldn't PBE (with dispersion
      correction) fit?<br>
    </p>
    <p>2. GAPW+6-31G? Any specific reason? I would take typical GPW
      together with MOLOPT bases.</p>
    <p>3. Your cell size is >30x30x30 A quite loaded with atoms.
      Surely it will be slow and memory-consuming.</p>
    <p>4. Convergence issues are quite common with metal complexes, some
      efforts could be necessary to overcome.</p>
    <p>Yours,</p>
    <p>Anton<br>
    </p>
    <div class="moz-cite-prefix">Am 23.11.2023 um 10:10 schrieb K.AK:<br>
    </div>
    <blockquote type="cite"
      cite="mid:ac837fd8-7833-4871-a8b1-acf6099ccee5n@googlegroups.com">
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      Dear experts,<br>
      <div><br>
      </div>
      <div>
        <div>I try to optimize MOF structure by performing periodic DFT
          calculations. </div>
        <div><br>
        </div>
        <div>I have performed the calculations under the periodic
          conditions of the attached input file.</div>
        <div><br>
        </div>
        <div>But, the computation time is very long and the convergence
          is not good.</div>
        <div><br>
        </div>
        <div>Please advise about the cp2k simulation method and input
          file.</div>
        <div><br>
        </div>
        <div>
          <div>The input files have been attached below.</div>
          <div><br>
          </div>
        </div>
        <div><br>
        </div>
        <div>Many thanks,<br>
        </div>
        <div>K.AK</div>
      </div>
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