[CP2K-user] [CP2K:16245] The SCF iteration rate in QM/MM is significantly different from that in vacuo

方业广 bnuyeguangfang at gmail.com
Wed Nov 17 02:14:19 UTC 2021


Dear all, 

      I have tested the molecular dynamics of the same molecule in the gas 
phase and in the QM/MM environment, and found that the SCF iteration of 
QM/MM is dozens of times slower than that of vacuum.  Is this 
reasonable? As far as I know, the coupling between QM and MM should not 
affect the speed so much. 

The input and output files for the tests are  attached.




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 DBCSR| CPU Multiplication driver                                           XSMM
 DBCSR| Multrec recursion limit                                              512
 DBCSR| Multiplication stack size                                           1000
 DBCSR| Maximum elements for images                                    UNLIMITED
 DBCSR| Multiplicative factor virtual images                                   1
 DBCSR| Use multiplication densification                                       T
 DBCSR| Multiplication size stacks                                             3
 DBCSR| Use memory pool for CPU allocation                                     F
 DBCSR| Number of 3D layers                                               SINGLE
 DBCSR| Use MPI memory allocation                                              F
 DBCSR| Use RMA algorithm                                                      F
 DBCSR| Use Communication thread                                               T
 DBCSR| Communication thread load                                             87
 DBCSR| MPI: My node id                                                        0
 DBCSR| MPI: Number of nodes                                                  64
 DBCSR| OMP: Current number of threads                                         1
 DBCSR| OMP: Max number of threads                                             1
 DBCSR| Split modifier for TAS multiplication algorithm                  1.0E+00


  **** **** ******  **  PROGRAM STARTED AT               2021-11-17 09:47:43.330
 ***** ** ***  *** **   PROGRAM STARTED ON                      ja0802.para.bscc
 **    ****   ******    PROGRAM STARTED BY                               scb3056
 ***** **    ** ** **   PROGRAM PROCESS ID                                116292
  **** **  *******  **  PROGRAM STARTED IN /public1/home/scb3056/fangyg/test/for
                                           um

 CP2K| version string:                                          CP2K version 8.1
 CP2K| source code revision number:                                  git:0b61f2f
 CP2K| cp2kflags: omp libint fftw3 libxc parallel mpi3 scalapack xsmm max_contr=
 CP2K|            4 mkl
 CP2K| is freely available from                            https://www.cp2k.org/
 CP2K| Program compiled at                          Mon Aug 16 10:31:22 CST 2021
 CP2K| Program compiled on                                       ln131.para.bscc
 CP2K| Program compiled for                           Linux-x86-64-intel-minimal
 CP2K| Data directory path                    /public1/soft/cp2k/cp2k-8.1.0/data
 CP2K| Input file name                                                    md.inp
 
 GLOBAL| Force Environment number                                              1
 GLOBAL| Basis set file name                                        BASIS_MOLOPT
 GLOBAL| Potential file name                                           POTENTIAL
 GLOBAL| MM Potential file name                                     MM_POTENTIAL
 GLOBAL| Coordinate file name                                        complex.pdb
 GLOBAL| Method name                                                        CP2K
 GLOBAL| Project name                                                         MD
 GLOBAL| Preferred FFT library                                             FFTW3
 GLOBAL| Preferred diagonalization lib.                                       SL
 GLOBAL| Run type                                                             MD
 GLOBAL| All-to-all communication in single precision                          F
 GLOBAL| FFTs using library dependent lengths                                  F
 GLOBAL| Global print level                                                  LOW
 GLOBAL| MPI I/O enabled                                                       T
 GLOBAL| Total number of message passing processes                            64
 GLOBAL| Number of threads for this process                                    1
 GLOBAL| This output is from process                                           0
 GLOBAL| CPU model name                          AMD EPYC 7452 32-Core Processor
 GLOBAL| CPUID                                                              1002

 MEMORY| system memory details [Kb]
 MEMORY|                        rank 0           min           max       average
 MEMORY| MemTotal            264056840     264056840     264056840     264056840
 MEMORY| MemFree             240031296     240031296     240054260     240053639
 MEMORY| Buffers                     0             0             0             0
 MEMORY| Cached                9263668       9240356       9263668       9241307
 MEMORY| Slab                  1656972       1656972       1656972       1656972
 MEMORY| SReclaimable           273912        273912        273912        273912
 MEMORY| MemLikelyFree       249568876     249568528     249569280     249568859



                      ************* ******** ***********   
                     ************* **********************  
                     ****     **** ****      ***********   
                     ******** ****  *******     ****       
                     *******  ****   *******   ****        
                     ****     ****       ****  ****        
                     ****     **** **********  ****        
                      ****     **** ********    ****       
                     FRONTIERS IN SIMULATION TECHNOLOGY    
                                                           
                        C.J. Mundy, S. Balasubramanian,    
                     Ken Bagchi, J. Hutter, Ari Seitsonen  
                      IFW Kuo, T. Laino, J. VandeVondele   
                                 Version 1.0               

                                                           


 EWALD| Summation is done by:                                               SPME
 EWALD| Alpha parameter [       ANGSTROM^-1]                              0.4000
 EWALD| Real Space Cutoff [          ANGSTROM]                            8.4348
 EWALD| G-space max. Miller index                         80        80        80
 EWALD| Spline interpolation order                                             6
          ----------------------------------------------------------------------
 COLVARS| COLVAR INPUT INDEX:        1
 COLVARS| BOND          >>> ATOMS:                                     5       8
          ----------------------------------------------------------------------
 
 FORCEFIELD| WARNING: A non Critical ForceField parameter is missing! CP2K GOES!
 FORCEFIELD| Non critical parameters are:Urey-Bradley,Torsions,Impropers, Opbends and 1-4
 FORCEFIELD| All missing parameters will not contribute to the potential energy!
 FORCEFIELD| Activate the print key FF_INFO to have a list of missing parameters
 
 CHARGE_INFO| Total Charge of the Classical System:                    -0.000000

 SPLINE_INFO| Generating 28 splines for NONBONDED14 interactions 
              Due to 7 different atomic kinds
  ...2  ...4  ...6  ...8  ...10  ...12  ...14  ...16  ...18  ...20  ...22
  ...24  ...26  ...28
 SPLINE_INFO| Number of unique splines computed:            12
 SPLINE_INFO| Done

 SPLINE_INFO| Generating 28 splines for NONBONDED interactions 
              Due to 7 different atomic kinds
  ...2  ...4  ...6  ...8  ...10  ...12  ...14  ...16  ...18  ...20  ...22
  ...24  ...26  ...28
 SPLINE_INFO| Number of unique splines computed:            12
 SPLINE_INFO| Done

 *******************************************************************************
 *******************************************************************************
 **                                                                           **
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 **    ##   ##            ##          ##              ##                      **
 **   ##     ##                       ##            ######                    **
 **   ##     ##  ##   ##  ##   #####  ##  ##   ####   ##    #####    #####    **
 **   ##     ##  ##   ##  ##  ##      ## ##   ##      ##   ##   ##  ##   ##   **
 **   ##  ## ##  ##   ##  ##  ##      ####     ###    ##   ######   ######    **
 **    ##  ###   ##   ##  ##  ##      ## ##      ##   ##   ##       ##        **
 **     #######   #####   ##   #####  ##  ##  ####    ##    #####   ##        **
 **           ##                                                    ##        **
 **                                                                           **
 **                                                ... make the atoms dance   **
 **                                                                           **
 **            Copyright (C) by CP2K developers group (2000 - 2020)           **
 **                      J. Chem. Phys. 152, 194103 (2020)                    **
 **                                                                           **
 *******************************************************************************


 TOTAL NUMBERS AND MAXIMUM NUMBERS

  Total number of            - Atomic kinds:                                   3
                             - Atoms:                                         10
                             - Shell sets:                                    10
                             - Shells:                                        46
                             - Primitive Cartesian functions:                 50
                             - Cartesian basis functions:                    122
                             - Spherical basis functions:                    114

  Maximum angular momentum of- Orbital basis functions:                        2
                             - Local part of the GTH pseudopotential:          2
                             - Non-local part of the GTH pseudopotential:      0


 SCF PARAMETERS         Density guess:                                   RESTART
                        --------------------------------------------------------
                        max_scf:                                             256
                        max_scf_history:                                       0
                        max_diis:                                              4
                        --------------------------------------------------------
                        eps_scf:                                        1.00E-05
                        eps_scf_history:                                0.00E+00
                        eps_diis:                                       1.00E-01
                        eps_eigval:                                     1.00E-05
                        --------------------------------------------------------
                        level_shift [a.u.]:                                 0.00
                        --------------------------------------------------------
                        No outer SCF

 *******************************************************************************
 *******************************************************************************
 **                                                                           **
 **             #######  ##     ## ##     ## ##     ##                        **
 **            ##     ## ###   ### ###   ### ###   ###                        **
 **            ##     ## #### #### #### #### #### ####                        **
 **            ##     ## ## ### ## ## ### ## ## ### ##                        **
 **            ##  ## ## ##     ## ##     ## ##     ##                        **
 **            ##    ##  ##     ## ##     ## ##     ##  T.Laino and F.Mohamed **
 **             ##### ## ##     ## ##     ## ##     ##  2005 - 2015           **
 **                                                                           **
 **                                                     Calculation Started.. **
 *******************************************************************************
 *******************************************************************************

 METADYN| Meta Dynamics Protocol 
 METADYN| Number of interval time steps to spawn hills                        50
 METADYN| Number of previously spawned hills                                   0
 METADYN| Spawning the Hills 
 METADYN| Height of the Spawned Gaussian                                   0.000
 METADYN| Number of collective variables                                       1
          ----------------------------------------------------------------------
 METAVARS| Collective Variable Number                                          1
 METAVARS| Scaling factor                                               0.056692
 METAVARS| Number of Walls present                                             2

 METAVARS| Wall Number:              1           Type of Wall:        REFLECTIVE
 METAVARS| Wall direction                                              WALL_PLUS
 METAVARS| Wall location                                                4.440856

 METAVARS| Wall Number:              2           Type of Wall:        REFLECTIVE
 METAVARS| Wall direction                                             WALL_MINUS
 METAVARS| Wall location                                                2.267671
          ----------------------------------------------------------------------
 
 MD_PAR| Molecular dynamics protocol (MD input parameters)
 MD_PAR| Ensemble type                                                       NVT
 MD_PAR| Number of time steps                                                  3
 MD_PAR| Time step [fs]                                                 1.000000
 MD_PAR| Temperature [K]                                              300.000000
 MD_PAR| Temperature tolerance [K]                                      0.000000
 MD_PAR| Print MD information every                                    1 step(s)
 MD_PAR| File type   Print frequency [steps]                          File names
 MD_PAR| Coordinates          1                                         traj.xyz
 MD_PAR| Velocities           1                                     MD-vel-1.xyz
 MD_PAR| Energies             1                                        MD-1.ener
 MD_PAR| Dump                 1                                     MD-1.restart

 ROT| Rotational analysis information
 ROT| Principal axes and moments of inertia [a.u.]
 ROT|                           1                   2                   3
 ROT| Eigenvalues      3.88048832733E+10   3.95934872685E+10   4.02510649601E+10
 ROT|      x              0.998201731624      0.051426277598     -0.030800015501
 ROT|      y             -0.059597866692      0.906562688808     -0.417842297460
 ROT|      z              0.006434070886      0.418926520089      0.907997342231
 ROT| Number of rotovibrational vectors                                        6

 DOF| Calculation of degrees of freedom
 DOF| Number of atoms                                                       4594
 DOF| Number of intramolecular constraints                                     0
 DOF| Number of intermolecular constraints                                     0
 DOF| Invariants (translations + rotations)                                    3
 DOF| Degrees of freedom                                                   13779

 DOF| Restraints information
 DOF| Number of intramolecular restraints                                      0
 DOF| Number of intermolecular restraints                                      0

 THERMOSTAT| Thermostat information for PARTICLES
 THERMOSTAT| Type of thermostat                               Nose-Hoover-Chains
 THERMOSTAT| Nose-Hoover-Chain length                                          3
 THERMOSTAT| Nose-Hoover-Chain time constant [fs]                     100.000000
 THERMOSTAT| Order of Yoshida integrator                                       3
 THERMOSTAT| Number of multiple time steps                                     2
 THERMOSTAT| Initial potential energy                         0.000000000000E+00
 THERMOSTAT| Initial kinetic energy                           0.475022301493E-03
 THERMOSTAT| End of thermostat information for PARTICLES

 MD_VEL| Velocities initialization
 MD_VEL| Initial temperature [K]                                      300.000000
 MD_VEL| COM velocity            -0.0000000000    -0.0000000000    -0.0000000000

  Translating the system in order to center the QM fragment in the QM box.

