Error when running geo_opt

Eric Shamay eric.... at gmail.com
Mon Aug 10 23:50:41 UTC 2009


Yes, this works well. It was indeed the starting geometry.

Thanks for the help!

On Aug 7, 4:57 pm, Axel <akoh... at gmail.com> wrote:
> On Aug 7, 4:53 pm, Eric Shamay <eric.... at gmail.com> wrote:
>
> > Toe,
>
> > Thanks for looking into this. The geometry is very wrong - it's only a
> > prelim guess of the perfluorodecyl silane that I was hoping to relax
> > and minimize using cp2k. I will try to find a better starting geometry
> > to work with than what I have and see if that fixes it all up.
>
> why don't you just relax it with a minimal classical force field?
> just using parameters as if all heavy atoms were carbons should
> do the trick. then you have better starting geometry without overlap
> of the cores, which is probably the reason for the failure you are
> seeing with QS.
>
> axel.
>
>
>
> > Thanks!
> > ~Eric
>
> > On Aug 7, 12:09 pm, Teodoro Laino <teodor... at gmail.com> wrote:
>
> > > Hi Eric,
>
> > > this error had nothing to do with GEO_OPT.
>
> > > The geometry of your system looks a bit weird.. are you sure it is ok
> > > (see the nice arrow in the pic ;-) )?!
>
> > > Anyway, the error you get is the effect of some linear dependence at the
> > > basis set level (or geometry totally wrong).
> > > If the geometry is correct, try to use the MOLOPT basis set. It should
> > > behave better for these kind of problems (possibly even with
> > > the arrow one ;-) )
>
> > > Teo
>
> > > Eric Shamay wrote:
> > > > Hello cp2k,
>
> > > > I'm running into trouble when trying to do a GEO_OPT run. I'm posting
> > > > the input file and the tail of the error produced down below. If
> > > > anyone has run into this type of problem before I'd appreciate your
> > > > insight.
>
> > > > ****************************************** input file
> > > > **************************************
>
> > > > &FORCE_EVAL
> > > >   METHOD Quickstep
> > > >   &DFT
> > > >     EXCITATIONS TDDFPT
> > > >     LSD
> > > >     &MGRID
> > > >       CUTOFF 150
> > > >       NGRIDS 4
> > > >       REL_CUTOFF 40
> > > >     &END MGRID
> > > >     &QS
> > > >     &END QS
> > > >     &SCF
> > > >       &OUTER_SCF
> > > >          EPS_SCF 3.0E-5
> > > >       &END OUTER_SCF
> > > >       EPS_SCF 1.0E-5
> > > >       MAX_SCF 200
> > > >       &MIXING
> > > >         METHOD DIRECT_P_MIXING
> > > >         ALPHA 0.2
> > > >       &END
> > > >       SCF_GUESS ATOMIC
> > > >      &OT T
> > > >          MINIMIZER CG
> > > >          PRECONDITIONER FULL_ALL
> > > >          ENERGY_GAP 0.500  # make larger if poor initial guess on the
> > > > preconditioner
> > > >       &END OT
> > > >     &END SCF
> > > >     &XC
> > > >      &XC_GRID
> > > >         XC_DERIV SPLINE2_SMOOTH
> > > >         XC_SMOOTH_RHO NN10
> > > >       &END XC_GRID
> > > >       &XC_FUNCTIONAL BLYP
> > > >         &PADE
> > > >         &END PADE
> > > >       &END XC_FUNCTIONAL
> > > >     &END XC
> > > >     &TDDFPT
> > > >       INVERT_S Y
> > > >       KERNEL Y
> > > >       MAX_KV 60
> > > >       NEV 3
> > > >       OE_CORR NONE
> > > >       PRECOND N
> > > >       REORTHO 2
> > > >       RES_ETYPE SINGLETS
> > > >       RESTARTS 4
> > > >    &END TDDFPT
> > > >    BASIS_SET_FILE_NAME /home/eric/cp2k/tests/QS/GTH_BASIS_SETS
> > > >    POTENTIAL_FILE_NAME /home/eric/cp2k/tests/QS/POTENTIAL
> > > >   &END DFT
> > > >   &SUBSYS
> > > >     &CELL
> > > >       ABC 15.0 10.0 10.0
> > > >      PERIODIC XYZ
> > > >     &END CELL
> > > >     &COORD
> > > >   C          1.344000        0.000000        0.000000
> > > >   F          0.000000        0.000000        0.000000
> > > >   F          1.344000        1.344000        0.000000
> > > >   F          1.344000       -1.344000        0.000000
> > > >   C          2.688000        0.000000        0.000000
> > > >   F          2.688000        1.344000        0.000000
> > > >   F          2.688000       -1.344000        0.000000
> > > >   C          4.032000        0.000000        0.000000
> > > >   F          4.032000        1.344000        0.000000
> > > >   F          4.032000       -1.344000        0.000000
> > > >   C          5.376000        0.000000        0.000000
> > > >   F          5.376000        1.344000        0.000000
> > > >   F          5.376000       -1.344000        0.000000
> > > >   C          6.720000        0.000000        0.000000
> > > >   F          6.720000        1.344000        0.000000
> > > >   F          6.720000       -1.344000        0.000000
> > > >   C          8.064000        0.000000        0.000000
> > > >   F          8.064000        1.344000        0.000000
> > > >   F          8.064000       -1.344000        0.000000
> > > >   C          9.408000        0.000000        0.000000
> > > >   F          9.408000        1.344000        0.000000
> > > >   F          9.408000       -1.344000        0.000000
> > > >   C         10.752000        0.000000        0.000000
