[CP2K-user] [CP2K:15083] convergence problem

alberto albesan... at gmail.com
Mon Apr 5 23:04:31 UTC 2021


Thanks!

Il giorno lunedì 5 aprile 2021 alle 23:50:10 UTC+2 tkuehne ha scritto:

> Dear Alberto, 
>
> please also consider the other comments made by Marcella: 
> "The diagonalization should work, but probably with a smaller ALPHA 
> parameter.
> However,  OT with a proper preconditioner should be more efficient in this 
> case.“ 
> With ALPHA equal to 0.4 you have no chance to ever converge your SCF. 
> Please look out for previous mailing list entries and read the HOWTOs at 
> cp2k.org regarding mixing when using diagonalization, or the OT 
> minimizer. 
>
> Best, 
> Thomas
>
> Am 05.04.2021 um 23:09 schrieb alberto <alb... at gmail.com>:
>
>
> Hi,
> I modified the input by doubling the initial cell (C2/c  Z=4) along the b 
> axis and now I have a supercell that contains 8 molecules of pentacarbonyl 
> iron.
> I used the PBE functional instead of LDA and the MOLOPT basis set. I also 
> set EPS_DEFAULT to 10^-10 and EPS_SCF to 10^-9, finally I set all the 
> parameters in the GEO_OPT section to 10^-6.
> However, despite these changes, the calculation still does not converge.
> Did I mistake by chance in the input to double the cell?
> (In &CELL I multiplied the value of side b by two and in &COORD I put all 
> the xyz coordinates of the 88 atoms (8 molecules of Fe(CO)5 contained in 
> the supercell)).
> Or do I have to build an even bigger supercell?
> I attach the input and report below a part of the output:
>
>
>  *******************************************************************************
>  ***                     STARTING GEOMETRY OPTIMIZATION                    
>   ***
>  ***                           CONJUGATE GRADIENTS                        
>    ***
>
>  *******************************************************************************
>
>  Number of electrons:                                                      
>   528
>  Number of occupied orbitals:                                              
>   264
>  Number of molecular orbitals:                                            
>    264
>
>  Number of orbital functions:                                              
>  1248
>  Number of independent orbital functions:                                  
>  1248
>
>  Extrapolation method: initial_guess
>
>  Atomic guess: The first density matrix is obtained in terms of atomic 
> orbitals
>                and electronic configurations assigned to each atomic kind
>
>  Guess for atomic kind: Fe
>
>  Electronic structure
>     Total number of core electrons                                        
>  10.00
>     Total number of valence electrons                                      
> 16.00
>     Total number of electrons                                              
> 26.00
>     Multiplicity                                                   not 
> specified
>     S   [  2.00  2.00] 2.00  2.00
>     P   [  6.00] 6.00
>     D      6.00
>
>
>
>  *******************************************************************************
>                   Iteration          Convergence                    
>  Energy [au]
>
>  *******************************************************************************
>                           1         14.8249                    
> -106.795406193471
>                           2         2.03661                    
> -120.287466467107
>                           3         2.46377                    
> -122.352697916379
>                           4        0.576092                    
> -122.852545249184
>                           5        0.329756E-01                
> -122.888353225416
>                           6        0.623378E-03                
> -122.888489236999
>                           7        0.564325E-04                
> -122.888489283114
>                           8        0.164041E-04                
> -122.888489283468
>                           9        0.106484E-06                
> -122.888489283501
>
>  Energy components [Hartree]           Total Energy ::        
>  -122.888489283501
>                                         Band Energy ::          
> -21.752000268978
>                                      Kinetic Energy ::          
>  66.582412286099
>                                    Potential Energy ::        
>  -189.470901569599
>                                       Virial (-V/T) ::            
> 2.845659913243
>                                         Core Energy ::        
>  -215.392822441651
>                                           XC Energy ::          
> -12.609477201747
>                                      Coulomb Energy ::          
> 105.113810359898
>                        Total Pseudopotential Energy ::        
>  -282.035412197494
>                        Local Pseudopotential Energy ::        
>  -259.215609175121
>                     Nonlocal Pseudopotential Energy ::          
> -22.819803022372
>                                         Confinement ::            
> 0.601774697437
>
>  Orbital energies  State     L     Occupation   Energy[a.u.]          
> Energy[eV]
>
>                        1     0          2.000      -3.491927          
> -95.020158
>                        2     0          2.000      -0.162226          
>  -4.414387
>
>                        1     1          6.000      -2.160435          
> -58.788434
>
>                        1     2          6.000      -0.246847          
>  -6.717056
>
>
>  Total Electron Density at R=0:                                        
>  0.007824
>
>  Guess for atomic kind: C
>
>  Electronic structure
>     Total number of core electrons                                        
>   2.00
>     Total number of valence electrons                                      
>  4.00
>     Total number of electrons                                              
>  6.00
>     Multiplicity                                                   not 
> specified
>     S   [  2.00] 2.00
>     P      2.00
>
>
>
>  *******************************************************************************
>                   Iteration          Convergence                    
>  Energy [au]
>
>  *******************************************************************************
>                           1        0.427148E-01                  
> -5.227811253113
>                           2        0.218489E-01                  
> -5.228672519307
>                           3        0.666851E-04                  
> -5.228969180638
>                           4        0.102221E-07                  
> -5.228969183366
>
>  Energy components [Hartree]           Total Energy ::          
>  -5.228969183366
>                                         Band Energy ::           -
> 1.112012594120 <(201)%20259-4120>
>                                      Kinetic Energy ::            
> 3.667652954033
>                                    Potential Energy ::          
>  -8.896622137400
>                                       Virial (-V/T) ::            
> 2.425699009394
>                                         Core Energy ::          
>  -8.354438099696
>                                           XC Energy ::          
>  -1.430507543452
>                                      Coulomb Energy ::            
> 4.555976459783
>                        Total Pseudopotential Energy ::          
> -12.054077133824
>                        Local Pseudopotential Energy ::          
> -12.576063923110
>                     Nonlocal Pseudopotential Energy ::            
> 0.521986789286
>                                         Confinement ::            
> 0.319860800937
>
>  Orbital energies  State     L     Occupation   Energy[a.u.]          