 Number of electrons:                                                         48
 Number of occupied orbitals:                                                 24
 Number of molecular orbitals:                                                24

 Number of orbital functions:                                                114
 Number of independent orbital functions:                                    114

 Extrapolation method: initial_guess

 *** WARNING in qs_initial_guess.F:309 :: User requested to restart the   ***
 *** wavefunction from the file named: MD-RESTART.wfn. This file does not ***
 *** exist. Please check the existence of the file or change properly the ***
 *** value of the keyword WFN_RESTART_FILE_NAME. Calculation continues    ***
 *** using ATOMIC GUESS.                                                  ***



 SCF WAVEFUNCTION OPTIMIZATION

  ----------------------------------- OT ---------------------------------------
  Minimizer      : DIIS                : direct inversion
                                         in the iterative subspace
                                         using   7 DIIS vectors
                                         safer DIIS on
  Preconditioner : FULL_SINGLE_INVERSE : inversion of 
                                         H + eS - 2*(Sc)(c^T*H*c+const)(Sc)^T
  Precond_solver : DEFAULT
  stepsize       :    0.08000000                  energy_gap     :    0.08000000
  eps_taylor     :   0.10000E-15                  max_taylor     :             4
  ----------------------------------- OT ---------------------------------------

  Step     Update method      Time    Convergence         Total energy    Change
  ------------------------------------------------------------------------------
     1 OT DIIS     0.80E-01    6.0     0.16007137      -112.1488486533 -1.12E+02
     2 OT DIIS     0.80E-01    3.2     0.10289018      -114.9512177831 -2.80E+00
     3 OT DIIS     0.80E-01    3.2     0.06910800      -116.1316481868 -1.18E+00
     4 OT DIIS     0.80E-01    3.2     0.05160064      -117.0607653975 -9.29E-01
     5 OT DIIS     0.80E-01    3.2     0.03318113      -117.6851558299 -6.24E-01
     6 OT DIIS     0.80E-01    3.2     0.02662863      -117.8354762340 -1.50E-01
     7 OT DIIS     0.80E-01    3.2     0.01737838      -118.0378220901 -2.02E-01
     8 OT DIIS     0.80E-01    3.2     0.01148663      -118.1358287526 -9.80E-02
     9 OT DIIS     0.80E-01    3.2     0.00871590      -118.1879631232 -5.21E-02
    10 OT DIIS     0.80E-01    3.2     0.00586993      -118.2117692138 -2.38E-02
    11 OT DIIS     0.80E-01    3.2     0.00442134      -118.2274686274 -1.57E-02
    12 OT DIIS     0.80E-01    3.2     0.00323829      -118.2363652142 -8.90E-03
    13 OT DIIS     0.80E-01    3.2     0.00238978      -118.2425174726 -6.15E-03
    14 OT DIIS     0.80E-01    3.2     0.00184652      -118.2455302170 -3.01E-03
    15 OT DIIS     0.80E-01    3.2     0.00140522      -118.2475262554 -2.00E-03
    16 OT DIIS     0.80E-01    3.2     0.00112472      -118.2487631427 -1.24E-03
    17 OT DIIS     0.80E-01    3.2     0.00090748      -118.2495449265 -7.82E-04
    18 OT DIIS     0.80E-01    3.2     0.00073238      -118.2500676834 -5.23E-04
    19 OT DIIS     0.80E-01    3.2     0.00060771      -118.2504537585 -3.86E-04
    20 OT DIIS     0.80E-01    3.2     0.00051078      -118.2507357619 -2.82E-04
    21 OT DIIS     0.80E-01    3.2     0.00044551      -118.2509072153 -1.71E-04
    22 OT DIIS     0.80E-01    3.2     0.00038139      -118.2510687779 -1.62E-04
    23 OT DIIS     0.80E-01    3.2     0.00032880      -118.2511922294 -1.23E-04
    24 OT DIIS     0.80E-01    3.2     0.00029120      -118.2512676739 -7.54E-05
    25 OT DIIS     0.80E-01    3.2     0.00025435      -118.2513462350 -7.86E-05
    26 OT DIIS     0.80E-01    3.2     0.00022785      -118.2513969240 -5.07E-05
    27 OT DIIS     0.80E-01    3.2     0.00020223      -118.2514417142 -4.48E-05
    28 OT DIIS     0.80E-01    3.2     0.00017913      -118.2514811192 -3.94E-05
    29 OT DIIS     0.80E-01    3.2     0.00015217      -118.2515190006 -3.79E-05
    30 OT DIIS     0.80E-01    3.2     0.00012977      -118.2515455258 -2.65E-05
    31 OT DIIS     0.80E-01    3.2     0.00010997      -118.2515649547 -1.94E-05
    32 OT DIIS     0.80E-01    3.2     0.00009006      -118.2515790498 -1.41E-05
    33 OT DIIS     0.80E-01    3.2     0.00007304      -118.2515879752 -8.93E-06
    34 OT DIIS     0.80E-01    3.2     0.00005973      -118.2515933985 -5.42E-06
    35 OT DIIS     0.80E-01    3.2     0.00004989      -118.2515961838 -2.79E-06
    36 OT DIIS     0.80E-01    3.2     0.00004143      -118.2515980114 -1.83E-06
    37 OT DIIS     0.80E-01    3.2     0.00003501      -118.2515991627 -1.15E-06
    38 OT DIIS     0.80E-01    3.2     0.00003053      -118.2515998622 -6.99E-07
    39 OT DIIS     0.80E-01    3.2     0.00002698      -118.2516003501 -4.88E-07
    40 OT DIIS     0.80E-01    3.2     0.00002412      -118.2516007278 -3.78E-07
    41 OT DIIS     0.80E-01    3.2     0.00002204      -118.2516009772 -2.49E-07
    42 OT DIIS     0.80E-01    3.2     0.00002017      -118.2516012406 -2.63E-07
    43 OT DIIS     0.80E-01    3.2     0.00001871      -118.2516014677 -2.27E-07
    44 OT DIIS     0.80E-01    3.2     0.00001728      -118.2516016701 -2.02E-07
    45 OT DIIS     0.80E-01    3.2     0.00001586      -118.2516018837 -2.14E-07
    46 OT DIIS     0.80E-01    3.2     0.00001449      -118.2516020913 -2.08E-07
    47 OT DIIS     0.80E-01    3.2     0.00001322      -118.2516022675 -1.76E-07
    48 OT DIIS     0.80E-01    3.2     0.00001193      -118.2516024360 -1.69E-07
    49 OT DIIS     0.80E-01    3.2     0.00001068      -118.2516025716 -1.36E-07
    50 OT DIIS     0.80E-01    3.2     0.00000933      -118.2516026955 -1.24E-07

  *** SCF run converged in    50 steps ***


  Electronic density on regular grids:        -47.9999998061        0.0000001939
  Core density on regular grids:               47.9999999987       -0.0000000013
  Total charge density on r-space grids:        0.0000001927
  Total charge density g-space grids:           0.0000001927

  Overlap energy of the core charge distribution:               0.00000013217887
  Self energy of the core charge distribution:               -301.67942807122279
  Core Hamiltonian energy:                                     85.89072308802810
  Hartree energy:                                             125.35411776354471
  Exchange-correlation energy:                                -20.36523697676691
  Hartree-Fock Exchange energy:                                -6.04683879625239
  QM/MM Electrostatic energy:                                  -1.40493983497391

  Total energy:                                              -118.25160269546434

 ENERGY| Total FORCE_EVAL ( QMMM ) energy [a.u.]:           -136.905472697818425

 MD_INI| MD initialization
 MD_INI| Potential energy [hartree]                          -0.136905472698E+03
 MD_INI| Total kinetic energy [hartree]                       0.654533229227E+01
 MD_INI| QM kinetic energy [hartree]                          0.173943669988E-01
 MD_INI| Total temperature [K]                                        300.000000
 MD_INI| QM temperature [K]                                           366.180008
 MD_INI| Pressure [bar]                                       1.373018828856E+04
 MD_INI| Cell volume [bohr^3]                                 4.336220625571E+05
 MD_INI| Cell volume [ang^3]                                  6.425615938541E+04
 MD_INI| Cell lengths [bohr]      7.66102391E+01  7.55113899E+01  7.49569814E+01
 MD_INI| Cell lengths [ang]       4.05403925E+01  3.99589065E+01  3.96655262E+01
 MD_INI| Cell angles [deg]        9.00000000E+01  9.00000000E+01  9.00000000E+01

  Translating the system in order to center the QM fragment in the QM box.

 Number of electrons:                                                         48
 Number of occupied orbitals:                                                 24
 Number of molecular orbitals:                                                24

 Number of orbital functions:                                                114
 Number of independent orbital functions:                                    114

 Extrapolation method: ASPC


 SCF WAVEFUNCTION OPTIMIZATION

  ----------------------------------- OT ---------------------------------------
  Minimizer      : DIIS                : direct inversion
                                         in the iterative subspace
                                         using   7 DIIS vectors
                                         safer DIIS on
  Preconditioner : FULL_SINGLE_INVERSE : inversion of 
                                         H + eS - 2*(Sc)(c^T*H*c+const)(Sc)^T
  Precond_solver : DEFAULT
  stepsize       :    0.08000000                  energy_gap     :    0.08000000
  eps_taylor     :   0.10000E-15                  max_taylor     :             4
  ----------------------------------- OT ---------------------------------------

  Step     Update method      Time    Convergence         Total energy    Change
  ------------------------------------------------------------------------------
     1 OT DIIS     0.80E-01    3.7     0.00126811      -118.2671862014 -1.18E+02
     2 OT DIIS     0.80E-01    3.2     0.00076142      -118.2674604204 -2.74E-04
     3 OT DIIS     0.80E-01    3.2     0.00032059      -118.2676185359 -1.58E-04
     4 OT DIIS     0.80E-01    3.2     0.00012169      -118.2676506413 -3.21E-05
     5 OT DIIS     0.80E-01    3.2     0.00006034      -118.2676544707 -3.83E-06
     6 OT DIIS     0.80E-01    3.2     0.00002348      -118.2676555559 -1.09E-06
     7 OT DIIS     0.80E-01    3.2     0.00001167      -118.2676557060 -1.50E-07
     8 OT DIIS     0.80E-01    3.2     0.00000515      -118.2676557509 -4.49E-08

  *** SCF run converged in     8 steps ***


  Electronic density on regular grids:        -47.9999998049        0.0000001951
  Core density on regular grids:               47.9999999987       -0.0000000013
  Total charge density on r-space grids:        0.0000001939
  Total charge density g-space grids:           0.0000001939

  Overlap energy of the core charge distribution:               0.00000010455794
  Self energy of the core charge distribution:               -301.67942807122279
  Core Hamiltonian energy:                                     85.79786358195773
  Hartree energy:                                             125.42239461270066
  Exchange-correlation energy:                                -20.34636039364445
  Hartree-Fock Exchange energy:                                -6.03960641819669
  QM/MM Electrostatic energy:                                  -1.42251916705332

  Total energy:                                              -118.26765575090091

 ENERGY| Total FORCE_EVAL ( QMMM ) energy [a.u.]:           -135.810374045537571

 MD| ***************************************************************************
 MD| Step number                                                               1
 MD| Time [fs]                                                          1.000000
 MD| Conserved quantity [hartree]                            -0.130069776626E+03
 MD| ---------------------------------------------------------------------------
 MD|                                          Instantaneous             Averages
 MD| CPU time per MD step [s]                    340.511154           340.511154
 MD| Energy drift per atom [K]           0.199258859648E+02   0.000000000000E+00
 MD| Potential energy [hartree]         -0.135810374046E+03  -0.135810374046E+03
 MD| Total kinetic energy [hartree]      0.573909355676E+01   0.573909355676E+01
 MD| QM kinetic energy [hartree]         0.159489175516E-01   0.159489175516E-01
 MD| Total temperature [K]                       263.046701           263.046701
 MD| QM temperature [K]                          335.750922           335.750922
 MD| Pressure [bar]                      6.002965231874E+03   6.002965231874E+03
 MD| ***************************************************************************

  Translating the system in order to center the QM fragment in the QM box.

