[CP2K-user] [CP2K:17458] Re: orthogonal lattice gives same exact energy as strained--PBC being applied?

Matt Watkins mattwatkinsuk at gmail.com
Wed Aug 10 15:06:03 UTC 2022


Hi,
the energy does change but in the SCF loop it is given with reduced number 
of figures

(base) mattw at DESKTOP:~/NMR/nmr1$ grep 'Total energy:' *out
  Total energy:                                           
 -23467.23741478025477
(base) mattw at DESKTOP:~/NMR/nmr1$ cd madeorthogonal/
(base) mattw at DESKTOP:~/NMR/nmr1/madeorthogonal$ grep 'Total energy:' *out
  Total energy:                                           
 -23467.23741478026932

You could test the orthogonal / nonorthogonal hypothesis on a smaller 
system! I suspect you are correct that there is an assumption in one of the 
operators that the box is orthogonal.
Matt

On Wednesday, 10 August 2022 at 14:23:05 UTC+1 reco... at gmail.com wrote:

> This is too weird. I just ran across the strangest thing. I am trying to 
> figure out why nmr is not working--I get things like at the bottom (see 
> NMR). So I wanted to see if the problem was that the cell was not 
> orthogonal, so I strained the cell to make it orthogonal without changing 
> the positions of the atoms in the cell. It gave exactly the same energy as 
> if periodic boundary conditions (PBC) are not being used!! 
>
> CP2K| version string:                 CP2K version 2022.1 (Development 
> Version)
>  CP2K| source code revision number:                                 
>  git:2de0518
>  CP2K| cp2kflags: omp libint fftw3 libxc pexsi elpa parallel mpi3 
> scalapack cosm
>  CP2K|            a xsmm max_contr=4 plumed2 spglib mkl sirius libvori 
> libbqb
>
>
> *Unmodified:*
> CELL_TOP| Volume [angstrom^3]:                                     
>  1195.278954
>  CELL_TOP| Vector a [angstrom    12.264     0.000     0.000   |a| =   
>  12.263717
>  CELL_TOP| Vector b [angstrom    -0.012    12.207     0.000   |b| =   
>  12.206735
>  CELL_TOP| Vector c [angstrom     0.010    -0.018     7.985   |c| =     
> 7.984530
>  CELL_TOP| Angle (b,c), alpha [degree]:                               
>  90.131000
>  CELL_TOP| Angle (a,c), beta  [degree]:                               
>  89.925000
>  CELL_TOP| Angle (a,b), gamma [degree]:                               
>  90.057000
>  CELL_TOP| Numerically orthorhombic:                                       
>    NO
>  
>    43 OT DIIS     0.15E+00   69.7     4.9884E-12    *-23467.2374147803* 
>  1.09E-11
>
>   *** SCF run converged in    43 steps ***
>
>
>   Electronic density on regular grids:      -1079.0687219005      530.
> 9312780995 <(931)%20278-0995>
>   Core density on regular grids:             1610.0000000000       
>  0.0000000000
>   Hard and soft densities (Lebedev):        -8290.7114735740    -7759.
> 7802260448 <(780)%20226-0448>
>   Total Rho_soft + Rho1_hard - Rho1_soft    -1609.9999694297
>   Total charge density (r-space):               0.0000305703
>   Total Rho_soft + Rho0_soft (g-space):         0.0000329359
>
>   Overlap energy of the core charge distribution:               
> 0.00000104541775
>   Self energy of the core charge distribution:             
> -14539.93646441583769
>   Core Hamiltonian energy:                                 
>  -9218.15471874043033
>   Hartree energy:                                           
>  3922.43227166635324
>   Exchange-correlation energy:                               
> -646.66529311302361
>
>   GAPW| Exc from hard and soft atomic rho1:                 
> -1396.13990389988862
>   GAPW| local Eh = 1 center integrals:                     
>  -1588.77330732284054
>
>   Total energy:                                           
>  -23467.23741478025477
>
>   outer SCF iter =    1 RMS gradient =   0.50E-11 energy =     
> -23467.2374147803
>
>
> *Made orthogonal*
> CELL_TOP| Volume [angstrom^3]:                                     
>  1200.135541
>  CELL_TOP| Vector a [angstrom    12.260     0.000     0.000   |a| =   
>  12.260000
>  CELL_TOP| Vector b [angstrom     0.000    12.260     0.000   |b| =   
>  12.260000
>  CELL_TOP| Vector c [angstrom     0.000     0.000     7.985   |c| =     
> 7.984530
>  CELL_TOP| Angle (b,c), alpha [degree]:                               
>  90.000000
>  CELL_TOP| Angle (a,c), beta  [degree]:                               
>  90.000000
>  CELL_TOP| Angle (a,b), gamma [degree]:                               
>  90.000000
>  CELL_TOP| Numerically orthorhombic:                                       
>   YES
>
> *Note even volume is different*
>
>   44 OT DIIS     0.15E+00   69.8     4.5499E-12   * -23467.2374147803 *
> -3.27E-11
> EXACT SAME AS ABOVE!
>   *** SCF run converged in    44 steps ***
>
>
>   Electronic density on regular grids:      -1079.0687219005      530.
> 9312780995 <(931)%20278-0995>
>   Core density on regular grids:             1610.0000000000       
>  0.0000000000
>   Hard and soft densities (Lebedev):        -8290.7115342968    -7759.
> 7802867676 <(780)%20286-7676>
>   Total Rho_soft + Rho1_hard - Rho1_soft    -1609.9999694297
>   Total charge density (r-space):               0.0000305703
>   Total Rho_soft + Rho0_soft (g-space):         0.0000329359
>
>   Overlap energy of the core charge distribution:               
> 0.00000104541775
>   Self energy of the core charge distribution:             
> -14539.93646441583769
>   Core Hamiltonian energy:                                 
>  -9218.15471874045579
>   Hartree energy:                                           
>  3922.43227166633824
>   Exchange-correlation energy:                               
> -646.66529311301952
>
>   GAPW| Exc from hard and soft atomic rho1:                 
> -1396.13990389988476
>   GAPW| local Eh = 1 center integrals:                     
>  -1588.77330732282644
>
>   Total energy:                                           
>  -23467.23741478026932
>
>   outer SCF iter =    1 RMS gradient =   0.45E-11 energy =     
> -23467.2374147803
>   outer SCF loop converged in   1 iterations or   44 steps
>
>
> Note both show
> POISSON| Solver                                                       
>  PERIODIC
>  POISSON| Periodicity                                                     
>    XYZ
> in input .INC FILES
>        PERIODIC  XYZ FOR BOTH
> seems cell periodicity is not output?
>
> Any help appreciated! Files attached.
> ----NMR
>
> Shielding atom at atomic positions. # tensors printed 165
>
> 1O O 2.390434 2.226322 0.031347
>
> SIGMA from SOFT J
>
> XX = ********** XY = ********** XZ = **********
>
> YX = ********** YY = ********** YZ = **********
>
> ZX = ********** ZY = ********** ZZ = **********
>
> SIGMA from LOCAL J
>
> XX = -5315.3694 XY = ********** XZ = **********
>
> YX = 98.5820 YY = ********** YZ = **********
>
> ZX = 1884.0679 ZY = ********** ZZ = **********
>
> SIGMA TOTAL
>
> XX = ********** XY = ********** XZ = **********
>
> YX = ********** YY = ********** YZ = **********
>
> ZX = ********** ZY = ********** ZZ = **********
>
> ISOTROPY = ************ ANISOTROPY = ************
>

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