> Energy[eV]
>
>                        1     0          2.000      -0.418938          
> -11.399891
>
>                        1     1          2.000      -0.137068          
>  -3.729809
>
>
>  Total Electron Density at R=0:                                        
>  0.015856
>
>  Guess for atomic kind: O
>
>  Electronic structure
>     Total number of core electrons                                        
>   2.00
>     Total number of valence electrons                                      
>  6.00
>     Total number of electrons                                              
>  8.00
>     Multiplicity                                                   not 
> specified
>     S   [  2.00] 2.00
>     P      4.00
>
>
>
>  *******************************************************************************
>                   Iteration          Convergence                    
>  Energy [au]
>
>  *******************************************************************************
>                           1        0.708315                    
>  -15.576645311500
>                           2        0.608879                    
>  -15.587933561584
>                           3        0.102828E-01                
>  -15.656849565404
>                           4        0.113889E-02                
>  -15.656866888140
>                           5        0.434197E-03                
>  -15.656867072159
>                           6        0.263771E-03                
>  -15.656867091904
>                           7        0.478536E-06                
>  -15.656867103452
>
>  Energy components [Hartree]           Total Energy ::          
> -15.656867103452
>                                         Band Energy ::          
>  -3.000198112285
>                                      Kinetic Energy ::          
>  11.759971203220
>                                    Potential Energy ::          
> -27.416838306672
>                                       Virial (-V/T) ::            
> 2.331369510426
>                                         Core Energy ::          
> -26.140716385623
>                                           XC Energy ::          
>  -3.154051012914
>                                      Coulomb Energy ::          
>  13.637900295084
>                        Total Pseudopotential Energy ::          
> -37.935781716540
>                        Local Pseudopotential Energy ::          
> -39.218907440693
>                     Nonlocal Pseudopotential Energy ::            
> 1.283125724153
>                                         Confinement ::            
> 0.350941276976
>
>  Orbital energies  State     L     Occupation   Energy[a.u.]          
> Energy[eV]
>
>                        1     0          2.000      -0.864471          
> -23.523463
>
>                        1     1          4.000      -0.317814          
>  -8.648154
>
>
>  Total Electron Density at R=0:                                        
>  0.000068
>  Re-scaling the density matrix to get the right number of electrons
>                   # Electrons              Trace(P)               Scaling 
> factor
>                           528               527.990                        
> 1.000
>
>
>  SCF WAVEFUNCTION OPTIMIZATION
>
>   Step     Update method      Time    Convergence         Total energy    
> Change
>   
> ------------------------------------------------------------------------------
>      1 P_Mix/Diag. 0.40E+00   62.7     1.69092602     -1851.6808675581 
> -1.85E+03
>      2 P_Mix/Diag. 0.40E+00  104.9     0.91560856     -1853.5283348327 
> -1.85E+00
>      3 P_Mix/Diag. 0.40E+00  103.7     1.02289324     -1851.8136773239  
> 1.71E+00
>      4 P_Mix/Diag. 0.40E+00   98.2     1.41348942     -1847.7932049729  
> 4.02E+00
>      5 P_Mix/Diag. 0.40E+00   96.7     1.20443292     -1842.5746730660  
> 5.22E+00
>      6 P_Mix/Diag. 0.40E+00   97.4     1.30049803     -1834.8292755631  
> 7.75E+00
>      7 P_Mix/Diag. 0.40E+00   97.5     1.22092629     -1832.8966285502  
> 1.93E+00
>      8 P_Mix/Diag. 0.40E+00   97.1     1.25626273     -1827.5323998647  
> 5.36E+00
>      9 P_Mix/Diag. 0.40E+00   97.2     1.22716656     -1827.9738471293 
> -4.41E-01
>     10 P_Mix/Diag. 0.40E+00   97.2     1.24788747     -1824.0201462744  
> 3.95E+00
>     11 P_Mix/Diag. 0.40E+00   99.4     1.22972041     -1824.6169634874 
> -5.97E-01