 Number of electrons:                                                         48
 Number of occupied orbitals:                                                 24
 Number of molecular orbitals:                                                24

 Number of orbital functions:                                                114
 Number of independent orbital functions:                                    114

 Extrapolation method: ASPC


 SCF WAVEFUNCTION OPTIMIZATION

  ----------------------------------- OT ---------------------------------------
  Minimizer      : DIIS                : direct inversion
                                         in the iterative subspace
                                         using   7 DIIS vectors
                                         safer DIIS on
  Preconditioner : FULL_SINGLE_INVERSE : inversion of 
                                         H + eS - 2*(Sc)(c^T*H*c+const)(Sc)^T
  Precond_solver : DEFAULT
  stepsize       :    0.08000000                  energy_gap     :    0.08000000
  eps_taylor     :   0.10000E-15                  max_taylor     :             4
  ----------------------------------- OT ---------------------------------------

  Step     Update method      Time    Convergence         Total energy    Change
  ------------------------------------------------------------------------------
     1 OT DIIS     0.80E-01    3.6     0.00055483      -118.2910525250 -1.18E+02
     2 OT DIIS     0.80E-01    3.1     0.00031662      -118.2911039542 -5.14E-05
     3 OT DIIS     0.80E-01    3.2     0.00013094      -118.2911302711 -2.63E-05
     4 OT DIIS     0.80E-01    3.2     0.00004280      -118.2911357593 -5.49E-06
     5 OT DIIS     0.80E-01    3.2     0.00002358      -118.2911361994 -4.40E-07
     6 OT DIIS     0.80E-01    3.1     0.00000674      -118.2911363772 -1.78E-07

  *** SCF run converged in     6 steps ***


  Electronic density on regular grids:        -47.9999997819        0.0000002181
  Core density on regular grids:               47.9999999988       -0.0000000012
  Total charge density on r-space grids:        0.0000002169
  Total charge density g-space grids:           0.0000002169

  Overlap energy of the core charge distribution:               0.00000009549439
  Self energy of the core charge distribution:               -301.67942807122279
  Core Hamiltonian energy:                                     85.74935823296528
  Hartree energy:                                             125.45879098389440
  Exchange-correlation energy:                                -20.33660714955371
  Hartree-Fock Exchange energy:                                -6.03577414037640
  QM/MM Electrostatic energy:                                  -1.44747632841449

  Total energy:                                              -118.29113637721333

 ENERGY| Total FORCE_EVAL ( QMMM ) energy [a.u.]:           -135.816542786673722

 MD| ***************************************************************************
 MD| Step number                                                               2
 MD| Time [fs]                                                          2.000000
 MD| Conserved quantity [hartree]                            -0.130133162721E+03
 MD| ---------------------------------------------------------------------------
 MD|                                          Instantaneous             Averages
 MD| CPU time per MD step [s]                     93.621338           217.066246
 MD| Energy drift per atom [K]           0.155689591859E+02   0.778447959295E+01
 MD| Potential energy [hartree]         -0.135816542787E+03  -0.135813458416E+03
 MD| Total kinetic energy [hartree]      0.568104502113E+01   0.571006928895E+01
 MD| QM kinetic energy [hartree]         0.145935682172E-01   0.152712428844E-01
 MD| Total temperature [K]                       260.386094           261.716397
 MD| QM temperature [K]                          307.218591           321.484756
 MD| Pressure [bar]                     -6.381292500983E+03  -1.891636345546E+02
 MD| ***************************************************************************

  Translating the system in order to center the QM fragment in the QM box.

 Number of electrons:                                                         48
 Number of occupied orbitals:                                                 24
 Number of molecular orbitals:                                                24

 Number of orbital functions:                                                114
 Number of independent orbital functions:                                    114

 Extrapolation method: ASPC


 SCF WAVEFUNCTION OPTIMIZATION

  ----------------------------------- OT ---------------------------------------
  Minimizer      : DIIS                : direct inversion
                                         in the iterative subspace
                                         using   7 DIIS vectors
                                         safer DIIS on
  Preconditioner : FULL_SINGLE_INVERSE : inversion of 
                                         H + eS - 2*(Sc)(c^T*H*c+const)(Sc)^T
  Precond_solver : DEFAULT
  stepsize       :    0.08000000                  energy_gap     :    0.08000000
  eps_taylor     :   0.10000E-15                  max_taylor     :             4
  ----------------------------------- OT ---------------------------------------

  Step     Update method      Time    Convergence         Total energy    Change
  ------------------------------------------------------------------------------
     1 OT DIIS     0.80E-01    3.7     0.00038766      -118.3225296351 -1.18E+02
     2 OT DIIS     0.80E-01    3.2     0.00022039      -118.3225547008 -2.51E-05
     3 OT DIIS     0.80E-01    3.2     0.00009133      -118.3225674044 -1.27E-05
     4 OT DIIS     0.80E-01    3.2     0.00003042      -118.3225700673 -2.66E-06
     5 OT DIIS     0.80E-01    3.2     0.00001736      -118.3225702806 -2.13E-07
     6 OT DIIS     0.80E-01    3.2     0.00000474      -118.3225703785 -9.79E-08

  *** SCF run converged in     6 steps ***


  Electronic density on regular grids:        -47.9999997457        0.0000002543
  Core density on regular grids:               47.9999999987       -0.0000000013
  Total charge density on r-space grids:        0.0000002530
  Total charge density g-space grids:           0.0000002530

  Overlap energy of the core charge distribution:               0.00000009886945
  Self energy of the core charge distribution:               -301.67942807122279
  Core Hamiltonian energy:                                     85.75162869605586
  Hartree energy:                                             125.45792107133452
  Exchange-correlation energy:                                -20.33752073875611
  Hartree-Fock Exchange energy:                                -6.03596625566824
  QM/MM Electrostatic energy:                                  -1.47920517910945

  Total energy:                                              -118.32257037849675

 ENERGY| Total FORCE_EVAL ( QMMM ) energy [a.u.]:           -136.396260252041372

 MD| ***************************************************************************
 MD| Step number                                                               3
 MD| Time [fs]                                                          3.000000
 MD| Conserved quantity [hartree]                            -0.130254811854E+03
 MD| ---------------------------------------------------------------------------
 MD|                                          Instantaneous             Averages
 MD| CPU time per MD step [s]                     93.626603           175.919698
 MD| Energy drift per atom [K]           0.720724560173E+01   0.759206826254E+01
 MD| Potential energy [hartree]         -0.136396260252E+03  -0.136007725695E+03
 MD| Total kinetic energy [hartree]      0.613839878414E+01   0.585284578735E+01
 MD| QM kinetic energy [hartree]         0.143958407657E-01   0.149794421782E-01
 MD| Total temperature [K]                       281.348533           268.260442
 MD| QM temperature [K]                          303.056103           315.341872
 MD| Pressure [bar]                     -9.925144784124E+03  -3.434490684411E+03
 MD| ***************************************************************************

 -------------------------------------------------------------------------------
 -                                                                             -
 -                                DBCSR STATISTICS                             -
 -                                                                             -
 -------------------------------------------------------------------------------
 COUNTER                                    TOTAL       BLAS       SMM       ACC
 flops     5 x    24 x    24                46080       0.0%    100.0%      0.0%
 flops     5 x     5 x    24               295200       0.0%    100.0%      0.0%
 flops     5 x    24 x     5               792000       0.0%    100.0%      0.0%
 flops     5 x    13 x    24              2046720       0.0%    100.0%      0.0%
 flops    13 x     5 x    24              2046720       0.0%    100.0%      0.0%
 flops    18 x    24 x    18              4603392       0.0%    100.0%      0.0%
 flops    13 x    24 x     5              8236800       0.0%    100.0%      0.0%
 flops     5 x    24 x    13              8236800       0.0%    100.0%      0.0%
 flops    13 x    24 x    18              9974016       0.0%    100.0%      0.0%
 flops    18 x    24 x    13              9974016       0.0%    100.0%      0.0%
 flops    24 x    24 x    18             11612160       0.0%    100.0%      0.0%
 flops    18 x    24 x    24             14349312       0.0%    100.0%      0.0%
 flops    24 x    24 x    24             15261696       0.0%    100.0%      0.0%
 flops    13 x    13 x    24             23946624       0.0%    100.0%      0.0%
 flops    24 x    24 x    13             25159680       0.0%    100.0%      0.0%
 flops    13 x    24 x    24             31569408       0.0%    100.0%      0.0%
 flops    13 x    24 x    13            107273088       0.0%    100.0%      0.0%
 flops inhomo. stacks                           0       0.0%      0.0%      0.0%
 flops total                       275.423712E+06       0.0%    100.0%      0.0%
 flops max/rank                     74.941824E+06       0.0%    100.0%      0.0%
 matmuls inhomo. stacks                         0       0.0%      0.0%      0.0%
 matmuls total                              31346       0.0%    100.0%      0.0%
 number of processed stacks                 31346       0.0%    100.0%      0.0%
 average stack size                                     0.0       1.0       0.0
 marketing flops                   298.766016E+06
 -------------------------------------------------------------------------------
 # multiplications                           1507
 max memory usage/rank               2.293146E+09
 # max total images/rank                        1
 # max 3D layers                                1
 # MPI messages exchanged                 1350272
 MPI messages size (bytes):
  total size                       422.011296E+06
  min size                           0.000000E+00
  max size                           4.608000E+03
  average size                     312.537994E+00
 MPI breakdown and total messages size (bytes):
             size <=      128             1159494                        0
       128 < size <=     8192              190778                422011296
      8192 < size <=    32768                   0                        0
     32768 < size <=   131072                   0                        0
    131072 < size <=  4194304                   0                        0
   4194304 < size <= 16777216                   0                        0
  16777216 < size                               0                        0
 -------------------------------------------------------------------------------
 -                                                                             -
 -                      DBCSR MESSAGE PASSING PERFORMANCE                      -
 -                                                                             -
 -------------------------------------------------------------------------------
 ROUTINE             CALLS      AVE VOLUME [Bytes]
 MP_Bcast               18                     12.
 MP_Allreduce         8159                      8.
 MP_Alltoall          5335                   5696.
 MP_ISend            48208                    580.
 MP_IRecv            48208                    432.
 -------------------------------------------------------------------------------

 -------------------------------------------------------------------------------
 -                                                                             -
 -                                GRID STATISTICS                              -
 -                                                                             -
 -------------------------------------------------------------------------------
 LP    KERNEL             BACKEND                              COUNT     PERCENT
 4     collocate ortho    REF                                  54714      32.66%
 4     integrate ortho    REF                                  52895      31.58%
 3     collocate ortho    REF                                  21009      12.54%
 3     integrate ortho    REF                                  20170      12.04%
 2     collocate ortho    REF                                   5476       3.27%
 2     integrate ortho    REF                                   5180       3.09%
 5     integrate ortho    REF                                   2954       1.76%
 0     collocate general  REF                                   2560       1.53%
 1     integrate general  REF                                   2560       1.53%
 -------------------------------------------------------------------------------

 MEMORY| Estimated peak process memory [MiB]                                2188

 -------------------------------------------------------------------------------
 -                                                                             -
 -                         MESSAGE PASSING PERFORMANCE                         -
 -                                                                             -
 -------------------------------------------------------------------------------

 ROUTINE             CALLS      AVE VOLUME [Bytes]
 MP_Group                5
 MP_Bcast             5036                 459769.
 MP_Allreduce         9305                 599186.
 MP_Sync               467
 MP_Alltoall          1490               46406982.
 MP_ISendRecv        29232                  67698.
 MP_Wait             37556
 MP_comm_split          50
 MP_ISend             7044                 902823.
 MP_IRecv             7040                 902503.
 MP_Recv                42                   2736.
 -------------------------------------------------------------------------------


 -------------------------------------------------------------------------------
 -                                                                             -
 -                           R E F E R E N C E S                               -
 -                                                                             -
 -------------------------------------------------------------------------------
 
 CP2K version 8.1, the CP2K developers group (2020).
 CP2K is freely available from https://www.cp2k.org/ .

