MD simulation of glass

Aniruddha Dive anirudd... at gmail.com
Thu Apr 13 22:12:31 UTC 2017


Thanks for your suggestion Matt.

I will try with GAPW

Aniruddha M Dive

On Wednesday, April 12, 2017 at 3:24:15 PM UTC-7, Matt W wrote:
>
> There is no problem using too high a cutoff, apart from performance.
>
> You could try using the GAPW method.
>
> Matt
>
> On Wednesday, April 12, 2017 at 9:28:18 PM UTC+1, Aniruddha Dive wrote:
>>
>> Hi All,
>>
>> I am trying to carry out MD simulation of glass (Na2SiS3) using CP2K. I 
>> am not sure as to what values of Cut - off and Relative Cut - Off should be 
>> suitable for these runs. For Na since it the pseudo potential is semi - 
>> core, I need to use a higher cut off (~ 900Ry). But would using such a high 
>> cut - off have effect on calculations related to Si and S which require a 
>> considerably low cut - off values. Will this high cut - off lead to excited 
>> states calculations of Si and S? I am getting the partial charges on Si to 
>> be negative when I run these calculations. The partial charges I expect on 
>> Si are of the order of +2.4 and on S are -1.2 but I am currently getting 
>> them to be way off from those numbers. Attached hereby is the input file 
>> along with the input coordinate file. 
>>
>>
>> Here is the portion of the Mulliken Charge Analysis from output:
>>
>>
>> !-----------------------------------------------------------------------------!
>>                      Mulliken Population Analysis
>>
>>  #  Atom  Element  Kind  Atomic population                           Net 
>> charge
>>        1     Si       1          4.100719                             
>> -0.100719
>>        2     Si       1          4.045726                             
>> -0.045726
>>        3     Si       1          4.032320                             
>> -0.032320
>>        4     Si       1          4.224169                             
>> -0.224169
>>        5     Si       1          4.165061                             
>> -0.165061
>>        6     Si       1          4.200970                             
>> -0.200970
>>        7     Si       1          4.206992                             
>> -0.206992
>>        8     Si       1          4.119460                             
>> -0.119460
>>        9     Si       1          4.061532                             
>> -0.061532
>>       10     Si       1          4.061220                             
>> -0.061220
>>       11     Si       1          4.200596                             
>> -0.200596
>>       12     Si       1          4.185296                             
>> -0.185296
>>       13     Si       1          4.207879                             
>> -0.207879
>>       14     Si       1          4.227356                             
>> -0.227356
>>       15     Si       1          4.215376                             
>> -0.215376
>>       16     Si       1          4.060717                             
>> -0.060717
>>       17     Si       1          4.382398                             
>> -0.382398
>>       18     Si       1          4.159860                             
>> -0.159860
>>       19     Si       1          4.189585                             
>> -0.189585
>>       20     Si       1          4.036421                             
>> -0.036421
>>       21     Si       1          4.156344                             
>> -0.156344
>>       22     Si       1          4.156304                             
>> -0.156304
>>       23     Si       1          4.245355                             
>> -0.245355
>>       24     Si       1          4.203485                             
>> -0.203485
>>       25     Na       2          8.477253                              
>> 0.522747
>>       26     Na       2          8.695937                              
>> 0.304063
>>       27     Na       2          8.638158                              
>> 0.361842
>>       28     Na       2          8.557866                              
>> 0.442134
>>       29     Na       2          8.578021                              
>> 0.421979
>>       30     Na       2          8.484658                              
>> 0.515342
>>       31     Na       2          8.694122                              
>> 0.305878
>>       32     Na       2          8.416273                              
>> 0.583727
>>       33     Na       2          8.759774                              
>> 0.240226
>>       34     Na       2          8.645345                              
>> 0.354655
>>       35     Na       2          8.624249                              
>> 0.375751
>>       36     Na       2          8.645152                              
>> 0.354848
>>       37     Na       2          8.734614                              
>> 0.265386
>>       38     Na       2          8.655715                              
>> 0.344285
>>       39     Na       2          8.636360                              
>> 0.363640
>>       40     Na       2          8.750006                              
>> 0.249994
>>       41     Na       2          8.722905                              
>> 0.277095
>>       42     Na       2          8.464161                              
>> 0.535839
>>       43     Na       2          8.553667                              
>> 0.446333
>>       44     Na       2          8.432465                              
>> 0.567535
>>       45     Na       2          8.679302                              
>> 0.320698
>>       46     Na       2          8.486568                              
>> 0.513432
>>       47     Na       2          8.622156                              
>> 0.377844
>>       48     Na       2          8.591266                              
>> 0.408734
>>       49     Na       2          8.788040                              
>> 0.211960
>>       50     Na       2          8.617889                              
>> 0.382111
>>       51     Na       2          8.632749                              
>> 0.367251
>>       52     Na       2          8.601660                              
>> 0.398340
>>       53     Na       2          8.471636                              
>> 0.528364
>>       54     Na       2          8.643551                              
>> 0.356449
>>       55     Na       2          8.598352                              
>> 0.401648
>>       56     Na       2          8.904097                              
>> 0.095903
>>       57     Na       2          8.608580                              
>> 0.391420
>>       58     Na       2          8.874381                              
>> 0.125619
>>       59     Na       2          8.482866                              
>> 0.517134
>>       60     Na       2          8.637200                              
>> 0.362800
>>       61     Na       2          8.760227                              
>> 0.239773
>>       62     Na       2          8.493302                              
>> 0.506698
>>       63     Na       2          8.718374                              
>> 0.281626
>>       64     Na       2          8.990367                              
>> 0.009633
>>       65     Na       2          8.711820                              