>     12 P_Mix/Diag. 0.40E+00  100.0     1.24229237     -1822.0246113641  
> 2.59E+00
>     13 P_Mix/Diag. 0.40E+00   96.6     1.23413457     -1822.7804509206 
> -7.56E-01
>     14 P_Mix/Diag. 0.40E+00  102.0     1.24337481     -1818.2257573281  
> 4.55E+00
>     15 P_Mix/Diag. 0.40E+00  102.2     1.33929099     -1819.0972529629 
> -8.71E-01
>     16 P_Mix/Diag. 0.40E+00  102.1     1.66323686     -1811.3814811141  
> 7.72E+00
>     17 P_Mix/Diag. 0.40E+00   99.9     1.44700743     -1811.9508178679 
> -5.69E-01
>     18 P_Mix/Diag. 0.40E+00  101.1     5.36013228     -1801.9699460004  
> 9.98E+00
>     19 P_Mix/Diag. 0.40E+00  100.2    14.77488581     -1750.5158775272  
> 5.15E+01
>     20 P_Mix/Diag. 0.40E+00  101.6    10.91072116     -1436.1218181856  
> 3.14E+02
>     21 P_Mix/Diag. 0.40E+00  102.9    13.21277811     -1394.9166145334  
> 4.12E+01
>     22 P_Mix/Diag. 0.40E+00   98.2    12.00300339     -1325.1212541013  
> 6.98E+01
>     23 P_Mix/Diag. 0.40E+00   98.1     8.68757983     -1302.6763819085  
> 2.24E+01
>     24 P_Mix/Diag. 0.40E+00   95.9    16.63552589     -1285.1428858449  
> 1.75E+01
>     25 P_Mix/Diag. 0.40E+00   96.9    18.20488057     -1212.6433885733  
> 7.25E+01
>     26 P_Mix/Diag. 0.40E+00   96.9    12.35664328     -1111.8052793195  
> 1.01E+02
>     27 P_Mix/Diag. 0.40E+00   98.2    33.06806566     -1337.1684278721 
> -2.25E+02
>     28 P_Mix/Diag. 0.40E+00   98.2    16.61930989     -1034.4727815068  
> 3.03E+02
>     29 P_Mix/Diag. 0.40E+00   98.8     9.12791551     -1115.0880365726 
> -8.06E+01
>     30 P_Mix/Diag. 0.40E+00   96.6    14.52402953     -1461.6901199471 
> -3.47E+02
>     31 P_Mix/Diag. 0.40E+00  101.7    32.04778754     -1392.3294706673  
> 6.94E+01
>     32 P_Mix/Diag. 0.40E+00   98.2    17.17382715      -964.7040633562  
> 4.28E+02
>     33 P_Mix/Diag. 0.40E+00   97.5    31.91519006     -1235.3388640364 
> -2.71E+02
>     34 P_Mix/Diag. 0.40E+00  100.1    20.69924660      -985.1143873470  
> 2.50E+02
>     35 P_Mix/Diag. 0.40E+00  100.9    25.79642224      -999.7363038951 
> -1.46E+01
>     36 P_Mix/Diag. 0.40E+00  101.8    38.33198147     -1051.5722739128 
> -5.18E+01
>     37 P_Mix/Diag. 0.40E+00  101.1    17.94601028      -943.5935470500  
> 1.08E+02
>     38 P_Mix/Diag. 0.40E+00  103.1    80.31329474     -1163.5431903152 
> -2.20E+02
>     39 P_Mix/Diag. 0.40E+00   99.5    36.76614890      -835.2760980829  
> 3.28E+02
>     40 P_Mix/Diag. 0.40E+00   97.8    19.81123303     -1073.8011620784 
> -2.39E+02
>     41 P_Mix/Diag. 0.40E+00   96.2    31.01187840     -1051.9119791259  
> 2.19E+01
>     42 P_Mix/Diag. 0.40E+00   97.6    17.39183279      -846.9831106824  
> 2.05E+02
>     43 P_Mix/Diag. 0.40E+00   96.8    24.03408634     -1129.2563041911 
> -2.82E+02
>     44 P_Mix/Diag. 0.40E+00   95.4    16.90530493      -910.1306525099  
> 2.19E+02
>     45 P_Mix/Diag. 0.40E+00   95.7    59.27570620     -1131.4800219994 
> -2.21E+02
>     46 P_Mix/Diag. 0.40E+00   97.6    30.02882019      -860.8775491868  
> 2.71E+02
>     47 P_Mix/Diag. 0.40E+00   97.3    17.01555337      -933.2187974271 
> -7.23E+01
>     48 P_Mix/Diag. 0.40E+00   99.0    35.26329159     -1211.9912170956 
> -2.79E+02
>     49 P_Mix/Diag. 0.40E+00   98.8    18.66880664      -804.5908610578  
> 4.07E+02
>     50 P_Mix/Diag. 0.40E+00   99.8    23.05648944     -1165.6938452478 
> -3.61E+02
>     51 P_Mix/Diag. 0.40E+00  100.1    18.28000308      -859.9367249030  
> 3.06E+02
>     52 P_Mix/Diag. 0.40E+00   99.6    23.66008469     -1041.3457288030 
> -1.81E+02
>     53 P_Mix/Diag. 0.40E+00  100.4    22.11861643      -971.4475072560  
> 6.99E+01
>     54 P_Mix/Diag. 0.40E+00  102.0    16.40678499      -918.7612939608  
> 5.27E+01
>     55 P_Mix/Diag. 0.40E+00   99.7    58.34775622     -1228.9231857448 
> -3.10E+02
>     56 P_Mix/Diag. 0.40E+00  100.6    27.96182255      -810.5552115589  
> 4.18E+02
>     57 P_Mix/Diag. 0.40E+00  102.5    21.76037575     -1158.2789845268 
> -3.48E+02
>     58 P_Mix/Diag. 0.40E+00  101.2    22.94670510      -859.8094035901  
> 2.98E+02
>     59 P_Mix/Diag. 0.40E+00  100.5    25.28596991      -967.9594635827 
> -1.08E+02
>     60 P_Mix/Diag. 0.40E+00   98.1    25.05988117      -971.9374423966 
> -3.98E+00
>     61 P_Mix/Diag. 0.40E+00   98.0    13.44070904      -912.0768553982  
> 5.99E+01
>     62 P_Mix/Diag. 0.40E+00   97.4    46.75959133     -1225.0185705532 