 Kuehne,Thomas D.; Iannuzzi,Marcella; Del Ben,Mauro;
 Rybkin,Vladimir V.; Seewald,Patrick; Stein,Frederick; Laino,Teodoro;
 Khaliullin,Rustam Z.; Schuett,Ole; Schiffmann,Florian; Golze,Dorothea;
 Wilhelm,Jan; Chulkov,Sergey; Bani-Hashemian,Mohammad Hossein;
 Weber,Valery; Borstnik,Urban; Taillefumier,Mathieu;
 Jakobovits,Alice Shoshana; Lazzaro,Alfio; Pabst,Hans; Mueller,Tiziano;
 Schade,Robert; Guidon,Manuel; Andermatt,Samuel; Holmberg,Nico;
 Schenter,Gregory K.; Hehn,Anna; Bussy,Augustin; Belleflamme,Fabian;
 Tabacchi,Gloria; Gloess,Andreas; Lass,Michael; Bethune,Iain;
 Mundy,Christopher J.; Plessl,Christian; Watkins,Matt;
 VandeVondele,Joost; Krack,Matthias; Hutter,Juerg. 
 The Journal of Chemical Physics, 152 (19), (2020). 
 CP2K: An electronic structure and molecular dynamics software package -
 Quickstep: Efficient and accurate electronic structure calculations.
 https://doi.org/10.1063/5.0007045

 Schuett, Ole; Messmer, Peter; Hutter, Juerg; VandeVondele, Joost. 
 Electronic Structure Calculations on Graphics Processing Units, John
 Wiley & Sons, Ltd, 173-190 (2016). 
 GPU-Accelerated Sparse Matrix-Matrix Multiplication for
 Linear Scaling Density Functional Theory.
 https://doi.org/10.1002/9781118670712.ch8

 Borstnik, U; VandeVondele, J; Weber, V; Hutter, J. 
 PARALLEL COMPUTING, 40 (5-6), 47-58 (2014). 
 Sparse matrix multiplication: The distributed block-compressed sparse
 row library.
 https://doi.org/10.1016/j.parco.2014.03.012

 Hutter, J; Iannuzzi, M; Schiffmann, F; VandeVondele, J. 
 WIREs Comput Mol Sci., 4 (1), 15-25 (2014). 
 CP2K: atomistic simulations of condensed matter systems.
 https://doi.org/10.1002/wcms.1159

 Guidon, M; Hutter, J; VandeVondele, J. 
 JOURNAL OF CHEMICAL THEORY AND COMPUTATION, 5 (11), 3010-3021 (2009). 
 Robust Periodic Hartree-Fock Exchange for Large-Scale Simulations Using
 Gaussian Basis Sets.
 https://doi.org/10.1021/ct900494g

 Guidon, M; Schiffmann, F; Hutter, J; VandeVondele, J. 
 JOURNAL OF CHEMICAL PHYSICS, 128 (21), 214104 (2008). 
 Ab initio molecular dynamics using hybrid density functionals.
 https://doi.org/10.1063/1.2931945

 VandeVondele, J; Hutter, J. 
 JOURNAL OF CHEMICAL PHYSICS, 127 (11), 114105 (2007). 
 Gaussian basis sets for accurate calculations on molecular systems in
 gas and condensed phases.
 https://doi.org/10.1063/1.2770708

 Kuhne, TD; Krack, M; Mohamed, FR; Parrinello, M. 
 PHYSICAL REVIEW LETTERS, 98 (6), 066401 (2007). 
 Efficient and accurate Car-Parrinello-like approach to
 Born-Oppenheimer molecular dynamics.
 https://doi.org/10.1103/PhysRevLett.98.066401

 Laino, T; Mohamed, F; Laio, A; Parrinello, M. 
 JOURNAL OF CHEMICAL THEORY AND COMPUTATION, 1 (6), 1176-1184 (2005). 
 An efficient real space multigrid QM/MM electrostatic coupling.
 https://doi.org/10.1021/ct050123f

 Krack, M. 
 THEORETICAL CHEMISTRY ACCOUNTS, 114 (1-3), 145-152 (2005). 
 Pseudopotentials for H to Kr optimized for gradient-corrected
 exchange-correlation functionals.
 https://doi.org/10.1007/s00214-005-0655-y

 VandeVondele, J; Krack, M; Mohamed, F; Parrinello, M; Chassaing, T;
 Hutter, J. COMPUTER PHYSICS COMMUNICATIONS, 167 (2), 103-128 (2005). 
 QUICKSTEP: Fast and accurate density functional calculations using a
 mixed Gaussian and plane waves approach.
 https://doi.org/10.1016/j.cpc.2004.12.014

 Frigo, M; Johnson, SG. 
 PROCEEDINGS OF THE IEEE, 93 (2), 216-231 (2005). 
 The design and implementation of FFTW3.
 https://doi.org/10.1109/JPROC.2004.840301

 Kolafa, J. 
 JOURNAL OF COMPUTATIONAL CHEMISTRY, 25 (3), 335-342 (2004). 
 Time-reversible always stable predictor-corrector method for molecular dynamics of polarizable molecules.
 https://doi.org/10.1002/jcc.10385

 VandeVondele, J; Hutter, J. 
 JOURNAL OF CHEMICAL PHYSICS, 118 (10), 4365-4369 (2003). 
 An efficient orbital transformation method for electronic structure
 calculations.
 https://doi.org/10.1063/1.1543154

 Hartwigsen, C; Goedecker, S; Hutter, J. 
 PHYSICAL REVIEW B, 58 (7), 3641-3662 (1998). 
 Relativistic separable dual-space Gaussian pseudopotentials from H to Rn.
 https://doi.org/10.1103/PhysRevB.58.3641

 Lippert, G; Hutter, J; Parrinello, M. 
 MOLECULAR PHYSICS, 92 (3), 477-487 (1997). 
 A hybrid Gaussian and plane wave density functional scheme.
 https://doi.org/10.1080/002689797170220

 Perdew, JP; Burke, K; Ernzerhof, M. 
 PHYSICAL REVIEW LETTERS, 77 (18), 3865-3868 (1996). 
 Generalized gradient approximation made simple.
 https://doi.org/10.1103/PhysRevLett.77.3865

 Goedecker, S; Teter, M; Hutter, J. 
 PHYSICAL REVIEW B, 54 (3), 1703-1710 (1996). 
 Separable dual-space Gaussian pseudopotentials.
 https://doi.org/10.1103/PhysRevB.54.1703

 ESSMANN, U; PERERA, L; BERKOWITZ, ML; DARDEN, T; LEE, H; PEDERSEN, LG. 
 JOURNAL OF CHEMICAL PHYSICS, 103 (19), 8577-8593 (1995). 
 A SMOOTH PARTICLE MESH EWALD METHOD.
 https://doi.org/10.1063/1.470117

 NOSE, S. JOURNAL OF CHEMICAL PHYSICS, 81 (1), 511-519 (1984). 
 A UNIFIED FORMULATION OF THE CONSTANT TEMPERATURE MOLECULAR-DYNAMICS
 METHODS.
 https://doi.org/10.1063/1.447334

 NOSE, S. MOLECULAR PHYSICS, 52 (2), 255-268 (1984). 
 A MOLECULAR-DYNAMICS METHOD FOR SIMULATIONS IN THE CANONICAL ENSEMBLE.
 https://doi.org/10.1080/00268978400101201


 -------------------------------------------------------------------------------
 -                                                                             -
 -                                T I M I N G                                  -
 -                                                                             -
 -------------------------------------------------------------------------------
 SUBROUTINE                       CALLS  ASD         SELF TIME        TOTAL TIME
                                MAXIMUM       AVERAGE  MAXIMUM  AVERAGE  MAXIMUM
 CP2K                                 1  1.0    0.107    0.122  529.153  529.155
 qs_mol_dyn_low                       1  2.0    0.015    0.016  527.819  527.854
 qs_forces                            4  3.8    0.001    0.004  310.811  310.814
 velocity_verlet                      3  3.0    0.005    0.007  287.436  287.438
 rebuild_ks_matrix                   74  8.1    0.000    0.000  253.413  253.422
 qs_ks_build_kohn_sham_matrix        74  9.1    0.018    0.026  253.413  253.422
 qs_energies                          4  4.8    0.025    0.026  234.862  234.862
 scf_env_do_scf                       4  5.8    0.000    0.002  229.573  229.573
 scf_env_do_scf_inner_loop           70  6.3    0.020    0.036  212.808  212.810
 qs_ks_update_qs_env                 74  7.3    0.001    0.001  177.483  177.492
 pw_transfer                       1450 11.7    0.271    0.334  157.786  161.976
 fft_wrap_pw1pw2                   1282 12.8    0.028    0.036  155.109  159.276
 fft_wrap_pw1pw2_150                822 14.0   17.073   19.058  151.008  154.414
 qs_vxc_create                       74 10.1    0.003    0.005  120.034  120.080
 xc_vxc_pw_create                    74 11.1    2.462    3.117  120.031  120.076
 qmmm_forces                          4  3.8    0.001    0.003  117.781  117.782
 qmmm_forces_with_gaussian            4  4.8    0.088    0.098  115.457  116.497
 fft3d_ps                          1282 14.8   63.372   66.540  107.554  110.807
 pw_restrict_s3                      12  5.8   31.639   32.981  101.177  102.309
 qmmm_el_coupling                     4  3.8    0.000    0.000   97.206   98.164
 qmmm_elec_with_gaussian              4  4.8    0.062    0.104   97.185   98.142
 pw_integral_ab                    2336  7.5   82.084   83.640   83.270   86.197
 qmmm_elec_with_gaussian:spline       4  5.8    0.000    0.000   81.168   82.139
 pw_prolongate_s3                    12  6.8   25.699   27.005   81.168   82.139
 qs_ks_update_qs_env_forces           4  4.8    0.000    0.000   75.935   75.935
 hfx_ks_matrix                       74 10.1    0.004    0.009   72.446   72.477
 derivatives_four_center              4  8.8    0.027    0.207   65.565   65.569
 derivatives_four_center_main         4  9.8    0.001    0.001   65.338   65.343
 derivatives_four_center_bin        416 10.8   60.894   63.407   60.894   63.407
 xc_rho_set_and_dset_create          74 12.1    1.005    1.153   53.163   56.295
 qs_rho_update_rho                   74  7.4    0.001    0.001   52.625   52.632
 calculate_rho_elec                  74  8.4    0.361    0.395   52.624   52.631
 density_rs2pw                       74  9.4    0.007    0.008   44.493   45.720
 sum_up_and_integrate                74 10.1    1.412    1.511   33.604   33.631
 integrate_v_rspace                  74 11.1    0.004    0.005   32.192   32.368
 potential_pw2rs                     74 12.1    0.019    0.021   31.510   31.689
 rs_pw_transfer                     616 11.6    0.012    0.018   29.324   29.917
 mp_alltoall_z22v                  1282 16.8   21.797   28.477   21.797   28.477
 x_to_yz                            682 16.2   13.350   14.330   24.354   25.901
 mp_sum_dm3                          20  5.8   25.243   25.347   25.243   25.347
 pw_axpy                           1708  8.5   23.368   24.574   23.368   24.574
 yz_to_x                            600 15.3    8.850   10.001   19.643   23.647
 pw_zero                           1922  7.3   20.498   21.752   20.498   21.752
 pw_scatter_p                       682 15.2   16.207   17.849   16.207   17.849
 init_scf_loop                        4  6.8    0.000    0.001   16.758   16.759
 pw_gather_p                        600 14.3   13.940   15.214   13.940   15.214
 pw_derive                          456 12.5   12.329   13.159   12.329   13.159
 rs_pw_transfer_PW2RS_150            78 13.9    6.744    7.016   10.587   10.863
 -------------------------------------------------------------------------------