>> 0.288180
>>       66     Na       2          8.710667                              
>> 0.289333
>>       67     Na       2          8.519989                              
>> 0.480011
>>       68     Na       2          8.506799                              
>> 0.493201
>>       69     Na       2          8.603574                              
>> 0.396426
>>       70     Na       2          8.707061                              
>> 0.292939
>>       71     Na       2          8.649891                              
>> 0.350109
>>       72     Na       2          8.573187                              
>> 0.426813
>>       73     S        3          6.413211                             
>> -0.413211
>>       74     S        3          5.934268                              
>> 0.065732
>>       75     S        3          6.036948                             
>> -0.036948
>>       76     S        3          6.321484                             
>> -0.321484
>>       77     S        3          5.974429                              
>> 0.025571
>>       78     S        3          6.303399                             
>> -0.303399
>>       79     S        3          6.517641                             
>> -0.517641
>>       80     S        3          6.336776                             
>> -0.336776
>>       81     S        3          6.272697                             
>> -0.272697
>>       82     S        3          5.857828                              
>> 0.142172
>>       83     S        3          5.883922                              
>> 0.116078
>>       84     S        3          6.311134                             
>> -0.311134
>>       85     S        3          6.810646                             
>> -0.810646
>>       86     S        3          6.113015                             
>> -0.113015
>>       87     S        3          6.168490                             
>> -0.168490
>>       88     S        3          6.256089                             
>> -0.256089
>>       89     S        3          6.301347                             
>> -0.301347
>>       90     S        3          5.947002                              
>> 0.052998
>>       91     S        3          6.288852                             
>> -0.288852
>>       92     S        3          6.156621                             
>> -0.156621
>>       93     S        3          6.250532                             
>> -0.250532
>>       94     S        3          6.445222                             
>> -0.445222
>>       95     S        3          6.014573                             
>> -0.014573
>>       96     S        3          6.454676                             
>> -0.454676
>>       97     S        3          6.179396                             
>> -0.179396
>>       98     S        3          5.887622                              
>> 0.112378
>>       99     S        3          6.366055                             
>> -0.366055
>>      100     S        3          5.951562                              
>> 0.048438
>>      101     S        3          6.276227                             
>> -0.276227
>>      102     S        3          6.193922                             
>> -0.193922
>>      103     S        3          6.016116                             
>> -0.016116
>>      104     S        3          6.464048                             
>> -0.464048
>>      105     S        3          6.167156                             
>> -0.167156
>>      106     S        3          5.933141                              
>> 0.066859
>>      107     S        3          6.012865                             
>> -0.012865
>>      108     S        3          6.157836                             
>> -0.157836
>>      109     S        3          6.152618                             
>> -0.152618
>>      110     S        3          6.329449                             
>> -0.329449
>>      111     S        3          6.046476                             
>> -0.046476
>>      112     S        3          6.178587                             
>> -0.178587
>>      113     S        3          6.045632                             
>> -0.045632
>>      114     S        3          6.232212                             
>> -0.232212
>>      115     S        3          6.381129                             
>> -0.381129
>>      116     S        3          6.002099                             
>> -0.002099
>>      117     S        3          6.031752                             
>> -0.031752
>>      118     S        3          6.134130                             
>> -0.134130
>>      119     S        3          5.983090                              
>> 0.016910
>>      120     S        3          6.431342                             
>> -0.431342
>>      121     S        3          6.332564                             
>> -0.332564
>>      122     S        3          6.245917                             
>> -0.245917
>>      123     S        3          6.008792                             
>> -0.008792
>>      124     S        3          6.028775                             
>> -0.028775
>>      125     S        3          6.148420                             
>> -0.148420
>>      126     S        3          6.381323                             
>> -0.381323
>>      127     S        3          6.198058                             
>> -0.198058
>>      128     S        3          6.344164                             
>> -0.344164
>>      129     S        3          6.094589                             
>> -0.094589
>>      130     S        3          6.028368                             
>> -0.028368
>>      131     S        3          6.399015                             
>> -0.399015
>>      132     S        3          6.092985                             
>> -0.092985
>>      133     S        3          6.263275                             
>> -0.263275
>>      134     S        3          6.430725                             
>> -0.430725
>>      135     S        3          6.339478                             
>> -0.339478
>>      136     S        3          6.226800                             
>> -0.226800
>>      137     S        3          6.467115                             
>> -0.467115
>>      138     S        3          6.031300                             
>> -0.031300
>>      139     S        3          6.082477                             
>> -0.082477
>>      140     S        3          5.936620                              
>> 0.063380
>>      141     S        3          6.067240                             
>> -0.067240
>>      142     S        3          5.926741                              
>> 0.073259
>>      143     S        3          6.531579                             
>> -0.531579
>>      144     S        3          6.271021                             
>> -0.271021
>>  # Total charge                            960.000000                 
>> -0.000000
>>
>> Kindly let me know what can I do to resolve the issue.
>>
>> Thanking you,
>>
>> Regards,
>> Aniruddha M Dive
>> PhD Candidate
>> Washington State University
>>
>
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