> -3.13E+02
>     63 P_Mix/Diag. 0.40E+00   96.3    23.14237412      -799.0353482555  
> 4.26E+02
>     64 P_Mix/Diag. 0.40E+00   97.0    20.62323300     -1180.7020991927 
> -3.82E+02
>     65 P_Mix/Diag. 0.40E+00   97.1    23.55555111      -884.8111282719  
> 2.96E+02
>     66 P_Mix/Diag. 0.40E+00  102.4    24.20461551      -943.2449315052 
> -5.84E+01
>     67 P_Mix/Diag. 0.40E+00   97.9    23.40294593      -976.0677604109 
> -3.28E+01
>     68 P_Mix/Diag. 0.40E+00   99.3    11.06519571      -902.6105618312  
> 7.35E+01
>     69 P_Mix/Diag. 0.40E+00  100.3    57.53271386     -1292.1019352485 
> -3.89E+02
>     70 P_Mix/Diag. 0.40E+00   99.2    27.39194427      -859.3231449036  
> 4.33E+02
>     71 P_Mix/Diag. 0.40E+00  100.5    30.70054471     -1172.1215599654 
> -3.13E+02
>     72 P_Mix/Diag. 0.40E+00  101.9    27.19461440      -954.6060695234  
> 2.18E+02
>     73 P_Mix/Diag. 0.40E+00  104.0    24.02562309      -925.2962626414  
> 2.93E+01
>     74 P_Mix/Diag. 0.40E+00  102.4    56.53403632     -1027.3554004412 
> -1.02E+02
>     75 P_Mix/Diag. 0.40E+00  100.5    24.80098770      -922.4786081760  
> 1.05E+02
>     76 P_Mix/Diag. 0.40E+00   98.1    64.14930634     -1183.5887565546 
> -2.61E+02
>     77 P_Mix/Diag. 0.40E+00   96.5    31.67544217      -862.6067421481  
> 3.21E+02
>     78 P_Mix/Diag. 0.40E+00   98.0    20.26283157     -1142.7381930936 
> -2.80E+02
>     79 P_Mix/Diag. 0.40E+00   95.3    31.01402812      -947.6284938342  
> 1.95E+02
>     80 P_Mix/Diag. 0.40E+00   95.9    23.77409716      -908.9230914378  
> 3.87E+01
>     81 P_Mix/Diag. 0.40E+00   97.7    23.84615164     -1064.0101803204 
> -1.55E+02
>     82 P_Mix/Diag. 0.40E+00   99.5    11.25709918      -919.7549446962  
> 1.44E+02
>     83 P_Mix/Diag. 0.40E+00   96.1    45.26275480     -1246.9030665712 
> -3.27E+02
>     84 P_Mix/Diag. 0.40E+00   97.1    24.45558940      -816.3139885235  
> 4.31E+02
>     85 P_Mix/Diag. 0.40E+00   98.6    19.36050278     -1085.2679225233 
> -2.69E+02
>     86 P_Mix/Diag. 0.40E+00   97.1    38.62693630     -1049.2946714099  
> 3.60E+01
>     87 P_Mix/Diag. 0.40E+00  100.2    21.51755196      -840.5690565649  
> 2.09E+02
>     88 P_Mix/Diag. 0.40E+00  101.2    21.99078821     -1066.2780932869 
> -2.26E+02
>     89 P_Mix/Diag. 0.40E+00  102.0    10.74427656      -892.3558279894  
> 1.74E+02
>     90 P_Mix/Diag. 0.40E+00  101.4    51.37315652     -1231.5382917367 
> -3.39E+02
>     91 P_Mix/Diag. 0.40E+00  101.8    26.72278034      -825.0355016352  
> 4.07E+02
>     92 P_Mix/Diag. 0.40E+00  102.5    17.33755788     -1094.6337011870 
> -2.70E+02
>     93 P_Mix/Diag. 0.40E+00  101.3    42.09998983     -1084.7522524272  
> 9.88E+00
>     94 P_Mix/Diag. 0.40E+00   99.4    20.44362626      -856.8792234441  
> 2.28E+02
>     95 P_Mix/Diag. 0.40E+00   96.7    22.38018358     -1096.1064504797 
> -2.39E+02
>     96 P_Mix/Diag. 0.40E+00   95.4    10.89486027      -868.0550739178  
> 2.28E+02
>     97 P_Mix/Diag. 0.40E+00   97.1    53.29467002     -1197.7300238728 
> -3.30E+02
>     98 P_Mix/Diag. 0.40E+00   96.8    27.80027985      -795.0907375629  
> 4.03E+02
>     99 P_Mix/Diag. 0.40E+00  102.8    14.35694411     -1096.3682527208 
> -3.01E+02
>    100 P_Mix/Diag. 0.40E+00  100.6    35.80110189     -1135.3741412955 
> -3.90E+01
>    101 P_Mix/Diag. 0.40E+00  100.4    19.81139096      -875.5256510285  
> 2.60E+02
>    102 P_Mix/Diag. 0.40E+00  102.9    22.75624724     -1116.3541827784 
> -2.41E+02
>    103 P_Mix/Diag. 0.40E+00   97.8    11.11886225      -894.5904055750  
> 2.22E+02
>    104 P_Mix/Diag. 0.40E+00  100.0    51.80956888     -1188.7262862865 
> -2.94E+02
>    105 P_Mix/Diag. 0.40E+00   99.5    26.08561112      -816.4883844255  
> 3.72E+02
>    106 P_Mix/Diag. 0.40E+00   97.3    14.20610318     -1081.8377752873 
> -2.65E+02
>    107 P_Mix/Diag. 0.40E+00   98.5    33.66786187     -1159.0609364273 
> -7.72E+01
>    108 P_Mix/Diag. 0.40E+00   98.4    18.33644970      -871.7220495279  
> 2.87E+02
>    109 P_Mix/Diag. 0.40E+00   98.5    23.00560669     -1118.3105782284 
> -2.47E+02
>    110 P_Mix/Diag. 0.40E+00   97.1    11.20743010      -872.5451841925  
> 2.46E+02
>    111 P_Mix/Diag. 0.40E+00   96.7    65.62905561     -1238.9527674375 
> -3.66E+02
>    112 P_Mix/Diag. 0.40E+00   95.7    32.82823036      -826.6879860593  
> 4.12E+02
>    113 P_Mix/Diag. 0.40E+00   97.3    19.38725959     -1069.1230989736 