 The number of warnings for this run is : 1
 
 -------------------------------------------------------------------------------
  **** **** ******  **  PROGRAM ENDED AT                 2021-11-17 09:56:33.329
 ***** ** ***  *** **   PROGRAM RAN ON                          ja0802.para.bscc
 **    ****   ******    PROGRAM RAN BY                                   scb3056
 ***** **    ** ** **   PROGRAM PROCESS ID                                116292
  **** **  *******  **  PROGRAM STOPPED IN /public1/home/scb3056/fangyg/test/for
                                           um
-------------- next part --------------
 DBCSR| CPU Multiplication driver                                           XSMM
 DBCSR| Multrec recursion limit                                              512
 DBCSR| Multiplication stack size                                           1000
 DBCSR| Maximum elements for images                                    UNLIMITED
 DBCSR| Multiplicative factor virtual images                                   1
 DBCSR| Use multiplication densification                                       T
 DBCSR| Multiplication size stacks                                             3
 DBCSR| Use memory pool for CPU allocation                                     F
 DBCSR| Number of 3D layers                                               SINGLE
 DBCSR| Use MPI memory allocation                                              F
 DBCSR| Use RMA algorithm                                                      F
 DBCSR| Use Communication thread                                               T
 DBCSR| Communication thread load                                             87
 DBCSR| MPI: My node id                                                        0
 DBCSR| MPI: Number of nodes                                                  64
 DBCSR| OMP: Current number of threads                                         1
 DBCSR| OMP: Max number of threads                                             1
 DBCSR| Split modifier for TAS multiplication algorithm                  1.0E+00


  **** **** ******  **  PROGRAM STARTED AT               2021-11-17 09:50:09.749
 ***** ** ***  *** **   PROGRAM STARTED ON                      ga2008.para.bscc
 **    ****   ******    PROGRAM STARTED BY                               scb3056
 ***** **    ** ** **   PROGRAM PROCESS ID                                129715
  **** **  *******  **  PROGRAM STARTED IN /public1/home/scb3056/fangyg/test/for
                                           um/vacuo

 CP2K| version string:                                          CP2K version 8.1
 CP2K| source code revision number:                                  git:0b61f2f
 CP2K| cp2kflags: omp libint fftw3 libxc parallel mpi3 scalapack xsmm max_contr=
 CP2K|            4 mkl
 CP2K| is freely available from                            https://www.cp2k.org/
 CP2K| Program compiled at                          Mon Aug 16 10:31:22 CST 2021
 CP2K| Program compiled on                                       ln131.para.bscc
 CP2K| Program compiled for                           Linux-x86-64-intel-minimal
 CP2K| Data directory path                    /public1/soft/cp2k/cp2k-8.1.0/data
 CP2K| Input file name                                                 vacuo.inp
 
 GLOBAL| Force Environment number                                              1
 GLOBAL| Basis set file name                                        BASIS_MOLOPT
 GLOBAL| Potential file name                                           POTENTIAL
 GLOBAL| MM Potential file name                                     MM_POTENTIAL
 GLOBAL| Coordinate file name                                          vacuo.pdb
 GLOBAL| Method name                                                        CP2K
 GLOBAL| Project name                                                         md
 GLOBAL| Preferred FFT library                                             FFTW3
 GLOBAL| Preferred diagonalization lib.                                       SL
 GLOBAL| Run type                                                             MD
 GLOBAL| All-to-all communication in single precision                          F
 GLOBAL| FFTs using library dependent lengths                                  F
 GLOBAL| Global print level                                                  LOW
 GLOBAL| MPI I/O enabled                                                       T
 GLOBAL| Total number of message passing processes                            64
 GLOBAL| Number of threads for this process                                    1
 GLOBAL| This output is from process                                           0
 GLOBAL| CPU model name                          AMD EPYC 7452 32-Core Processor
 GLOBAL| CPUID                                                              1002

 MEMORY| system memory details [Kb]
 MEMORY|                        rank 0           min           max       average
 MEMORY| MemTotal            263793368     263793368     263793368     263793368
 MEMORY| MemFree             239345284     239345284     239345284     239345284
 MEMORY| Buffers                     0             0             0             0
 MEMORY| Cached                9224172       9224172       9224172       9224172
 MEMORY| Slab                  1737256       1737256       1737256       1737256
 MEMORY| SReclaimable           326520        326520        326520        326520
 MEMORY| MemLikelyFree       248895976     248895976     248895976     248895976

          ----------------------------------------------------------------------
 COLVARS| COLVAR INPUT INDEX:        1
 COLVARS| BOND          >>> ATOMS:                                     5       8
          ----------------------------------------------------------------------
 
 GENERATE|  Preliminary Number of Bonds generated:                             8

 GENERATE| WARNING in connectivity generation!
 GENERATE| Two molecules/residues named (MOL1) have different  number of atoms.
 GENERATE| Molecule starting at position (8) has Nr. <2> of atoms.
 GENERATE| while the other same molecules have Nr. <6> of atoms!
 GENERATE| Increasing bondparm_factor by 1.05.. An error was found in the generated
 GENERATE| connectivity. Retry...
 GENERATE| Present value of BONDPARM_FACTOR (   1.155000 ).

 
 GENERATE|  Preliminary Number of Bonds generated:                             8

 GENERATE| WARNING in connectivity generation!
 GENERATE| Two molecules/residues named (MOL1) have different  number of atoms.
 GENERATE| Molecule starting at position (8) has Nr. <2> of atoms.
 GENERATE| while the other same molecules have Nr. <6> of atoms!
 GENERATE| Increasing bondparm_factor by 1.05.. An error was found in the generated
 GENERATE| connectivity. Retry...
 GENERATE| Present value of BONDPARM_FACTOR (   1.212750 ).

 
 GENERATE|  Preliminary Number of Bonds generated:                             8

 GENERATE| WARNING in connectivity generation!
 GENERATE| Two molecules/residues named (MOL1) have different  number of atoms.
 GENERATE| Molecule starting at position (8) has Nr. <2> of atoms.
 GENERATE| while the other same molecules have Nr. <6> of atoms!
 GENERATE| Increasing bondparm_factor by 1.05.. An error was found in the generated
 GENERATE| connectivity. Retry...
 GENERATE| Present value of BONDPARM_FACTOR (   1.273388 ).

 
 GENERATE|  Preliminary Number of Bonds generated:                             8

 GENERATE| WARNING in connectivity generation!
 GENERATE| Two molecules/residues named (MOL1) have different  number of atoms.
 GENERATE| Molecule starting at position (8) has Nr. <2> of atoms.
 GENERATE| while the other same molecules have Nr. <6> of atoms!
 GENERATE| Increasing bondparm_factor by 1.05.. An error was found in the generated
 GENERATE| connectivity. Retry...
 GENERATE| Present value of BONDPARM_FACTOR (   1.337057 ).

 
 GENERATE|  Preliminary Number of Bonds generated:                             8

 GENERATE| WARNING in connectivity generation!
 GENERATE| Two molecules/residues named (MOL1) have different  number of atoms.
 GENERATE| Molecule starting at position (8) has Nr. <2> of atoms.
 GENERATE| while the other same molecules have Nr. <6> of atoms!
 GENERATE| Increasing bondparm_factor by 1.05.. An error was found in the generated
 GENERATE| connectivity. Retry...
 GENERATE| Present value of BONDPARM_FACTOR (   1.403910 ).

 
 GENERATE|  Preliminary Number of Bonds generated:                             8

 GENERATE| WARNING in connectivity generation!
 GENERATE| Two molecules/residues named (MOL1) have different  number of atoms.
 GENERATE| Molecule starting at position (8) has Nr. <2> of atoms.
 GENERATE| while the other same molecules have Nr. <6> of atoms!
 GENERATE| Increasing bondparm_factor by 1.05.. An error was found in the generated
 GENERATE| connectivity. Retry...
 GENERATE| Present value of BONDPARM_FACTOR (   1.474105 ).

 
 GENERATE|  Preliminary Number of Bonds generated:                             8

 GENERATE| WARNING in connectivity generation!
 GENERATE| Two molecules/residues named (MOL1) have different  number of atoms.
 GENERATE| Molecule starting at position (8) has Nr. <2> of atoms.
 GENERATE| while the other same molecules have Nr. <6> of atoms!
 GENERATE| Increasing bondparm_factor by 1.05.. An error was found in the generated
 GENERATE| connectivity. Retry...
 GENERATE| Present value of BONDPARM_FACTOR (   1.547810 ).

 
 GENERATE|  Preliminary Number of Bonds generated:                            12

 GENERATE| WARNING in connectivity generation!
 GENERATE| Two molecules/residues named (MOL1) have different  number of atoms.
 GENERATE| Molecule starting at position (8) has Nr. <2> of atoms.
 GENERATE| while the other same molecules have Nr. <6> of atoms!
 GENERATE| Increasing bondparm_factor by 1.05.. An error was found in the generated
 GENERATE| connectivity. Retry...
 GENERATE| Present value of BONDPARM_FACTOR (   1.625201 ).

 
 GENERATE|  Preliminary Number of Bonds generated:                            14

 GENERATE| WARNING in connectivity generation!
 GENERATE| Two molecules/residues named (MOL1) have different  number of atoms.
 GENERATE| Molecule starting at position (8) has Nr. <2> of atoms.
 GENERATE| while the other same molecules have Nr. <6> of atoms!
 GENERATE| Increasing bondparm_factor by 1.05.. An error was found in the generated
 GENERATE| connectivity. Retry...
 GENERATE| Present value of BONDPARM_FACTOR (   1.706461 ).

 
 GENERATE|  Preliminary Number of Bonds generated:                            14

 GENERATE| WARNING in connectivity generation!
 GENERATE| Two molecules/residues named (MOL1) have different  number of atoms.
 GENERATE| Molecule starting at position (8) has Nr. <2> of atoms.
 GENERATE| while the other same molecules have Nr. <6> of atoms!
 GENERATE| Increasing bondparm_factor by 1.05.. An error was found in the generated
 GENERATE| connectivity. Retry...
 GENERATE| Present value of BONDPARM_FACTOR (   1.791784 ).

 
 GENERATE|  Preliminary Number of Bonds generated:                            15

 GENERATE| WARNING in connectivity generation!
 GENERATE| Two molecules/residues named (MOL1) have different  number of atoms.
 GENERATE| Molecule starting at position (8) has Nr. <2> of atoms.
 GENERATE| while the other same molecules have Nr. <6> of atoms!
 GENERATE| Increasing bondparm_factor by 1.05.. An error was found in the generated
 GENERATE| connectivity. Retry...
 GENERATE| Present value of BONDPARM_FACTOR (   1.881373 ).

