<div dir="ltr">Dear All,<div><br></div><div>I am trying to do non-periodic GAPW calculation on Fe atom using Ahlrichs-def2-QZVP basis set. I have specified the multiplicity as 5 (4 unpaired electrons, 2*S+1 = 5) in the &DFT section. Why does the output say:</div><div><br></div><div>







<p class="p1"><span class="s1">   Multiplicity                                                   not specified</span></p>
<p class="p1"><span class="s1">    S      2.00  2.00  2.00  2.00</span></p>
<p class="p1"><span class="s1">    P      6.00  6.00</span></p>
<p class="p1"><span class="s1">    D      6.00</span></p><p class="p1"><span class="s1">---------</span></p><p class="p1"><span class="s1">  Integrated absolute spin density  :                               2.9072369397</span></p><p class="p1"><span class="s1">  Ideal and single determinant S**2 :                    6.000000       6.014181</span></p><p class="p2"><span class="s1"> </span></p><p class="p2"><span class="s1"> </span></p><p class="p1"><span class="s1"> MULLIKEN POPULATION ANALYSIS      </span></p><p class="p2"><span class="s1"> </span></p><p class="p1"><span class="s1"> #  Atom  Element  Kind  Atomic population (alpha,beta)   Net charge  Spin moment</span></p><p class="p1"><span class="s1">       1     Fe       1                   15.000000    11.000000     0.000000     4.000000</span></p><p class="p1"><span class="s1">















</span></p><p class="p1"><span class="s1"> # Total charge and spin        15.000000    11.000000     0.000000     4.000000</span></p><p class="p1"><span class="s1"><br></span></p><p class="p1"><span class="s1"><br></span></p><p class="p1"><span class="s1">What am I doing wrong? Please help. This is how my input looks like:</span></p><p class="p1"><span class="s1"><br></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">&GLOBAL</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">  PROJECT Fe_12</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">  RUN_TYPE ENERGY</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">  PRINT_LEVEL MEDIUM</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">  WALLTIME 86400</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">&END GLOBAL</font></span></p><p class="p2"><font size="1" face="courier new, monospace" color="#674ea7"><span class="s1"></span><br></font></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">&FORCE_EVAL</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">  METHOD Quickstep</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">  &DFT</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">    BASIS_SET_FILE_NAME /share/apps/cp2k/cp2k/tests/QS/EMSL_BASIS_SETS</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">    POTENTIAL_FILE_NAME /share/apps/cp2k/cp2k/tests/QS/POTENTIAL</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">    CHARGE 0</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">    MULTIPLICITY 5</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">    UKS T</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">    &MGRID</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">      CUTOFF 400</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">      REL_CUTOFF 60</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">    &END MGRID</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">    &QS</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">      METHOD GAPW</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">      EPS_DEFAULT 1.0E-12</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">    &END QS</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">    &SCF</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">      MAX_SCF 500</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">      &OUTER_SCF</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">        EPS_SCF 1.0E-6</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">        MAX_SCF 60</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">      &END OUTER_SCF</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">    &END SCF</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">    &POISSON</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">      PERIODIC NONE</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">      PSOLVER WAVELET</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">    &END POISSON</font></span></p><p class="p2"><font size="1" face="courier new, monospace" color="#674ea7"><span class="s1"></span></font></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">    &XC</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">      &XC_FUNCTIONAL PBE</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">      &END XC_FUNCTIONAL</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">      &XC_GRID</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">        XC_SMOOTH_RHO NN10</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">        XC_DERIV SPLINE2_SMOOTH</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">      &END XC_GRID</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">    &END XC</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">  &END DFT</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">  &SUBSYS</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">    &CELL</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">      ABC 7.00 7.00 7.00</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">      PERIODIC NONE</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">    &END CELL</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">    &COORD</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">      Fe    0.0000    0.0000    0.0000</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">    &END COORD</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">    &TOPOLOGY</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">      &CENTER_COORDINATES</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">      &END</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">    &END</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">    &KIND Fe</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">      BASIS_SET Ahlrichs-def2-QZVP</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">      POTENTIAL ALL</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">    &END KIND</font></span></p><p class="p2"><font size="1" face="courier new, monospace" color="#674ea7"><span class="s1"></span></font></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">  &END SUBSYS</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">















































































</font></span></p><p class="p1"><span class="s1"><font size="1" face="courier new, monospace" color="#674ea7">&END FORCE_EVAL</font></span></p></div></div>