> -2.42E+02
>    114 P_Mix/Diag. 0.40E+00   96.8    44.05441053     -1064.0691519896  
> 5.05E+00
>    115 P_Mix/Diag. 0.40E+00   97.1    21.80973421      -823.0198435086  
> 2.41E+02
>    116 P_Mix/Diag. 0.40E+00   98.1    24.43896596     -1077.3956558775 
> -2.54E+02
>    117 P_Mix/Diag. 0.40E+00   99.0    12.34308471      -867.4388990297  
> 2.10E+02
>    118 P_Mix/Diag. 0.40E+00   98.7    87.75237500     -1218.4938729448 
> -3.51E+02
>    119 P_Mix/Diag. 0.40E+00   98.4    42.45927820      -882.0255822316  
> 3.36E+02
>    120 P_Mix/Diag. 0.40E+00   99.0    22.48035977     -1034.2700212223 
> -1.52E+02
>    121 P_Mix/Diag. 0.40E+00   99.4    31.62997437     -1086.0436209964 
> -5.18E+01
>    122 P_Mix/Diag. 0.40E+00   95.8    17.74546462      -839.4765661623  
> 2.47E+02
>    123 P_Mix/Diag. 0.40E+00   97.6    37.47067790     -1107.0880120993 
> -2.68E+02
>    124 P_Mix/Diag. 0.40E+00   98.1    18.14715773      -898.5309040155  
> 2.09E+02
>    125 P_Mix/Diag. 0.40E+00   98.1    37.95382684     -1076.9081598424 
> -1.78E+02
>    126 P_Mix/Diag. 0.40E+00   95.6    21.35246371      -949.1274613873  
> 1.28E+02
>    127 P_Mix/Diag. 0.40E+00   97.2    16.45524120      -959.4569479527 
> -1.03E+01
>    128 P_Mix/Diag. 0.40E+00   98.0    33.52162195     -1207.1859894609 
> -2.48E+02
>    129 P_Mix/Diag. 0.40E+00   98.1    18.03581293      -820.8095617582  
> 3.86E+02
>    130 P_Mix/Diag. 0.40E+00   96.5    24.32217110     -1169.5026175257 
> -3.49E+02
>    131 P_Mix/Diag. 0.40E+00   97.1    18.41300418      -864.2056309297  
> 3.05E+02
>    132 P_Mix/Diag. 0.40E+00   98.3    24.88125411     -1017.9233010706 
> -1.54E+02
>    133 P_Mix/Diag. 0.40E+00   98.0    21.63608416      -983.4173091982  
> 3.45E+01
>    134 P_Mix/Diag. 0.40E+00   96.3    14.46172571      -919.4776228422  
> 6.39E+01
>    135 P_Mix/Diag. 0.40E+00   96.3    55.53616574     -1230.4687549313 
> -3.11E+02
>    136 P_Mix/Diag. 0.40E+00   97.5    26.72883699      -823.9104763529  
> 4.07E+02
>    137 P_Mix/Diag. 0.40E+00   98.1    21.99264748     -1166.1687536714 
> -3.42E+02
>    138 P_Mix/Diag. 0.40E+00   95.3    21.90205040      -894.1451754196  
> 2.72E+02
>    139 P_Mix/Diag. 0.40E+00   96.0    24.64821764      -941.0486213079 
> -4.69E+01
>    140 P_Mix/Diag. 0.40E+00   96.6    23.59007469     -1009.4650250052 
> -6.84E+01
>    141 P_Mix/Diag. 0.40E+00   95.5    11.19653600      -910.3270098712  
> 9.91E+01
>    142 P_Mix/Diag. 0.40E+00   99.4    35.12338189     -1243.7468433805 
> -3.33E+02
>    143 P_Mix/Diag. 0.40E+00   97.0    19.22011435      -785.0286929800  
> 4.59E+02
>    144 P_Mix/Diag. 0.40E+00   96.3    22.88174741     -1156.3171428551 
> -3.71E+02
>    145 P_Mix/Diag. 0.40E+00   96.7    28.52534682      -881.8826315770  
> 2.74E+02
>    146 P_Mix/Diag. 0.40E+00   97.0    24.83395145      -895.2961402888 
> -1.34E+01
>    147 P_Mix/Diag. 0.40E+00   95.7    23.30075503     -1019.2035119347 
> -1.24E+02
>    148 P_Mix/Diag. 0.40E+00   97.7    11.05468470      -910.4546396591  
> 1.09E+02
>    149 P_Mix/Diag. 0.40E+00   95.8    42.72608972     -1253.4781387895 
> -3.43E+02
>    150 P_Mix/Diag. 0.40E+00   96.3    23.08051794      -791.7513269410  
> 4.62E+02
>    151 P_Mix/Diag. 0.40E+00   96.0    20.39854372     -1159.8896868165 
> -3.68E+02
>    152 P_Mix/Diag. 0.40E+00   96.5    26.49778812      -928.4568627257  
> 2.31E+02
>    153 P_Mix/Diag. 0.40E+00   97.4    21.61417357      -887.6815489935  
> 4.08E+01
>    154 P_Mix/Diag. 0.40E+00   97.7    23.28419341     -1034.7510821646 
> -1.47E+02
>    155 P_Mix/Diag. 0.40E+00   96.8    11.10357402      -899.4608692489  
> 1.35E+02
>    156 P_Mix/Diag. 0.40E+00   96.7    51.85070315     -1231.9506855794 
> -3.32E+02
>    157 P_Mix/Diag. 0.40E+00   96.7    26.44245406      -794.7318377126  
> 4.37E+02
>    158 P_Mix/Diag. 0.40E+00   95.9    18.95863693     -1153.9898143475 
> -3.59E+02
>    159 P_Mix/Diag. 0.40E+00   98.2    32.18559018      -992.7458612110  
> 1.61E+02
>    160 P_Mix/Diag. 0.40E+00  100.0    21.65239287      -876.6226186752  
> 1.16E+02
>    161 P_Mix/Diag. 0.40E+00   95.5    22.98451693     -1060.1059192849 
> -1.83E+02
>    162 P_Mix/Diag. 0.40E+00   98.6    11.05631984      -906.7147780665  
> 1.53E+02
>    163 P_Mix/Diag. 0.40E+00   98.0    48.33439880     -1243.3470399355 
> -3.37E+02
>    164 P_Mix/Diag. 0.40E+00  100.1    25.56369641      -803.4049706786  