 
 GENERATE|  Preliminary Number of Bonds generated:                            18
 GENERATE|  Achieved consistency in connectivity generation.
 GENERATE|  Number of Bonds generated:                                        18
 GENERATE|  Preliminary Number of Bends generated:                            60
 GENERATE|  Number of Bends generated:                                        60
 GENERATE|  Number of UB generated:                                           60
 GENERATE|  Preliminary Number of Torsions generated:                        166
 GENERATE|  Number of Torsions generated:                                    166
 GENERATE|  Number of Impropers generated:                                     3
 GENERATE|  Number of 1-4 interactions generated:                             10

 *******************************************************************************
 *******************************************************************************
 **                                                                           **
 **     #####                         ##              ##                      **
 **    ##   ##            ##          ##              ##                      **
 **   ##     ##                       ##            ######                    **
 **   ##     ##  ##   ##  ##   #####  ##  ##   ####   ##    #####    #####    **
 **   ##     ##  ##   ##  ##  ##      ## ##   ##      ##   ##   ##  ##   ##   **
 **   ##  ## ##  ##   ##  ##  ##      ####     ###    ##   ######   ######    **
 **    ##  ###   ##   ##  ##  ##      ## ##      ##   ##   ##       ##        **
 **     #######   #####   ##   #####  ##  ##  ####    ##    #####   ##        **
 **           ##                                                    ##        **
 **                                                                           **
 **                                                ... make the atoms dance   **
 **                                                                           **
 **            Copyright (C) by CP2K developers group (2000 - 2020)           **
 **                      J. Chem. Phys. 152, 194103 (2020)                    **
 **                                                                           **
 *******************************************************************************


 TOTAL NUMBERS AND MAXIMUM NUMBERS

  Total number of            - Atomic kinds:                                  10
                             - Atoms:                                         10
                             - Shell sets:                                    10
                             - Shells:                                        46
                             - Primitive Cartesian functions:                 50
                             - Cartesian basis functions:                    122
                             - Spherical basis functions:                    114

  Maximum angular momentum of- Orbital basis functions:                        2
                             - Local part of the GTH pseudopotential:          2
                             - Non-local part of the GTH pseudopotential:      0


 SCF PARAMETERS         Density guess:                                   RESTART
                        --------------------------------------------------------
                        max_scf:                                             256
                        max_scf_history:                                       0
                        max_diis:                                              4
                        --------------------------------------------------------
                        eps_scf:                                        1.00E-05
                        eps_scf_history:                                0.00E+00
                        eps_diis:                                       1.00E-01
                        eps_eigval:                                     1.00E-05
                        --------------------------------------------------------
                        level_shift [a.u.]:                                 0.00
                        --------------------------------------------------------
                        No outer SCF

 METADYN| Meta Dynamics Protocol 
 METADYN| Number of interval time steps to spawn hills                        50
 METADYN| Number of previously spawned hills                                   0
 METADYN| Spawning the Hills 
 METADYN| Height of the Spawned Gaussian                                   0.000
 METADYN| Number of collective variables                                       1
          ----------------------------------------------------------------------
 METAVARS| Collective Variable Number                                          1
 METAVARS| Scaling factor                                               0.226767
 METAVARS| Number of Walls present                                             2

 METAVARS| Wall Number:              1           Type of Wall:        REFLECTIVE
 METAVARS| Wall direction                                              WALL_PLUS
 METAVARS| Wall location                                                6.614041

 METAVARS| Wall Number:              2           Type of Wall:        REFLECTIVE
 METAVARS| Wall direction                                             WALL_MINUS
 METAVARS| Wall location                                                5.669178
          ----------------------------------------------------------------------
 
 MD_PAR| Molecular dynamics protocol (MD input parameters)
 MD_PAR| Ensemble type                                                       NVT
 MD_PAR| Number of time steps                                                  3
 MD_PAR| Time step [fs]                                                 1.000000
 MD_PAR| Temperature [K]                                              300.000000
 MD_PAR| Temperature tolerance [K]                                      0.000000
 MD_PAR| Print MD information every                                    1 step(s)
 MD_PAR| File type   Print frequency [steps]                          File names
 MD_PAR| Coordinates         10                                         traj.xyz
 MD_PAR| Velocities           1                                     md-vel-1.xyz
 MD_PAR| Energies             1                                        md-1.ener
 MD_PAR| Dump                20                                     md-1.restart

 ROT| Rotational analysis information
 ROT| Principal axes and moments of inertia [a.u.]
 ROT|                           1                   2                   3
 ROT| Eigenvalues      1.12824771224E+06   2.11271414485E+06   2.60002565658E+06
 ROT|      x              0.933516582996     -0.162493784059      0.319597495945
 ROT|      y              0.332751610941      0.724581723408     -0.603537647143
 ROT|      z             -0.133503388302      0.669758983699      0.730479122950
 ROT| Number of rotovibrational vectors                                        6

 DOF| Calculation of degrees of freedom
 DOF| Number of atoms                                                         10
 DOF| Number of intramolecular constraints                                     0
 DOF| Number of intermolecular constraints                                     0
 DOF| Invariants (translations + rotations)                                    3
 DOF| Degrees of freedom                                                      27

 DOF| Restraints information
 DOF| Number of intramolecular restraints                                      0
 DOF| Number of intermolecular restraints                                      0

 THERMOSTAT| Thermostat information for PARTICLES
 THERMOSTAT| Type of thermostat                               Nose-Hoover-Chains
 THERMOSTAT| Nose-Hoover-Chain length                                          5
 THERMOSTAT| Nose-Hoover-Chain time constant [fs]                       5.000000
 THERMOSTAT| Order of Yoshida integrator                                       3
 THERMOSTAT| Number of multiple time steps                                     2
 THERMOSTAT| Initial potential energy                         0.000000000000E+00
 THERMOSTAT| Initial kinetic energy                           0.475022301493E-03
 THERMOSTAT| End of thermostat information for PARTICLES

 MD_VEL| Velocities initialization
 MD_VEL| Initial temperature [K]                                      300.000000
 MD_VEL| COM velocity            -0.0000000000     0.0000000000    -0.0000000000

 Number of electrons:                                                         48
 Number of occupied orbitals:                                                 24
 Number of molecular orbitals:                                                24

 Number of orbital functions:                                                114
 Number of independent orbital functions:                                    114

 Extrapolation method: initial_guess

 *** WARNING in qs_initial_guess.F:309 :: User requested to restart the    ***
 *** wavefunction from the file named: geom-RESTART.wfn. This file does    ***
 *** not exist. Please check the existence of the file or change properly  ***
 *** the value of the keyword WFN_RESTART_FILE_NAME. Calculation continues ***
 *** using ATOMIC GUESS.                                                   ***



 SCF WAVEFUNCTION OPTIMIZATION

  ----------------------------------- OT ---------------------------------------
  Minimizer      : DIIS                : direct inversion
                                         in the iterative subspace
                                         using   7 DIIS vectors
                                         safer DIIS on
  Preconditioner : FULL_SINGLE_INVERSE : inversion of 
                                         H + eS - 2*(Sc)(c^T*H*c+const)(Sc)^T
  Precond_solver : DEFAULT
  stepsize       :    0.08000000                  energy_gap     :    0.08000000
  eps_taylor     :   0.10000E-15                  max_taylor     :             4
  ----------------------------------- OT ---------------------------------------

  Step     Update method      Time    Convergence         Total energy    Change
  ------------------------------------------------------------------------------
     1 OT DIIS     0.80E-01   18.9     0.12487494      -112.2582270690 -1.12E+02
     2 OT DIIS     0.80E-01    0.1     0.10855209      -114.0048973417 -1.75E+00
     3 OT DIIS     0.80E-01    0.1     0.06831030      -114.9314352147 -9.27E-01
     4 OT DIIS     0.80E-01    0.1     0.05272501      -115.6960003460 -7.65E-01
     5 OT DIIS     0.80E-01    0.1     0.04083096      -116.1312640101 -4.35E-01
     6 OT DIIS     0.80E-01    0.1     0.03046176      -116.3934102316 -2.62E-01
     7 OT DIIS     0.80E-01    0.1     0.02138618      -116.5842086039 -1.91E-01
     8 OT DIIS     0.80E-01    0.1     0.01770227      -116.6652306114 -8.10E-02
     9 OT DIIS     0.80E-01    0.1     0.01169782      -116.7362610745 -7.10E-02
    10 OT DIIS     0.80E-01    0.1     0.00899540      -116.7761586265 -3.99E-02
    11 OT DIIS     0.80E-01    0.1     0.00843082      -116.7966829193 -2.05E-02
    12 OT DIIS     0.80E-01    0.1     0.00528658      -116.8179964126 -2.13E-02
    13 OT DIIS     0.80E-01    0.1     0.00442094      -116.8278291872 -9.83E-03
    14 OT DIIS     0.80E-01    0.1     0.00291102      -116.8376270293 -9.80E-03
    15 OT DIIS     0.80E-01    0.1     0.00226607      -116.8419035554 -4.28E-03
    16 OT DIIS     0.80E-01    0.1     0.00172590      -116.8448536826 -2.95E-03
    17 OT DIIS     0.80E-01    0.1     0.00137824      -116.8464264011 -1.57E-03
    18 OT DIIS     0.80E-01    0.1     0.00107383      -116.8472850202 -8.59E-04
    19 OT DIIS     0.80E-01    0.1     0.00086632      -116.8478026936 -5.18E-04
    20 OT DIIS     0.80E-01    0.1     0.00060392      -116.8482859791 -4.83E-04
    21 OT DIIS     0.80E-01    0.1     0.00046215      -116.8485124506 -2.26E-04
    22 OT DIIS     0.80E-01    0.1     0.00035630      -116.8485927384 -8.03E-05
    23 OT DIIS     0.80E-01    0.1     0.00027620      -116.8486447544 -5.20E-05
    24 OT DIIS     0.80E-01    0.1     0.00021539      -116.8486784310 -3.37E-05
    25 OT DIIS     0.80E-01    0.1     0.00017945      -116.8486959855 -1.76E-05
    26 OT DIIS     0.80E-01    0.1     0.00015116      -116.8487087741 -1.28E-05
    27 OT DIIS     0.80E-01    0.1     0.00013114      -116.8487171605 -8.39E-06
    28 OT DIIS     0.80E-01    0.1     0.00010832      -116.8487256577 -8.50E-06
    29 OT DIIS     0.80E-01    0.1     0.00009587      -116.8487315565 -5.90E-06
    30 OT DIIS     0.80E-01    0.1     0.00008842      -116.8487357493 -4.19E-06
    31 OT DIIS     0.80E-01    0.1     0.00007416      -116.8487405861 -4.84E-06
    32 OT DIIS     0.80E-01    0.1     0.00006315      -116.8487441214 -3.54E-06
    33 OT DIIS     0.80E-01    0.1     0.00005567      -116.8487463814 -2.26E-06
    34 OT DIIS     0.80E-01    0.1     0.00004821      -116.8487484545 -2.07E-06
    35 OT DIIS     0.80E-01    0.1     0.00004274      -116.8487498102 -1.36E-06
    36 OT DIIS     0.80E-01    0.1     0.00003631      -116.8487510848 -1.27E-06
    37 OT DIIS     0.80E-01    0.1     0.00003219      -116.8487520449 -9.60E-07
    38 OT DIIS     0.80E-01    0.1     0.00002998      -116.8487525736 -5.29E-07
    39 OT DIIS     0.80E-01    0.1     0.00002667      -116.8487531310 -5.57E-07
    40 OT DIIS     0.80E-01    0.1     0.00002451      -116.8487535298 -3.99E-07
    41 OT DIIS     0.80E-01    0.1     0.00002270      -116.8487539070 -3.77E-07
    42 OT DIIS     0.80E-01    0.1     0.00002090      -116.8487542706 -3.64E-07
    43 OT DIIS     0.80E-01    0.1     0.00001952      -116.8487545391 -2.69E-07
    44 OT DIIS     0.80E-01    0.1     0.00001798      -116.8487548169 -2.78E-07
    45 OT DIIS     0.80E-01    0.1     0.00001653      -116.8487551386 -3.22E-07
    46 OT DIIS     0.80E-01    0.1     0.00001547      -116.8487553628 -2.24E-07
    47 OT DIIS     0.80E-01    0.1     0.00001395      -116.8487556148 -2.52E-07
    48 OT DIIS     0.80E-01    0.1     0.00001263      -116.8487558063 -1.91E-07
    49 OT DIIS     0.80E-01    0.1     0.00001117      -116.8487559883 -1.82E-07
    50 OT DIIS     0.80E-01    0.1     0.00000983      -116.8487561267 -1.38E-07

  *** SCF run converged in    50 steps ***


  Electronic density on regular grids:        -47.9999999774        0.0000000226
  Core density on regular grids:               47.9999999987       -0.0000000013
  Total charge density on r-space grids:        0.0000000213
  Total charge density g-space grids:           0.0000000213

  Overlap energy of the core charge distribution:               0.00000013217887
  Self energy of the core charge distribution:               -301.67942807122284
  Core Hamiltonian energy:                                     85.89391241443138
  Hartree energy:                                             125.34944820741946
  Exchange-correlation energy:                                -20.36577040356821
  Hartree-Fock Exchange energy:                                -6.04691840597645

