[CP2K-user] [CP2K:18071] SCF run NOT converged

eitan eidelstein eitan.eidelstein at gmail.com
Tue Nov 22 12:55:07 UTC 2022


So, your suggestion is not to use k points at all (or only Gamma point)?

On Tuesday, November 22, 2022 at 1:03:31 PM UTC+2 Matthias Krack wrote:

> A supercell with at least ~12A in each direction is most likely more 
> efficient than a primitive cell with a large number of k points. 
> CP2K/Quickstep employs localized Gaussian functions as basis set and their 
> interaction range is not impacted by the cell size. Therefore many 
> computational steps do not benefit from a small cell. On the other hand, 
> several features are not yet available with k points and thus, if k points 
> are dispensable, more feature are available.
>
>  
>
> *From: *cp... at googlegroups.com <cp... at googlegroups.com> on behalf of 
> eitan eidelstein <eitan.ei... at gmail.com>
> *Date: *Tuesday, 22 November 2022 at 11:44
> *To: *cp2k <cp... at googlegroups.com>
> *Subject: *Re: [CP2K:18069] SCF run NOT converged
>
> Thanks, I will try those.
>
> Can you explain why MULTIPLE_UNIT_CELL 3 3 3 is helping for PERIODIC XYZ? 
> and why 3 instead of 2?
>
>  
>
> On Monday, November 21, 2022 at 6:26:18 PM UTC+2 Matthias Krack wrote:
>
> Hi
>
> · try a supercell, e.g. 3x3x3 (MULTIPLE_UNIT_CELL keyword in &CELL and 
> &TOPOLOGY section), instead of k points
>
> · Increase the cutoff to 400 Ry
>
> · Increase the smearing temperature if needed
>
>  
>
> HTH
>
>  
>
> M.
>
>  
>
> *From: *cp... at googlegroups.com <cp... at googlegroups.com> on behalf of 
> eitan eidelstein <eitan.ei... at gmail.com>
> *Date: *Monday, 21 November 2022 at 14:15
> *To: *cp2k <cp... at googlegroups.com>
> *Subject: *[CP2K:18066] SCF run NOT converged
>
> Hi,
>
> This calculation is not converging.
>
> I will be delighted for any sugestion.
>
> Thanks, 
>
> Eitan.
>
>  
>
> &FORCE_EVAL
>   METHOD Quickstep              
>   &DFT
>     BASIS_SET_FILE_NAME  BASIS_MOLOPT_UZH 
>     #BASIS_SET_FILE_NAME BASIS_SET
>     #POTENTIAL_FILE_NAME  POTENTIAL
>     POTENTIAL_FILE_NAME POTENTIAL_UZH
>     CHARGE 0
>     SPIN_POLARIZED .TRUE. # SPIN_POLIRIZED 
>     MULTIPLICITY 1
>     RELAX_MULTIPLICITY 0.1
>     &MGRID
>       CUTOFF 200
>     &END MGRID
>     &POISSON                
>       PERIODIC XYZ
>       poisson_solver periodic
>     &END POISSON
>     &SCF
>          SCF_GUESS ATOMIC
>          EPS_SCF 1.0E-10
>          MAX_SCF 1000
>          ADDED_MOS 100
>          &DIAGONALIZATION
>             ALGORITHM STANDARD
>             EPS_ADAPT 0.001
>          &END DIAGONALIZATION
>          &SMEAR  ON
>             METHOD FERMI_DIRAC
>             ELECTRONIC_TEMPERATURE [K] 300
>          &END SMEAR
>
>        &MIXING
>           METHOD BROYDEN_MIXING
>           ALPHA 0.2
>           BETA 1.5
>           NBROYDEN 8
>        &END MIXING
>
>     &END SCF
>     &XC         
>
>       &XC_FUNCTIONAL PBE 
>       &END XC_FUNCTIONAL
>     &END XC
>     &KPOINTS
>        SCHEME  MONKHORST-PACK  30 30 30   
>     &END KPOINTS
>
>     &PRINT 
>        &DOS
>           FILENAME dos 
>           NDIGITS 14
>        &END DOS
>        &PDOS
>           FILENAME pdos
>           # print all projected DOS available:
>           NLUMO -1
>           # split the density by quantum number:
>           COMPONENTS .TRUE.
>        &END PDOS
>     &END PRINT
>   &END DFT
>   &SUBSYS
>     &PRINT
>       &SYMMETRY
>         ALL
>       &END
>     &END PRINT
>     &CELL  # 8.104532945 4.0522664725
>       A [bohr] 8.104532945  4.0522664725 4.0522664725
>       B [bohr] 4.0522664725 8.104532945  4.0522664725
>       C [bohr] 4.0522664725 4.0522664725 8.104532945
>       PERIODIC XYZ
>     &END CELL
>     &KIND Co1
>       ELEMENT Co
>       BASIS_SET DZVP-MOLOPT-PBE-GTH-q17
>       #BASIS_SET DZV-GTH-PADE 
>       #POTENTIAL GTH-PBE
>       POTENTIAL GTH-PBE-q17
>       #&BS
>       #  &ALPHA
>       #  &END
>       #  &BETA
>       #  &END
>       #&END BS
>       #MAGNETIZATION 1.0
>     &END KIND
>     &KIND Co2
>       ELEMENT Co
>       BASIS_SET DZVP-MOLOPT-PBE-GTH-q17
>       #BASIS_SET DZV-GTH-PADE
>       #POTENTIAL GTH-PBE
>       POTENTIAL GTH-PBE-q17
>       #&BS
>       #  &ALPHA
>       #  &END
>       #  &BETA
>       #  &END
>       #&END BS
>       #MAGNETIZATION -1.0
>     &END KIND
>
>     &KIND O
>       ELEMENT O
>       BASIS_SET DZVP-MOLOPT-PBE-GTH-q6
>       #BASIS_SET DZVP-GTH-PADE
>       #POTENTIAL GTH-PBE
>       POTENTIAL GTH-PBE-q6
>     &END KIND
>     &COORD
>       SCALED
>         Co1 0.0 0.0 0.0
>         Co2 0.5 0.5 0.5
>         O 0.25 0.25 0.25
>         O 0.75 0.75 0.75
>     &END COORD
>
>   &END SUBSYS
> &END FORCE_EVAL
> &GLOBAL
>   PROJECT CoO
>   RUN_TYPE ENERGY
>   PRINT_LEVEL MEDIUM
> &END GLOBAL
>
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