According to cp2k documentation <a href="https://manual.cp2k.org/trunk/CP2K_INPUT/FORCE_EVAL/SUBSYS/KIND.html#POTENTIAL">https://manual.cp2k.org/trunk/CP2K_INPUT/FORCE_EVAL/SUBSYS/KIND.html#POTENTIAL</a> it is possible to set POTENTIAL variable value as ECP, in order to use Effective core potential. I've converted basis set from http://www.tc.uni-koeln.de/PP/clickpse.en.html according to CP2K documentation. The section KIND in my input file is:<div><i> &KIND V<br>BASIS_SET STOLL-PBE<br>POTENTIAL ECP<br>&POTENTIAL<br>V nelec 10<br>V ul<br>2 1.000000000 0.000000000 <br>V S<br>2 14.490000000 178.447971000 <br>2 6.524000000 19.831375000 <br>V P<br>2 14.300000000 109.529763000 <br>2 6.021000000 12.570310000 <br>V D<br>2 17.480000000 -19.219657000 <br>2 5.709000000 -0.642775000 <br>&END<br>&END KIND</i><br></div><div>The basis set in new file is:</div><div><i>V STOLL-PBE<br> 4<br> 2 0 0 7 1 0 # Gauss type functions l=0 set 1 (3s orbital)<br> 12.8432080 0.460448<br> 11.3757530 -0.495309<br> 5.4069740 -0.350821<br> 1.4659270 0.654979<br> 0.5980800 0.582548<br> 0.0887900 0.017081<br> 0.0353180 -0.007455<br> 2 0 0 7 1 0 </i><i># Gauss type functions l=0 set 2 (4s orbital)</i><i><br> 12.8432080 0.126932<br> 11.3757530 -0.139770<br> 5.4069740 -0.089862<br> 1.4659270 0.204669<br> 0.5980800 0.321169<br> 0.0887900 -0.657043<br> 0.0353180 -0.474893<br> 2 1 1 6 0 1 </i><i># Gauss type functions l=1 set 1 (3p orbital)</i><i><br> 31.8898680 0.004658<br> 8.2371780 -0.119249<br> 4.3283730 0.125195<br> 1.5405260 0.620704<br> 0.5280810 0.416780<br> 0.0899620 0.014015<br> 2 2 2 5 1 </i><i># Gauss type functions l=2 set 1 (3d orbital)</i><i><br> 22.6804330 0.031628<br> 6.8613120 0.153807<br> 2.2754450 0.378661<br> 0.7319220 0.507276<br> 0.2007460 0.275921</i><br></div><div><br></div><div>CP2K starts normally but exit with error message:</div><div> <i>CPASSERT failed qs_mo_types.F:295</i><br></div><div>By checking source code I have error here:</div><div> <i>CPASSERT(nmo >= nomo)</i><br></div><div><br></div><div>Could someone kindly give a working example for force calculations with ECP potential.</div><div><br></div><div>Many thx in advance,<br>Eugene</div>
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