> 4.40E+02
>    165 P_Mix/Diag. 0.40E+00   98.8    17.61519964     -1132.2676782900 
> -3.29E+02
>    166 P_Mix/Diag. 0.40E+00  100.8    39.39491035     -1051.0428153931  
> 8.12E+01
>    167 P_Mix/Diag. 0.40E+00   96.9    21.92704671      -870.7920195518  
> 1.80E+02
>    168 P_Mix/Diag. 0.40E+00   99.4    23.32414374     -1069.7753085390 
> -1.99E+02
>    169 P_Mix/Diag. 0.40E+00   96.9    11.24971181      -908.1992907564  
> 1.62E+02
>    170 P_Mix/Diag. 0.40E+00   98.1    51.78341035     -1236.7988323693 
> -3.29E+02
>    171 P_Mix/Diag. 0.40E+00   97.9    27.03970382      -811.5864348553  
> 4.25E+02
>    172 P_Mix/Diag. 0.40E+00   97.0    17.89861734     -1086.4687449891 
> -2.75E+02
>    173 P_Mix/Diag. 0.40E+00   97.3    37.70174179     -1061.8461784396  
> 2.46E+01
>    174 P_Mix/Diag. 0.40E+00   96.7    20.55630156      -847.6131641385  
> 2.14E+02
>    175 P_Mix/Diag. 0.40E+00   96.8    22.09380119     -1084.0439963398 
> -2.36E+02
>    176 P_Mix/Diag. 0.40E+00   95.8    10.81042483      -860.5045599545  
> 2.24E+02
>    177 P_Mix/Diag. 0.40E+00   98.8    52.88756469     -1195.0593479107 
> -3.35E+02
>    178 P_Mix/Diag. 0.40E+00   97.4    27.64745391      -799.4990141057  
> 3.96E+02
>    179 P_Mix/Diag. 0.40E+00   97.5    17.31963976     -1106.4093184512 
> -3.07E+02
>    180 P_Mix/Diag. 0.40E+00   99.3    37.72008781     -1083.9979032916  
> 2.24E+01
>    181 P_Mix/Diag. 0.40E+00   97.8    19.48954723      -878.9588267277  
> 2.05E+02
>    182 P_Mix/Diag. 0.40E+00   97.8    22.77592349     -1096.6259150752 
> -2.18E+02
>    183 P_Mix/Diag. 0.40E+00   98.4    11.09666704      -889.0690481572  
> 2.08E+02
>    184 P_Mix/Diag. 0.40E+00  100.2    49.28010195     -1185.1296448309 
> -2.96E+02
>    185 P_Mix/Diag. 0.40E+00   99.5    26.07064171      -807.0850496218  
> 3.78E+02
>    186 P_Mix/Diag. 0.40E+00  100.2    16.92229569     -1106.9693792364 
> -3.00E+02
>    187 P_Mix/Diag. 0.40E+00   98.7    39.92314751     -1071.4952514972  
> 3.55E+01
>    188 P_Mix/Diag. 0.40E+00   97.2    20.38155575      -878.4704928595  
> 1.93E+02
>    189 P_Mix/Diag. 0.40E+00   96.5    22.91798216     -1083.3149090979 
> -2.05E+02
>    190 P_Mix/Diag. 0.40E+00   96.5    11.09445855      -916.2470022630  
> 1.67E+02
>    191 P_Mix/Diag. 0.40E+00   96.3    52.40347024     -1239.1045876382 
> -3.23E+02
>    192 P_Mix/Diag. 0.40E+00   95.8    27.81493643      -818.7601021872  
> 4.20E+02
>    193 P_Mix/Diag. 0.40E+00   97.1    17.07280948     -1096.8032139955 
> -2.78E+02
>    194 P_Mix/Diag. 0.40E+00   96.0    40.81129504     -1082.0573735074  
> 1.47E+01
>    195 P_Mix/Diag. 0.40E+00   95.8    20.34092813      -857.7832270641  
> 2.24E+02
>    196 P_Mix/Diag. 0.40E+00   96.9    22.32731258     -1095.3944780182 
> -2.38E+02
>    197 P_Mix/Diag. 0.40E+00   97.3    10.90936723      -867.8418310606  
> 2.28E+02
>    198 P_Mix/Diag. 0.40E+00   97.8    52.73079495     -1197.6914219998 
> -3.30E+02
>    199 P_Mix/Diag. 0.40E+00   99.4    27.49056462      -795.7733320720  
> 4.02E+02
>    200 P_Mix/Diag. 0.40E+00  100.5    14.74518526     -1096.3153384410 
> -3.01E+02
>    201 P_Mix/Diag. 0.40E+00  101.0    38.80524677     -1127.3284544486 
> -3.10E+01
>    202 P_Mix/Diag. 0.40E+00  102.1    19.95344422      -879.8809078868  
> 2.47E+02
>    203 P_Mix/Diag. 0.40E+00  103.8    22.76182497     -1116.3238782556 
> -2.36E+02
>    204 P_Mix/Diag. 0.40E+00  101.2    11.11757729      -893.1723120553  
> 2.23E+02
>    205 P_Mix/Diag. 0.40E+00  100.8    52.77243506     -1188.3421359044 
> -2.95E+02
>    206 P_Mix/Diag. 0.40E+00  100.7    26.08211235      -816.6670557902  
> 3.72E+02
>    207 P_Mix/Diag. 0.40E+00   99.2    14.25935556     -1081.1342523156 
> -2.64E+02
>    208 P_Mix/Diag. 0.40E+00   99.1    33.51671576     -1158.7480585940 
> -7.76E+01
>    209 P_Mix/Diag. 0.40E+00   98.7    18.31922308      -871.9899526035  
> 2.87E+02
>    210 P_Mix/Diag. 0.40E+00   98.3    22.98128847     -1118.2179284490 
> -2.46E+02
>    211 P_Mix/Diag. 0.40E+00   99.7    11.20498379      -873.0843896459  
> 2.45E+02
>    212 P_Mix/Diag. 0.40E+00   95.1    64.76941918     -1234.9852140197 
> -3.62E+02
>    213 P_Mix/Diag. 0.40E+00  100.0    32.45023417      -822.5316092032  
> 4.12E+02
>    214 P_Mix/Diag. 0.40E+00   99.4    19.11349914     -1075.9518671995 
> -2.53E+02