  Total energy:                                              -116.84875612673781

 ENERGY| Total FORCE_EVAL ( QS ) energy [a.u.]:             -116.848756217926649

 MD_INI| MD initialization
 MD_INI| Potential energy [hartree]                          -0.116848756218E+03
 MD_INI| Kinetic energy [hartree]                             0.128256021403E-01
 MD_INI| Temperature [K]                                              300.000000
 MD_INI| Cell volume [bohr^3]                                 6.748334583090E+03
 MD_INI| Cell volume [ang^3]                                  1.000000000000E+03
 MD_INI| Cell lengths [bohr]      1.88972613E+01  1.88972613E+01  1.88972613E+01
 MD_INI| Cell lengths [ang]       1.00000000E+01  1.00000000E+01  1.00000000E+01
 MD_INI| Cell angles [deg]        9.00000000E+01  9.00000000E+01  9.00000000E+01

 Number of electrons:                                                         48
 Number of occupied orbitals:                                                 24
 Number of molecular orbitals:                                                24

 Number of orbital functions:                                                114
 Number of independent orbital functions:                                    114

 Extrapolation method: ASPC


 SCF WAVEFUNCTION OPTIMIZATION

  ----------------------------------- OT ---------------------------------------
  Minimizer      : DIIS                : direct inversion
                                         in the iterative subspace
                                         using   7 DIIS vectors
                                         safer DIIS on
  Preconditioner : FULL_SINGLE_INVERSE : inversion of 
                                         H + eS - 2*(Sc)(c^T*H*c+const)(Sc)^T
  Precond_solver : DEFAULT
  stepsize       :    0.08000000                  energy_gap     :    0.08000000
  eps_taylor     :   0.10000E-15                  max_taylor     :             4
  ----------------------------------- OT ---------------------------------------

  Step     Update method      Time    Convergence         Total energy    Change
  ------------------------------------------------------------------------------
     1 OT DIIS     0.80E-01    3.2     0.00112695      -116.8477295812 -1.17E+02
     2 OT DIIS     0.80E-01    0.1     0.00069136      -116.8479473161 -2.18E-04
     3 OT DIIS     0.80E-01    0.1     0.00030810      -116.8480769687 -1.30E-04
     4 OT DIIS     0.80E-01    0.1     0.00012197      -116.8481061733 -2.92E-05
     5 OT DIIS     0.80E-01    0.1     0.00004754      -116.8481107865 -4.61E-06
     6 OT DIIS     0.80E-01    0.1     0.00002152      -116.8481114731 -6.87E-07
     7 OT DIIS     0.80E-01    0.1     0.00001156      -116.8481116044 -1.31E-07
     8 OT DIIS     0.80E-01    0.1     0.00000479      -116.8481116509 -4.65E-08

  *** SCF run converged in     8 steps ***


  Electronic density on regular grids:        -47.9999999571        0.0000000429
  Core density on regular grids:               47.9999999987       -0.0000000013
  Total charge density on r-space grids:        0.0000000416
  Total charge density g-space grids:           0.0000000416

  Overlap energy of the core charge distribution:               0.00000012911475
  Self energy of the core charge distribution:               -301.67942807122284
  Core Hamiltonian energy:                                     85.85598627021145
  Hartree energy:                                             125.37823521764788
  Exchange-correlation energy:                                -20.35863635957127
  Hartree-Fock Exchange energy:                                -6.04426883707062

  Total energy:                                              -116.84811165089063

 ENERGY| Total FORCE_EVAL ( QS ) energy [a.u.]:             -116.848111658696013

 MD| ***************************************************************************
 MD| Step number                                                               1
 MD| Time [fs]                                                          1.000000
 MD| Conserved quantity [hartree]                            -0.116835418936E+03
 MD| ---------------------------------------------------------------------------
 MD|                                          Instantaneous             Averages
 MD| CPU time per MD step [s]                    100.716271           100.716271
 MD| Energy drift per atom [K]           0.115754274049E+01   0.000000000000E+00
 MD| Potential energy [hartree]         -0.116848111659E+03  -0.116848111659E+03
 MD| Kinetic energy [hartree]            0.113061479493E-01   0.113061479493E-01
 MD| Temperature [K]                             264.458881           264.458881
 MD| ***************************************************************************

 Number of electrons:                                                         48
 Number of occupied orbitals:                                                 24
 Number of molecular orbitals:                                                24

 Number of orbital functions:                                                114
 Number of independent orbital functions:                                    114

 Extrapolation method: ASPC


 SCF WAVEFUNCTION OPTIMIZATION

  ----------------------------------- OT ---------------------------------------
  Minimizer      : DIIS                : direct inversion
                                         in the iterative subspace
                                         using   7 DIIS vectors
                                         safer DIIS on
  Preconditioner : FULL_SINGLE_INVERSE : inversion of 
                                         H + eS - 2*(Sc)(c^T*H*c+const)(Sc)^T
  Precond_solver : DEFAULT
  stepsize       :    0.08000000                  energy_gap     :    0.08000000
  eps_taylor     :   0.10000E-15                  max_taylor     :             4
  ----------------------------------- OT ---------------------------------------

  Step     Update method      Time    Convergence         Total energy    Change
  ------------------------------------------------------------------------------
     1 OT DIIS     0.80E-01    3.2     0.00032882      -116.8472640767 -1.17E+02
     2 OT DIIS     0.80E-01    0.1     0.00019855      -116.8472827557 -1.87E-05
     3 OT DIIS     0.80E-01    0.1     0.00006723      -116.8472938766 -1.11E-05
     4 OT DIIS     0.80E-01    0.1     0.00003036      -116.8472951264 -1.25E-06
     5 OT DIIS     0.80E-01    0.1     0.00001150      -116.8472953913 -2.65E-07
     6 OT DIIS     0.80E-01    0.1     0.00000477      -116.8472954301 -3.88E-08

  *** SCF run converged in     6 steps ***


  Electronic density on regular grids:        -47.9999999493        0.0000000507
  Core density on regular grids:               47.9999999987       -0.0000000013
  Total charge density on r-space grids:        0.0000000494
  Total charge density g-space grids:           0.0000000494

  Overlap energy of the core charge distribution:               0.00000013627888
  Self energy of the core charge distribution:               -301.67942807122284
  Core Hamiltonian energy:                                     85.84021573065401
  Hartree energy:                                             125.39096972285142
  Exchange-correlation energy:                                -20.35580294981887
  Hartree-Fock Exchange energy:                                -6.04324999884880

  Total energy:                                              -116.84729543010624

 ENERGY| Total FORCE_EVAL ( QS ) energy [a.u.]:             -116.847295435643915

 MD| ***************************************************************************
 MD| Step number                                                               2
 MD| Time [fs]                                                          2.000000
 MD| Conserved quantity [hartree]                            -0.116835379616E+03
 MD| ---------------------------------------------------------------------------
 MD|                                          Instantaneous             Averages
 MD| CPU time per MD step [s]                     35.476671            68.096471
 MD| Energy drift per atom [K]           0.239917588885E+01   0.119958794443E+01
 MD| Potential energy [hartree]         -0.116847295436E+03  -0.116847703547E+03
 MD| Kinetic energy [hartree]            0.981199679810E-02   0.105590723737E-01
 MD| Temperature [K]                             229.509617           246.984249
 MD| ***************************************************************************

 Number of electrons:                                                         48
 Number of occupied orbitals:                                                 24
 Number of molecular orbitals:                                                24

 Number of orbital functions:                                                114
 Number of independent orbital functions:                                    114

 Extrapolation method: ASPC


 SCF WAVEFUNCTION OPTIMIZATION

  ----------------------------------- OT ---------------------------------------
  Minimizer      : DIIS                : direct inversion
                                         in the iterative subspace
                                         using   7 DIIS vectors
                                         safer DIIS on
  Preconditioner : FULL_SINGLE_INVERSE : inversion of 
                                         H + eS - 2*(Sc)(c^T*H*c+const)(Sc)^T
  Precond_solver : DEFAULT
  stepsize       :    0.08000000                  energy_gap     :    0.08000000
  eps_taylor     :   0.10000E-15                  max_taylor     :             4
  ----------------------------------- OT ---------------------------------------

  Step     Update method      Time    Convergence         Total energy    Change
  ------------------------------------------------------------------------------
     1 OT DIIS     0.80E-01    3.1     0.00026414      -116.8468718871 -1.17E+02
     2 OT DIIS     0.80E-01    0.1     0.00016213      -116.8468840351 -1.21E-05
     3 OT DIIS     0.80E-01    0.1     0.00005273      -116.8468915665 -7.53E-06
     4 OT DIIS     0.80E-01    0.1     0.00002494      -116.8468922949 -7.28E-07
     5 OT DIIS     0.80E-01    0.1     0.00000738      -116.8468924857 -1.91E-07

  *** SCF run converged in     5 steps ***


  Electronic density on regular grids:        -47.9999999602        0.0000000398
  Core density on regular grids:               47.9999999987       -0.0000000013
  Total charge density on r-space grids:        0.0000000385
  Total charge density g-space grids:           0.0000000385

  Overlap energy of the core charge distribution:               0.00000014043946
  Self energy of the core charge distribution:               -301.67942807122284
  Core Hamiltonian energy:                                     85.83882444381089
  Hartree energy:                                             125.39274746399474
  Exchange-correlation energy:                                -20.35573733221211
  Hartree-Fock Exchange energy:                                -6.04329913050111

  Total energy:                                              -116.84689248569097

 ENERGY| Total FORCE_EVAL ( QS ) energy [a.u.]:             -116.846892499927975

 MD| ***************************************************************************
 MD| Step number                                                               3
 MD| Time [fs]                                                          3.000000
 MD| Conserved quantity [hartree]                            -0.116835392655E+03
 MD| ---------------------------------------------------------------------------
 MD|                                          Instantaneous             Averages
 MD| CPU time per MD step [s]                     35.096049            57.096331
 MD| Energy drift per atom [K]           0.198743204794E+01   0.146220264560E+01
 MD| Potential energy [hartree]         -0.116846892500E+03  -0.116847433198E+03
 MD| Kinetic energy [hartree]            0.891199327799E-02   0.100100460085E-01
 MD| Temperature [K]                             208.457892           234.142130
 MD| ***************************************************************************

 -------------------------------------------------------------------------------
 -                                                                             -
 -                                DBCSR STATISTICS                             -
 -                                                                             -
 -------------------------------------------------------------------------------
 COUNTER                                    TOTAL       BLAS       SMM       ACC
 flops     5 x    24 x    24                46080       0.0%    100.0%      0.0%
 flops     5 x     5 x    24               291600       0.0%    100.0%      0.0%
 flops     5 x    24 x     5               782400       0.0%    100.0%      0.0%
 flops    13 x     5 x    24              2021760       0.0%    100.0%      0.0%
 flops     5 x    13 x    24              2021760       0.0%    100.0%      0.0%
 flops    18 x    24 x    18              4541184       0.0%    100.0%      0.0%
 flops    13 x    24 x     5              8136960       0.0%    100.0%      0.0%
 flops     5 x    24 x    13              8136960       0.0%    100.0%      0.0%
 flops    13 x    24 x    18              9839232       0.0%    100.0%      0.0%
 flops    18 x    24 x    13              9839232       0.0%    100.0%      0.0%
 flops    24 x    24 x    18             11446272       0.0%    100.0%      0.0%
 flops    18 x    24 x    24             14141952       0.0%    100.0%      0.0%
 flops    24 x    24 x    24             14819328       0.0%    100.0%      0.0%
 flops    13 x    13 x    24             23654592       0.0%    100.0%      0.0%
 flops    24 x    24 x    13             24800256       0.0%    100.0%      0.0%
 flops    13 x    24 x    24             31120128       0.0%    100.0%      0.0%
 flops    13 x    24 x    13            105942720       0.0%    100.0%      0.0%
 flops inhomo. stacks                           0       0.0%      0.0%      0.0%
 flops total                       271.582416E+06       0.0%    100.0%      0.0%
 flops max/rank                     73.677744E+06       0.0%    100.0%      0.0%
 matmuls inhomo. stacks                         0       0.0%      0.0%      0.0%
 matmuls total                              30939       0.0%    100.0%      0.0%
 number of processed stacks                 30939       0.0%    100.0%      0.0%
 average stack size                                     0.0       1.0       0.0
 marketing flops                   294.646464E+06
 -------------------------------------------------------------------------------
 # multiplications                           1478
 max memory usage/rank             167.968768E+06
 # max total images/rank                        1
 # max 3D layers                                1
 # MPI messages exchanged                 1324288
 MPI messages size (bytes):
  total size                       415.876608E+06
  min size                           0.000000E+00
  max size                           4.608000E+03
  average size                     314.037903E+00
 MPI breakdown and total messages size (bytes):
             size <=      128             1136121                        0
       128 < size <=     8192              188167                415876608
      8192 < size <=    32768                   0                        0
     32768 < size <=   131072                   0                        0
    131072 < size <=  4194304                   0                        0
   4194304 < size <= 16777216                   0                        0
  16777216 < size                               0                        0
 -------------------------------------------------------------------------------
 -                                                                             -
 -                      DBCSR MESSAGE PASSING PERFORMANCE                      -
 -                                                                             -
 -------------------------------------------------------------------------------
 ROUTINE             CALLS      AVE VOLUME [Bytes]
 MP_Bcast               18                     12.
 MP_Allreduce         8005                      8.
 MP_Alltoall          5263                   5728.
 MP_ISend            47280                    581.
 MP_IRecv            47280                    434.
 -------------------------------------------------------------------------------