> > > >   F         10.752000        1.344000        0.000000
> > > >   F         10.752000       -1.344000        0.000000
> > > >   C         12.096000        0.000000        0.000000
> > > >   H         12.096000        1.344000        0.000000
> > > >   H         12.096000       -1.344000        0.000000
> > > >   C         13.440000        0.000000        0.000000
> > > >   H         13.440000        1.344000        0.000000
> > > >   H         13.440000       -1.344000        0.000000
> > > >   Si        14.500000        0.000000        0.000000
> > > >    &END COORD
> > > >     &KIND H
> > > >       BASIS_SET TZV2P-GTH
> > > >       POTENTIAL GTH-BLYP-q1
> > > >     &END KIND
> > > >     &KIND C
> > > >       BASIS_SET TZV2P-GTH
> > > >       POTENTIAL GTH-BLYP-q4
> > > >      MASS 2.0
> > > >     &END KIND
> > > >     &KIND F
> > > >       BASIS_SET TZV2P-GTH
> > > >       POTENTIAL GTH-BLYP-q7
> > > >     &END KIND
> > > >     &KIND Si
> > > >       BASIS_SET TZV2P-GTH
> > > >       POTENTIAL GTH-BLYP-q4
> > > >     &END KIND
> > > >   &END SUBSYS
> > > > &END FORCE_EVAL
> > > > &GLOBAL
> > > >   PROJECT_NAME pds-geo-opt
> > > >   RUN_TYPE GEO_OPT
> > > >   PRINT_LEVEL LOW
> > > >   PREFERRED_FFT_LIBRARY FFTW
> > > > &END GLOBAL
>
> > > > *******************************************************************************************
> > > > ******************************************* error output
> > > > *********************************
>
> > > >  SCF PARAMETERS         Density
> > > > guess:                                    ATOMIC
>
> > > > --------------------------------------------------------
>
> > > > max_scf:                                             200
>
> > > > max_scf_history:                                       0
>
> > > > max_diis:                                              4
>
> > > > --------------------------------------------------------
>
> > > > eps_scf:                                        1.00E-05
>
> > > > eps_scf_history:                                0.00E+00
>
> > > > eps_diis:                                       1.00E-01
>
> > > > eps_eigval:                                     1.00E-05
>
> > > > --------------------------------------------------------
> > > >                         level_shift
> > > > [a.u.]:                                 0.00
>
> > > > --------------------------------------------------------
> > > >                         Outer loop SCF in use
> > > >                         No variables optimised in outer loop
>
> > > > eps_scf                                         3.00E-05
>
> > > > max_scf                                               50
> > > >                         No outer loop optimization
>
> > > > step_size                                       5.00E-01
>
> > > >  2D_MC| Monte Carlo annealing to optimize the distribution_2d
> > > >  2D_MC| Number of
> > > > moves                                                   400000
> > > >  2D_MC| Number of annealing
> > > > cycles                                            10
> > > >  2D_MC| Number of reduction steps per
> > > > cycle                                    5
> > > >  2D_MC| Reduction factor per step
> > > > 0.8000000000
> > > >  2D_MC| Termination tolerance
> > > > 0.0200000000
> > > >  2D_MC| Maximum temperature
> > > > 0.5000000000
> > > >  2D_MC| Swap probability
> > > > 0.9000000000
> > > >  2D_MC| Number of processor
> > > > rows                                               1
> > > >  2D_MC| Number of processor
> > > > cols                                               1
> > > >  2D_MC| Number of
> > > > elements                                                    32
> > > >  2D_MC| What do we minimize                                 SMALLEST
> > > > MAXIMUM
> > > >  2D_MC| Cost of optimal
> > > > distribution                                      219490
> > > >  2D_MC| Cost of found
> > > > distribution                                        219490
> > > >  2D_MC| Difference in
> > > > percent                                                  0
>
> > > > *******************************************************************************
> > > >  ***                     STARTING GEOMETRY
> > > > OPTIMIZATION                      ***
> > > >  ***
> > > > BFGS                                  ***
>
> > > > *******************************************************************************
>
> > > >  Spin 1
>
> > > >  Number of electrons:                              84
> > > >  Number of occupied orbitals:                      84
> > > >  Number of molecular orbitals:                     84
>
> > > >  Spin 2
>
> > > >  Number of electrons:                              83
> > > >  Number of occupied orbitals:                      83
> > > >  Number of molecular orbitals:                     83
>
> > > >  Number of orbital functions:                     652
> > > >  Number of independent orbital functions:         652
>
> > ...
>
> > read more »


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