>    215 P_Mix/Diag. 0.40E+00   97.9    43.83614505     -1075.9052811544  
> 4.66E-02
>    216 P_Mix/Diag. 0.40E+00   98.8    21.73594696      -831.1490343055  
> 2.45E+02
>    217 P_Mix/Diag. 0.40E+00   97.1    23.14663205     -1087.9675843673 
> -2.57E+02
>    218 P_Mix/Diag. 0.40E+00   98.9    11.73901359      -874.7903004860  
> 2.13E+02
>    219 P_Mix/Diag. 0.40E+00   97.9    78.24342687     -1192.5158957229 
> -3.18E+02
>    220 P_Mix/Diag. 0.40E+00   99.7    38.71624789      -817.9093767680  
> 3.75E+02
>    221 P_Mix/Diag. 0.40E+00   98.3    21.15140928     -1018.9025214041 
> -2.01E+02
>    222 P_Mix/Diag. 0.40E+00   98.1    38.34288084     -1149.2244612837 
> -1.30E+02
>    223 P_Mix/Diag. 0.40E+00   97.6    20.28993271      -825.1728532594  
> 3.24E+02
>    224 P_Mix/Diag. 0.40E+00   97.4    23.70649458     -1123.4235028708 
> -2.98E+02
>    225 P_Mix/Diag. 0.40E+00   97.7    11.81476765      -859.5988312202  
> 2.64E+02
>    226 P_Mix/Diag. 0.40E+00   98.0    31.42550563     -1221.2317964554 
> -3.62E+02
>    227 P_Mix/Diag. 0.40E+00   97.2    19.49819969      -933.8789257217  
> 2.87E+02
>    228 P_Mix/Diag. 0.40E+00   98.1    17.87283388     -1012.0518290875 
> -7.82E+01
>    229 P_Mix/Diag. 0.40E+00   98.0    56.72650081     -1154.1250708120 
> -1.42E+02
>    230 P_Mix/Diag. 0.40E+00  100.0    27.36226064      -807.0742560965  
> 3.47E+02
>    231 P_Mix/Diag. 0.40E+00  100.6    22.11925333     -1142.6196427376 
> -3.36E+02
>    232 P_Mix/Diag. 0.40E+00  102.9    13.10044550      -850.7979577263  
> 2.92E+02
>    233 P_Mix/Diag. 0.40E+00  102.5    60.30493694     -1132.9797284904 
> -2.82E+02
>    234 P_Mix/Diag. 0.40E+00  102.9    31.15409644      -834.6236263149  
> 2.98E+02
>    235 P_Mix/Diag. 0.40E+00  103.6    15.51660776      -959.9625401973 
> -1.25E+02
>    236 P_Mix/Diag. 0.40E+00   99.2    38.99433728     -1220.7633762007 
> -2.61E+02
>    237 P_Mix/Diag. 0.40E+00   97.7    20.16385947      -830.2019189221  
> 3.91E+02
>    238 P_Mix/Diag. 0.40E+00   98.6    22.77711329     -1177.7307552645 
> -3.48E+02
>    239 P_Mix/Diag. 0.40E+00   96.7    15.97802379      -881.7114314148  
> 2.96E+02
>    240 P_Mix/Diag. 0.40E+00   97.0    25.33006438     -1056.4447125183 
> -1.75E+02
>    241 P_Mix/Diag. 0.40E+00   98.3    42.10315845      -927.2894306230  
> 1.29E+02
>    242 P_Mix/Diag. 0.40E+00   98.0    18.28678357      -931.5072979346 
> -4.22E+00
>    243 P_Mix/Diag. 0.40E+00   97.2    46.60186459     -1219.8051910978 
> -2.88E+02
>    244 P_Mix/Diag. 0.40E+00   96.7    23.56963381      -815.0397919155  
> 4.05E+02
>    245 P_Mix/Diag. 0.40E+00   97.5    22.20346113     -1172.7696305137 
> -3.58E+02
>    246 P_Mix/Diag. 0.40E+00   97.6    19.82352223      -878.3989108752  
> 2.94E+02
>    247 P_Mix/Diag. 0.40E+00   97.6    45.08615493     -1048.4788751056 
> -1.70E+02
>    248 P_Mix/Diag. 0.40E+00   96.7    30.44647676      -993.0197281219  
> 5.55E+01
>    249 P_Mix/Diag. 0.40E+00   97.3    17.79172438      -917.2567849516  
> 7.58E+01
>    250 P_Mix/Diag. 0.40E+00   96.1    48.75376149     -1200.3528428921 
> -2.83E+02
>    251 P_Mix/Diag. 0.40E+00   96.3    23.69503201      -793.7497071293  
> 4.07E+02
>    252 P_Mix/Diag. 0.40E+00   97.4    21.95553378     -1145.6032813331 
> -3.52E+02
>    253 P_Mix/Diag. 0.40E+00   96.2    38.03323687      -896.7793321383  
> 2.49E+02
>    254 P_Mix/Diag. 0.40E+00   95.9    25.25104518      -955.9091167439 
> -5.91E+01
>    255 P_Mix/Diag. 0.40E+00   97.1    23.63381200      -996.6516142650 
> -4.07E+01
>    256 P_Mix/Diag. 0.40E+00   97.6    13.83859878      -911.0735420978  
> 8.56E+01
>    257 P_Mix/Diag. 0.40E+00   96.7    68.67574089     -1233.8573555137 
> -3.23E+02
>    258 P_Mix/Diag. 0.40E+00   97.3    31.74069431      -812.6888717700  
> 4.21E+02
>    259 P_Mix/Diag. 0.40E+00   95.9    21.06207656     -1136.9012668149 
> -3.24E+02
>    260 P_Mix/Diag. 0.40E+00   98.7    29.95853333      -933.7068307891  
> 2.03E+02
>    261 P_Mix/Diag. 0.40E+00   97.4    24.12628025      -873.4409303622  
> 6.03E+01
>    262 P_Mix/Diag. 0.40E+00   98.0    23.36458436     -1034.0621101862 
> -1.61E+02
>    263 P_Mix/Diag. 0.40E+00   97.3    12.20733174      -900.5467424928  
> 1.34E+02
>    264 P_Mix/Diag. 0.40E+00   97.2    46.97197035     -1230.3069518724 
> -3.30E+02
>    265 P_Mix/Diag. 0.40E+00   99.2    24.31911296      -801.1766241399  
> 4.29E+02