 -------------------------------------------------------------------------------
 -                                                                             -
 -                                GRID STATISTICS                              -
 -                                                                             -
 -------------------------------------------------------------------------------
 LP    KERNEL             BACKEND                              COUNT     PERCENT
 4     collocate ortho    REF                                  60710      30.36%
 4     integrate ortho    REF                                  59022      29.51%
 3     collocate ortho    REF                                  29857      14.93%
 3     integrate ortho    REF                                  28597      14.30%
 2     collocate ortho    REF                                   6862       3.43%
 2     integrate ortho    REF                                   6486       3.24%
 5     integrate ortho    REF                                   3324       1.66%
 0     collocate general  REF                                   2560       1.28%
 1     integrate general  REF                                   2560       1.28%
 -------------------------------------------------------------------------------

 MEMORY| Estimated peak process memory [MiB]                                 161

 -------------------------------------------------------------------------------
 -                                                                             -
 -                         MESSAGE PASSING PERFORMANCE                         -
 -                                                                             -
 -------------------------------------------------------------------------------

 ROUTINE             CALLS      AVE VOLUME [Bytes]
 MP_Group                4
 MP_Bcast             3841                 277066.
 MP_Allreduce         9568                    118.
 MP_Sync               457
 MP_Alltoall          1737                1040931.
 MP_ISendRecv        38052                  10763.
 MP_Wait             49910
 MP_comm_split          50
 MP_ISend            11088                  38592.
 MP_IRecv            11088                  38592.
 MP_Recv                42                   2736.
 -------------------------------------------------------------------------------


 -------------------------------------------------------------------------------
 -                                                                             -
 -                           R E F E R E N C E S                               -
 -                                                                             -
 -------------------------------------------------------------------------------
 
 CP2K version 8.1, the CP2K developers group (2020).
 CP2K is freely available from https://www.cp2k.org/ .

 Kuehne,Thomas D.; Iannuzzi,Marcella; Del Ben,Mauro;
 Rybkin,Vladimir V.; Seewald,Patrick; Stein,Frederick; Laino,Teodoro;
 Khaliullin,Rustam Z.; Schuett,Ole; Schiffmann,Florian; Golze,Dorothea;
 Wilhelm,Jan; Chulkov,Sergey; Bani-Hashemian,Mohammad Hossein;
 Weber,Valery; Borstnik,Urban; Taillefumier,Mathieu;
 Jakobovits,Alice Shoshana; Lazzaro,Alfio; Pabst,Hans; Mueller,Tiziano;
 Schade,Robert; Guidon,Manuel; Andermatt,Samuel; Holmberg,Nico;
 Schenter,Gregory K.; Hehn,Anna; Bussy,Augustin; Belleflamme,Fabian;
 Tabacchi,Gloria; Gloess,Andreas; Lass,Michael; Bethune,Iain;
 Mundy,Christopher J.; Plessl,Christian; Watkins,Matt;
 VandeVondele,Joost; Krack,Matthias; Hutter,Juerg. 
 The Journal of Chemical Physics, 152 (19), (2020). 
 CP2K: An electronic structure and molecular dynamics software package -
 Quickstep: Efficient and accurate electronic structure calculations.
 https://doi.org/10.1063/5.0007045

 Schuett, Ole; Messmer, Peter; Hutter, Juerg; VandeVondele, Joost. 
 Electronic Structure Calculations on Graphics Processing Units, John
 Wiley & Sons, Ltd, 173-190 (2016). 
 GPU-Accelerated Sparse Matrix-Matrix Multiplication for
 Linear Scaling Density Functional Theory.
 https://doi.org/10.1002/9781118670712.ch8

 Borstnik, U; VandeVondele, J; Weber, V; Hutter, J. 
 PARALLEL COMPUTING, 40 (5-6), 47-58 (2014). 
 Sparse matrix multiplication: The distributed block-compressed sparse
 row library.
 https://doi.org/10.1016/j.parco.2014.03.012

 Hutter, J; Iannuzzi, M; Schiffmann, F; VandeVondele, J. 
 WIREs Comput Mol Sci., 4 (1), 15-25 (2014). 
 CP2K: atomistic simulations of condensed matter systems.
 https://doi.org/10.1002/wcms.1159

 Guidon, M; Hutter, J; VandeVondele, J. 
 JOURNAL OF CHEMICAL THEORY AND COMPUTATION, 5 (11), 3010-3021 (2009). 
 Robust Periodic Hartree-Fock Exchange for Large-Scale Simulations Using
 Gaussian Basis Sets.
 https://doi.org/10.1021/ct900494g

 Guidon, M; Schiffmann, F; Hutter, J; VandeVondele, J. 
 JOURNAL OF CHEMICAL PHYSICS, 128 (21), 214104 (2008). 
 Ab initio molecular dynamics using hybrid density functionals.
 https://doi.org/10.1063/1.2931945

 VandeVondele, J; Hutter, J. 
 JOURNAL OF CHEMICAL PHYSICS, 127 (11), 114105 (2007). 
 Gaussian basis sets for accurate calculations on molecular systems in
 gas and condensed phases.
 https://doi.org/10.1063/1.2770708

 Kuhne, TD; Krack, M; Mohamed, FR; Parrinello, M. 
 PHYSICAL REVIEW LETTERS, 98 (6), 066401 (2007). 
 Efficient and accurate Car-Parrinello-like approach to
 Born-Oppenheimer molecular dynamics.
 https://doi.org/10.1103/PhysRevLett.98.066401

 Krack, M. 
 THEORETICAL CHEMISTRY ACCOUNTS, 114 (1-3), 145-152 (2005). 
 Pseudopotentials for H to Kr optimized for gradient-corrected
 exchange-correlation functionals.
 https://doi.org/10.1007/s00214-005-0655-y

 VandeVondele, J; Krack, M; Mohamed, F; Parrinello, M; Chassaing, T;
 Hutter, J. COMPUTER PHYSICS COMMUNICATIONS, 167 (2), 103-128 (2005). 
 QUICKSTEP: Fast and accurate density functional calculations using a
 mixed Gaussian and plane waves approach.
 https://doi.org/10.1016/j.cpc.2004.12.014

 Frigo, M; Johnson, SG. 
 PROCEEDINGS OF THE IEEE, 93 (2), 216-231 (2005). 
 The design and implementation of FFTW3.
 https://doi.org/10.1109/JPROC.2004.840301

 Kolafa, J. 
 JOURNAL OF COMPUTATIONAL CHEMISTRY, 25 (3), 335-342 (2004). 
 Time-reversible always stable predictor-corrector method for molecular dynamics of polarizable molecules.
 https://doi.org/10.1002/jcc.10385

 VandeVondele, J; Hutter, J. 
 JOURNAL OF CHEMICAL PHYSICS, 118 (10), 4365-4369 (2003). 
 An efficient orbital transformation method for electronic structure
 calculations.
 https://doi.org/10.1063/1.1543154

 Hartwigsen, C; Goedecker, S; Hutter, J. 
 PHYSICAL REVIEW B, 58 (7), 3641-3662 (1998). 
 Relativistic separable dual-space Gaussian pseudopotentials from H to Rn.
 https://doi.org/10.1103/PhysRevB.58.3641

 Lippert, G; Hutter, J; Parrinello, M. 
 MOLECULAR PHYSICS, 92 (3), 477-487 (1997). 
 A hybrid Gaussian and plane wave density functional scheme.
 https://doi.org/10.1080/002689797170220

 Perdew, JP; Burke, K; Ernzerhof, M. 
 PHYSICAL REVIEW LETTERS, 77 (18), 3865-3868 (1996). 
 Generalized gradient approximation made simple.
 https://doi.org/10.1103/PhysRevLett.77.3865

 Goedecker, S; Teter, M; Hutter, J. 
 PHYSICAL REVIEW B, 54 (3), 1703-1710 (1996). 
 Separable dual-space Gaussian pseudopotentials.
 https://doi.org/10.1103/PhysRevB.54.1703

 NOSE, S. JOURNAL OF CHEMICAL PHYSICS, 81 (1), 511-519 (1984). 
 A UNIFIED FORMULATION OF THE CONSTANT TEMPERATURE MOLECULAR-DYNAMICS
 METHODS.
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 NOSE, S. MOLECULAR PHYSICS, 52 (2), 255-268 (1984). 
 A MOLECULAR-DYNAMICS METHOD FOR SIMULATIONS IN THE CANONICAL ENSEMBLE.
 https://doi.org/10.1080/00268978400101201


 -------------------------------------------------------------------------------
 -                                                                             -
 -                                T I M I N G                                  -
 -                                                                             -
 -------------------------------------------------------------------------------
 SUBROUTINE                       CALLS  ASD         SELF TIME        TOTAL TIME
                                MAXIMUM       AVERAGE  MAXIMUM  AVERAGE  MAXIMUM
 CP2K                                 1  1.0    0.022    0.025  171.571  171.571
 qs_mol_dyn_low                       1  2.0    0.111    0.112  171.345  171.348
 qs_forces                            4  3.8    0.001    0.002  171.003  171.004
 rebuild_ks_matrix                   73  8.1    0.000    0.000  167.000  167.004
 qs_ks_build_kohn_sham_matrix        73  9.1    0.009    0.012  167.000  167.004
 hfx_ks_matrix                       73 10.1    0.003    0.004  163.687  163.697
 qs_ks_update_qs_env_forces           4  4.8    0.000    0.000  135.809  135.810
 derivatives_four_center              4  8.8    0.032    0.192  135.550  135.553
 derivatives_four_center_main         4  9.8    0.001    0.001  135.338  135.345
 derivatives_four_center_bin        417 10.8  123.457  134.139  123.457  134.139
 velocity_verlet                      3  3.0    0.063    0.063  106.376  106.377
 qs_energies                          4  4.8    0.001    0.002   35.174   35.174
 scf_env_do_scf                       4  5.8    0.000    0.000   34.791   34.792
 qs_ks_update_qs_env                 73  7.3    0.001    0.001   31.195   31.198
 init_scf_loop                        4  6.8    0.000    0.000   28.288   28.289
 integrate_four_center               73 11.1    0.069    0.488   28.130   28.132
 mp_sum_lv                           31  5.3   11.882   19.738   11.882   19.738
 integrate_four_center_main          73 12.1    0.008    0.009   12.157   12.570
 integrate_four_center_bin         7738 13.1   12.149   12.561   12.149   12.561
 calc_screening_functions             1 12.0    8.268    8.368    9.346    9.455
 scf_env_do_scf_inner_loop           69  6.3    0.002    0.012    6.497    6.499
 calc_pair_dist_radii                 1 12.0    4.713    4.757    5.312    5.365
 -------------------------------------------------------------------------------

 The number of warnings for this run is : 1
 
 -------------------------------------------------------------------------------
  **** **** ******  **  PROGRAM ENDED AT                 2021-11-17 09:53:02.163
 ***** ** ***  *** **   PROGRAM RAN ON                          ga2008.para.bscc
 **    ****   ******    PROGRAM RAN BY                                   scb3056
 ***** **    ** ** **   PROGRAM PROCESS ID                                129715
  **** **  *******  **  PROGRAM STOPPED IN /public1/home/scb3056/fangyg/test/for
                                           um/vacuo
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