>    266 P_Mix/Diag. 0.40E+00   98.8    19.37157269     -1127.6037909096 
> -3.26E+02
>    267 P_Mix/Diag. 0.40E+00   99.2    38.90634632      -976.1453804543  
> 1.51E+02
>    268 P_Mix/Diag. 0.40E+00   98.7    22.02783441      -875.9114616287  
> 1.00E+02
>    269 P_Mix/Diag. 0.40E+00  100.0    23.25967956     -1045.5061031449 
> -1.70E+02
>    270 P_Mix/Diag. 0.40E+00   98.9    11.20239364      -903.0492143564  
> 1.42E+02
>    271 P_Mix/Diag. 0.40E+00  100.9    55.28912234     -1251.8164990852 
> -3.49E+02
>    272 P_Mix/Diag. 0.40E+00  100.5    28.25262859      -797.9065458854  
> 4.54E+02
>    273 P_Mix/Diag. 0.40E+00  103.7    17.81092337     -1129.6855558578 
> -3.32E+02
>    274 P_Mix/Diag. 0.40E+00  104.0    37.49112643     -1041.2092735401  
> 8.85E+01
>    275 P_Mix/Diag. 0.40E+00  101.8    21.82778389      -871.8048612001  
> 1.69E+02
>    276 P_Mix/Diag. 0.40E+00  103.5    23.07273707     -1069.6977429739 
> -1.98E+02
>    277 P_Mix/Diag. 0.40E+00   99.6    11.15719347      -892.6777804895  
> 1.77E+02
>    278 P_Mix/Diag. 0.40E+00   97.0    55.40276856     -1199.2438090379 
> -3.07E+02
>    279 P_Mix/Diag. 0.40E+00   99.8    28.66796423      -801.0559779926  
> 3.98E+02
>    280 P_Mix/Diag. 0.40E+00   99.3    17.62940096     -1126.5427122480 
> -3.25E+02
>    281 P_Mix/Diag. 0.40E+00  100.3    41.87172750     -1065.3229743732  
> 6.12E+01
>    282 P_Mix/Diag. 0.40E+00  100.1    21.35136376      -871.9246647736  
> 1.93E+02
>    283 P_Mix/Diag. 0.40E+00   96.2    23.36924083     -1074.9897309855 
> -2.03E+02
>    284 P_Mix/Diag. 0.40E+00  100.0    11.24984392      -906.8454308390  
> 1.68E+02
>    285 P_Mix/Diag. 0.40E+00   98.2    56.07469411     -1247.8500119442 
> -3.41E+02
>    286 P_Mix/Diag. 0.40E+00   96.1    29.44999514      -816.4175279935  
> 4.31E+02
>    287 P_Mix/Diag. 0.40E+00   98.8    17.75235653     -1087.9247857738 
> -2.72E+02
>    288 P_Mix/Diag. 0.40E+00  100.1    35.47297532     -1047.5502720444  
> 4.04E+01
>    289 P_Mix/Diag. 0.40E+00   98.4    20.85623425      -842.2586588867  
> 2.05E+02
>    290 P_Mix/Diag. 0.40E+00   95.5    22.67408867     -1073.0843407892 
> -2.31E+02
>    291 P_Mix/Diag. 0.40E+00  101.9    10.94722146      -860.3065908793  
> 2.13E+02
>    292 P_Mix/Diag. 0.40E+00  104.4    54.21481607     -1193.6159069033 
> -3.33E+02
>    293 P_Mix/Diag. 0.40E+00   99.7    27.38232795      -792.2533438689  
> 4.01E+02
>    294 P_Mix/Diag. 0.40E+00  103.1    16.99902606     -1114.6982782222 
> -3.22E+02
>    295 P_Mix/Diag. 0.40E+00  100.2    41.24936495     -1065.7493384422  
> 4.89E+01
>    296 P_Mix/Diag. 0.40E+00   97.3    20.66030037      -876.2511279178  
> 1.89E+02
>    297 P_Mix/Diag. 0.40E+00  102.7    22.76848352     -1079.0180419796 
> -2.03E+02
>    298 P_Mix/Diag. 0.40E+00   99.6    11.17073523      -894.7854932575  
> 1.84E+02
>    299 P_Mix/Diag. 0.40E+00  102.2    52.05827833     -1215.6511319679 
> -3.21E+02
>    300 P_Mix/Diag. 0.40E+00   98.3    27.88498962      -801.1240827513  
> 4.15E+02
>
>   Leaving inner SCF loop after reaching   300 steps.
>
>
>   Electronic density on regular grids:       -527.9999997528        
> 0.0000002472
>   Core density on regular grids:              527.9999999790      
>  -0.0000000210
>   Total charge density on r-space grids:        0.0000002262
>   Total charge density g-space grids:           0.0000002262
>
>   Overlap energy of the core charge distribution:              
>  0.00014062616239
>   Self energy of the core charge distribution:              
> -3799.25452676640361
>   Core Hamiltonian energy:                                  
>  1439.87930656668232
>   Hartree energy:                                            
> 1853.46940742339507
>   Exchange-correlation energy:                              
>  -295.21841060112149
>
>   Total energy:                                              
> -801.12408275128553
>
>  *** WARNING in qs_scf.F:576 :: SCF run NOT converged ***
>
>
> Thanks
>
>
> Alberto
>
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> .
> <FeCO5.Geo_Opt_cutoff400_PBE.inp>
>
>
>
>
> ==============================
> Thomas D. Kühne
> Dynamics of Condensed Matter
> Chair of Theoretical Chemistry
> University of Paderborn
> Warburger Str. 100
> D-33098 Paderborn
> Germany
> td... at mail.upb.de
> +49/(0)5251/60-5726 <+49%205251%20605726>
>
>
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